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We construct two strong-field path integral methods with full Coulomb distortion, in which the quantum pathways are mimicked by interfering electron orbits: the rate-based CQSFA (R-CQSFA) and the hybrid forward-boundary CQSFA (H-CQSFA). The…

We perform a detailed analysis of the different types of orbits in the Coulomb Quantum Orbit Strong-field Approximation (CQSFA), ranging from direct to those undergoing hard collisions. We show that some of them exhibit clear counterparts…

原子物理 · 物理学 2018-06-13 A. S. Maxwell , C. Figueira de Morisson Faria

We provide approximate analytic expressions for above-threshold ionization (ATI) transition probabilities and photoelectron angular distributions (PADs). These analytic expressions are more general than those existing in the literature and…

原子物理 · 物理学 2018-02-14 A. S. Maxwell , A. Al-Jawahiry , X. Y. Lai , C. Figueira de Morisson Faria

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

原子物理 · 物理学 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

Holography relies on the interference between a known reference and a signal of interest to reconstruct both the amplitude and phase of that signal. Commonly performed with photons and electrons, it finds numerous applications in imaging,…

Using the recently developed Coulomb Quantum Orbit Strong-Field Approximation (CQSFA), we perform a systematic analysis of several features encountered in above-threshold ionization (ATI) photoelectron angle-resolved distributions (PADs),…

原子物理 · 物理学 2017-10-11 A. S. Maxwell , A. Al-Jawahiry , T. Das , C. Figueira de Morisson Faria

Holography is a cornerstone characterisation and imaging technique that can be applied to the full electromagnetic spectrum, from X-rays to radio waves or even particles such as neutrons. The key property in all these holographic approaches…

量子物理 · 物理学 2021-01-12 Hugo Defienne , Bienvenu Ndagano , Ashley Lyons , Daniele Faccio

Parity violating elastic electron-nucleus scattering provides an accurate and model independent measurement of neutron densities, because the $Z^0$ couples primarily to neutrons. Coulomb distortion corrections to the parity violating…

核理论 · 物理学 2009-09-25 C. J. Horowitz

High harmonic generation in the interaction of femtosecond lasers with atoms and molecules opens the path to molecular orbital tomography and to probe the electronic dynamics with attosecond-{\AA}ngstr\"{o}m resolutions. Molecular orbital…

We study photoelectron angular distributions (PADs) near the ionization threshold with a newly developed Coulomb quantum-orbit strong-field approximation (CQSFA) theory. The CQSFA simulations present an excellent agreement with the result…

Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the…

原子物理 · 物理学 2016-02-22 Xiaohong Song , Cheng Lin , Zhihao Sheng , Peng Liu , Zhangjin Chen , Weifeng Yang , Shilin Hu , C. D. Lin , Jing Chen

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Strong-field photoelectron holography denotes the interference of various electron paths in laser-induced ionization of atoms, leading to interference patterns in the final momentum distribution. For a quantitative description of holography…

原子物理 · 物理学 2019-08-28 Simon Brennecke , Manfred Lein

Most implementations of Coulomb-distorted strong-field approaches that contain features such as tunneling and quantum interference use real trajectories in continuum propagation, while a fully consistent approach must use complex…

原子物理 · 物理学 2018-12-26 A. S. Maxwell , S. V. Popruzhenko , C. Figueira de Morisson Faria

Quantum interference between multiple pathways in molecular photodissociation often results in angular momentum polarization of atomic products and this can give deep insight into fundamental physical processes. For dissociation of diatomic…

化学物理 · 物理学 2022-04-26 Chaya Weeraratna , Arthur G. Suits , Oleg S. Vasyutinskii

The quantitative analysis of electron-optical phase images recorded using off-axis electron holography often relies on the use of computer simulations of electron propagation through a sample. However, simulations that make use of the…

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

原子物理 · 物理学 2017-03-08 Lisa Torlina , Olga Smirnova

Photoemission orbital tomography (POT) from photoelectron momentum maps (PMMs) has enabled detailed analysis of the shape and energy of molecular orbitals in the adsorbed state. This study proposes a new POT method based on the PhaseLift.…

材料科学 · 物理学 2025-06-03 Kaori Niki , Rena Asano , Ryuji Sakanoue , Manabu Hagiwara , Kazushi Mimura
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