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Underlying physical principles for the high efficiency of excitation energy transfer in light-harvesting complexes are not fully understood. Notably, the degree of robustness of these systems for transporting energy is not known considering…

量子物理 · 物理学 2015-03-19 Masoud Mohseni , Alireza Shabani , Seth Lloyd , Herschel Rabitz

Plasmonic antennas offer promising opportunities to control the emission of quantum objects. As a consequence, the fluorescence enhancement factor is widely used as a figure of merit for a practical antenna realization. However, the…

光学 · 物理学 2011-09-26 Jerome Wenger

The fundamental physical mechanisms of energy transfer in photosynthetic complexes is not yet fully understood. In particular, the degree of efficiency or sensitivity of these systems for energy transfer is not known given their…

量子物理 · 物理学 2013-05-30 Alireza Shabani , Masoud Mohseni , Herschel Rabitz , Seth Lloyd

The time-development of photoexcitations in molecular aggregates exhibits specific dynamics of electronic states and vibrational wavefunction. We discuss the dynamical formation of entanglement between electronic and vibrational degrees of…

量子物理 · 物理学 2007-05-23 Dmitri S. Kilin , Jeffrey A. Cina , Oleg V. Prezhdo

We present in this contribution a theoretical investigation of the spontaneous emission and energy transfer rates between quantum systems placed above a monolayer of conducting graphene. The conditions for strong and weak coupling between a…

Phototrophic organisms such as plants, photosynthetic bacteria and algae use microscopic complexes of pigment molecules to absorb sunlight. Within the light-harvesting complexes, which frequently have several functional and structural…

Understanding the mechanisms of efficient and robust energy transfer in light-harvesting systems provides new insights for the optimal design of artificial systems. In this paper, we use the Fenna-Matthews-Olson (FMO) protein complex and…

化学物理 · 物理学 2011-09-27 Jianlan Wu , Fan Liu , Young Shen , Jianshu Cao , Robert J. Silbey

The interplay between coherence and system-environment interactions is at the basis of a wide range of phenomena, from quantum information processing to charge and energy transfer in molecular systems, biomolecules, and photochemical…

量子物理 · 物理学 2025-11-30 Diego Fallas Padilla , Visal So , Abhishek Menon , Roman Zhuravel , Han Pu , Guido Pagano

Energy transfer from photoexcited zero-dimensional systems to metallic systems plays a prominent role in modern day materials science. A situation of particular interest concerns the interaction between a photoexcited dipole and an…

化学物理 · 物理学 2013-04-30 Zheyuan Chen , Stéphane Berciaud , Colin Nuckolls , Tony F. Heinz , Louis E. Brus

For many of the envisioned optoelectronic applications of graphene it is crucial to understand the sub-picosecond carrier dynamics immediately following photoexcitation, as well as the effect on the electrical conductivity - the…

We theoretically analyze the excitation energy transfer between two closely spaced linear molecular J-aggregates, whose excited states are Frenkel excitons. The aggregate with the higher (lower) exciton band edge energy is considered as the…

无序系统与神经网络 · 物理学 2007-05-23 C. Didraga , V. A. Malyshev , J. Knoester

The kinetic transport of electrons through graphene magnetic barriers is studied theoretically in presence of an external time harmonic scalar potential. The transmission coefficients are calculated in the framework of the non-perturbative…

介观与纳米尺度物理 · 物理学 2017-04-26 R. Biswas , S. Maiti , C. Sinha

We extend the conventional transfer matrix method to include anisotropic features for electron transmission in two-dimensional materials, such as breaking reflection law in pseudo-spin phases and wave vectors. This method allows to study…

材料科学 · 物理学 2022-12-15 Erik Díaz-Bautista , Yonatan Betancur-Ocampo , Alfredo Raya

We study the transport properties of Dirac fermions through gapped graphene through a magnetic barrier irradiated by a laser field oscillating in time. We use Floquet theory and the solution of Weber's differential equation to determine the…

介观与纳米尺度物理 · 物理学 2023-12-27 Rachid El Aitouni , Miloud Mekkaoui , Ahmed Jellal , Michael Schreiber

It is shown that thermally excited plasmon-polariton modes can strongly mediate, enhance and \emph{tune} the near-field radiation transfer between two closely separated graphene sheets. The dependence of near-field heat exchange on doping…

介观与纳米尺度物理 · 物理学 2013-05-30 Ognjen Ilic , Marinko Jablan , John D. Joannopoulos , Ivan Celanovic , Hrvoje Buljan , Marin Soljačić

We analyze a theoretical model for energy and electron transfer in an artificial photosynthetic system. The photosystem consists of a molecular triad (i.e., with a donor, a photosensitive unit, and an acceptor) coupled to four accessory…

生物物理 · 物理学 2015-05-20 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

We report high time-resolution measurements of photon statistics from pairs of dye molecules coupled by fluorescence resonance energy transfer (FRET). In addition to quantum-optical photon antibunching, we observe photon bunching on a…

凝聚态物理 · 物理学 2009-11-07 Andrew J. Berglund , Andrew C. Doherty , Hideo Mabuchi

Giant strides in ultrashort laser pulse technology have enabled real-time observation of dynamical processes in complex molecular systems. Specifically, the discovery of oscillatory transients in the two-dimensional electronic spectra of…

化学物理 · 物理学 2021-03-08 Akihito Ishizaki , Graham R. Fleming

We demonstrate that longitudinal plasmons in doped monolayer graphene can mediate highly efficient long-range energy transfer between nearby fluorophores, e.g., semiconductor quantum dots. We derive a simple analytical expression for the…

介观与纳米尺度物理 · 物理学 2015-06-11 Kirill A. Velizhanin , Tigran V. Shahbazyan

We investigate multichromophoric energy transfer allowing for bath-induced fluctuations at different sites to be correlated. As a prototype system we consider a light-harvesting antenna surrounding a reaction center. We show that the…

量子物理 · 物理学 2010-07-16 Francesca Fassioli , Ahsan Nazir , Alexandra Olaya-Castro