相关论文: Cavity-modified exciton dynamics in photosynthetic…
Polaritonic states arise when a bright optical transition of a molecular ensemble is resonantly matched to an optical cavity mode frequency. Here, we lay the groundwork to study the behavior of polaritons in clean, isolated systems by…
Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…
Coupled states of semiconductor quantum well (QW) excitons and photons in a two dimensional (2D) periodic lattice of microcavities are analyzed theoretically, revealing allowed bands and forbidden gaps in the energy spectrum of exciton…
A minimal, one-parameter model of the excitonic Hamiltonian for the light harvesting complex of purple bacteria (LH2) based on ab initio calculation of the excitonic energies is proposed. The set of input parameters contains positions of…
We study a hybrid system formed from an optomechanical resonator and a cavity mode strongly coupled to an excitonic transition inside a quantum well. We show that due to the mixing of cavity photon and exciton states, the emergent…
Carrier multiplication by singlet exciton fission enhances photovoltaic conversion efficiencies in organic solids. This decay of one singlet exciton into two triplet states promises to overcome the Shockley-Queisser limit as up to two…
Exciton-polaritons - hybrid light-matter quasiparticles - can undergo Bose-Einstein-like condensation at elevated temperatures owing to their lower effective mass. This becomes even more pronounced in the context of molecular polariton…
A theoretical description of radiation-matter coupling for semiconductor-based photonic crystal slabs is presented, in which quantum wells are embedded within the waveguide core layer. A full quantum theory is developed, by quantizing both…
The quantum dynamics of entanglement is widely revealed in photosynthetic light-harvesting complexes. Different from the previous work, we explore the properties of exciton transport and photosynthesis assisted by the quantum entanglement…
Strong interaction between light and a single quantum emitter is essential to a great number of applications, including single photon sources. Microcavities and plasmonic antennas have been used frequently to enhance these interactions…
Polaritons - hybrid light-matter states formed from the strong coupling of a bright molecular transition with a confined photonic mode - may offer new opportunities for optical control of molecular behavior. Vibrational strong coupling…
The exploitation of the strong light-matter coupling regime and exciton-polariton condensates has emerged as a compelling approach to introduce strong interactions and nonlinearities into numerous photonic applications, ranging from…
Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…
We propose collective nuclear polaritons formed by hybridizing a 229Th nuclear ensemble with a vacuum-ultraviolet cavity mode generated via four-wave mixing, achieving a collective light-matter coupling that scales as $\sqrt{N}$. In the…
Ultrastrong light-matter coupling has traditionally been studied in optical cavities, where it occurs when the light-matter coupling strength reaches a significant fraction of the transition frequency. This regime fundamentally alters the…
Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are…
Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be…
The quest to realise strongly interacting photons remains an outstanding challenge both for fundamental science and for applications. Here, we explore mediated photon-photon interactions in a highly imbalanced two-component mixture of…
We analyze the properties of strongly coupled excitons and photons in systems made of semiconducting two-dimensional transition-metal dichalcogenides embedded in optical cavities. Through a detailed microscopic analysis of the coupling we…
We study Frenkel exciton-polariton Bose-Einstein condensation in a two-dimensional defect-free triangular photonic crystal with an organic semiconductor active medium containing bound excitons with dipole moments oriented perpendicular to…