关联环境中能量转移的量子态调控
量子物理
2010-07-16 v2
摘要
我们研究了多色素能量转移，允许不同位点的浴致涨落相互关联。作为一个原型系统，我们考虑一个围绕反应中心的光捕获天线。我们证明，量子相干性与关联涨落之间的相互作用可以产生一个室温转移过程，该过程表现出对初始激子态对称性和离域程度的显著依赖性。我们的工作阐明了这些量子特征如何支持在紧密堆积的自然和人工光捕获复合物中精细调控能量转移效率。
引用
@article{arxiv.0907.5183,
title = {Quantum State Tuning of Energy Transfer in a Correlated Environment},
author = {Francesca Fassioli and Ahsan Nazir and Alexandra Olaya-Castro},
journal= {arXiv preprint arXiv:0907.5183},
year = {2010}
}
备注
Version published in JPC Letters. Analysis and conclusions are the same as in the original version but spectral density and reorganization energy considered correspond to more realistic values for the LH1-RC complex