相关论文: Devolatilization of Subducting Slabs, Part II: Vol…
The amount of H$_2$O and CO$_2$ that is carried into deep mantle by subduction beyond subarc depths is of fundamental importance to the deep volatile cycle but remains debated. Given the large uncertainties surrounding the spatio-temporal…
The effects of the hydration mechanism on continental crust recycling are analyzed through a 2D finite element thermo-mechanical model. Oceanic slab dehydration and consequent mantle wedge hydration are implemented using a dynamic method.…
Diffusive transport has implications for the long-term status of underground storage of hydrogen (H$_2$) fuel and carbon dioxide (CO$_2$), technologies which are being pursued to mitigate climate change and advance the energy transition.…
The oceanic mantle lithosphere has considerable potential to store chemically bound water, thereby being an important factor for the deep water cycle. However, the actual extent of hydrous alteration in such mantle rocks is debated.…
The dissolution and subsequent mass transfer of carbon dioxide gas into liquid barriers plays a vital role in many environmental and industrial applications. In this work, we study the downward dissolution and propagation dynamics of CO2…
Aims: The long-term carbon cycle for planets with a surface entirely covered by oceans works differently from that of the present-day Earth because inefficient erosion leads to a strong dependence of the weathering rate on the rate of…
Biphasic interfaces are complex but fascinating regimes that display a number of properties distinct from those of the bulk. The CO$_2$-H$_2$O interface, in particular, has been the subject of a number of studies on account of its…
The density-driven convection coupled with chemical reaction is the preferred mechanism for permanently storing CO2 in saline aquifers. This study uses a 2D visual Hele-Shaw cell to evaluate and visualize the density-driven convection…
Volatile elements - those that vaporize at low temperatures - are depleted in lunar rocks relative to terrestrial rocks. This systematic chemical depletion is evidence for vaporization and preferential removal of vapor from proto-lunar…
An understanding of the CO$_2$ + H$_2$O hydration reaction is crucial for modeling the effects of ocean acidification, for enabling novel carbon storage solutions, and as a model process in the geosciences. While the mechanism of this…
We numerically examine solutal convection in porous media, driven by the dissolution of carbon dioxide (CO2) into water---an effective mechanism for CO2 storage in saline aquifers. Dissolution is associated with slow diffusion of free-phase…
$\text{CO}_{2}$ flooding is central to carbon utilization technologies, yet conventional waterflooding models fail to capture the complex interactions between CO$_2$ and formation fluids. In this study, one- and two-dimensional nuclear…
Experimental studies of mantle petrology find that small concentrations of water and carbon dioxide have a large effect on the solidus temperature and distribution of melting in the upper mantle. However, it has remained unclear what effect…
The photoconversion of CO$_2$ to hydrocarbons is a sustainable route to its transformation into value-added compounds and, thereby, crucial to mitigating the energy and climate crises. CuPt nanoparticles on TiO$_2$ surfaces have been…
The complex interplay between the growth, drift, and sublimation of ice-covered pebbles can strongly influence the volatile distribution and evolution of disc composition, and therefore impact the composition of forming planets. Classic…
A comprehensive phase diagram of lowest-energy structures and compositions of the rutile TiO_2(110) surface in equilibrium with a surrounding gas phase at finite temperatures and pressures has been determined using density functional theory…
We present the first experiments of dissolution-driven convection of carbon dioxide (CO$_2$) in a confined brine-saturated porous medium at high pressures. We designed a novel Hele-Shaw cell that allows for both visual and quantitative…
Magmatism and volcanism transfer carbon from the solid Earth into the climate system. This transfer may be modulated by the glacial/interglacial cycling of water between oceans and continental ice sheets, which alters the surface loading of…
Massive steam and CO$_2$ atmospheres have been proposed for magma ocean outgassing of Earth and terrestrial planets. Yet formation of such atmospheres depends on volatile exchange with the molten interior, governed by volatile solubilities…
Radiative cooling by molecules is a crucial process for hydrodynamic escape, as it can efficiently remove the thermal energy driving the outflow, acquired through X-ray and extreme UV absorption. Carbon oxides, such as CO and CO2, and their…