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Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

Tailoring the properties of correlated oxides is accomplished by chemical doping, pressure, temperature or magnetic field. Photoexcitation is a valid alternative to reach out-of-equilibrium states otherwise inaccessible. Here, we…

Coherent control is an optical technique to manipulate quantum states of matter. The coherent control of 40-THz optical phonons in diamond was demonstrated by using a pair of sub-10-fs optical pulses. The optical phonons were detected via…

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…

We propose a kinetic model of transient nonequilibrium phenomena in metals exposed to ultrashort laser pulses when heated electrons affect the lattice through direct electron-phonon interaction. This model describes the destruction of a…

统计力学 · 物理学 2009-10-31 L. A. Falkovsky , E. G. Mishchenko

Charge density waves (CDW) and their concomitant periodic lattice distortions (PLD) govern the electronic properties in many layered transition-metal dichalcogenides. In particular, 1T-TaS2 undergoes a metal-to-insulator phase transition as…

We report our study on unconventional charge density waves (UCDW) (i.e. a charge density wave with wavevector dependent gap) in pure quasi-one dimensional conductors. We develop a new possible mechanism of establishment of such a low…

强关联电子 · 物理学 2009-11-11 András Ványolos , Balázs Dóra , Attila Virosztek

Charge-density wave (CDW) is one of the most fundamental quantum phenomena in solids. Different from ordinary metals in which only single particle excitations exist, CDW also has collective excitations and can carry electric current in a…

A practical approach is proposed for efficiently generating ultrashort attosecond pulses (APs) from realistic solid-state materials, aiming to optimize pulse width effectively. By adjusting the photon energy while maintaining a constant…

光学 · 物理学 2025-02-25 Xinyuan Zhang , Shiqi Hu , Mengxue Guan , Sheng Meng

Monolayer 2D semiconductors, such as WS2, exhibit uniquely strong light-matter interactions due to exciton resonances that enable atomically-thin optical elements. Similar to geometry-dependent plasmon and Mie resonances, these intrinsic…

Ultrafast laser material processing has received significant attention due to a growing need for the fabrication of miniaturized devices at micro- and nanoscales. The traditional phenomenological laws, such as Fourier's law of heat…

计算物理 · 物理学 2015-11-12 Yuwen Zhang , D. Y. Tzou , J. K. Chen

Ultrafast optical switching of materials properties is of great relevance both for future technological applications as well as gaining fundamental physical insights to microscopic couplings and nonequilibrium phenomena. Transition-metal…

材料科学 · 物理学 2024-10-04 Till Domröse , Claus Ropers

Revealing the interactions binding electronic and lattice components of cooperative quantum order is central to sculpting new states of matter. This challenge is epitomized by the charge density wave material 1T-TiSe$_2$, where…

Controlling light polarization is one of the most essential routines in modern optical technology. Since the demonstration of optical pulse shaping by spatial light modulators and its potential in controlling the quantum reaction pathways,…

We present measurements of the pulse length of ultracold electron bunches generated by near-threshold two-photon photoionization of a laser-cooled gas. The pulse length has been measured using a resonant $3$ GHz deflecting cavity in…

原子物理 · 物理学 2017-03-24 J. G. H. Franssen , T. L. I. Frankort , E. J. D. Vredenbregt , O. J. Luiten

First principles-based predictions of lattice thermal conductivity (TC) from perturbation theory have achieved significant success. Usually, it only included three-phonon (3ph) scattering processes, only recently four-phonon (4ph)…

材料科学 · 物理学 2025-03-25 H. F. Feng , B. Liu , Xin-Gao Gong , Zhi-Xin Guo

Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Ultrafast optical excitation in charge-density wave (CDW) crystals can transiently suppress long-range order, driving the lattice toward higher symmetry on femtosecond timescales. Here, we formulate and implement a first-principles theory…

材料科学 · 物理学 2026-04-13 Christoph Emeis , Fabio Caruso

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…