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Despite the exciting implications of the Kitaev spin-Hamiltonian, finding and confirming the quantum spin liquid state has proven incredibly difficult. Recently the applicability of the model has been expanded through the development of a…

Theoretical studies have predicted the existence of topological magnons in honeycomb compounds with zig-zag antiferromagnetic (AFM) order. Here we report the discovery of zig-zag AFM order in the layered and non-centrosymmetric honeycomb…

强关联电子 · 物理学 2019-01-23 Jennifer R. Morey , Allen Scheie , John P. Sheckelton , Craig M. Brown , Tyrel M. McQueen

The nature of the effective spin Hamiltonian and magnetic order in the honeycomb iridates is explored by considering a trigonal crystal field effect and spin-orbit coupling. Starting from a Hubbard model, an effective spin Hamiltonian is…

强关联电子 · 物理学 2012-07-10 Subhro Bhattacharjee , Sung-Sik Lee , Yong Baek Kim

The microscopic spin-spin correlations in the 2D layered spin-1 honeycomb lattice compound Na2Ni2TeO6 have been investigated by neutron diffraction and inelastic neutron scattering. The honeycomb lattice of spin-1 Ni2+ ions, within the…

强关联电子 · 物理学 2022-02-17 A. K. Bera , S. M. Yusuf , L. Keller , F. Yokaichiya , J. R. Stewart

We discuss the ground state of the spin-orbital model for spin-one ions with partially filled $t_{2g}$ levels on a honeycomb lattice. We find that the orbital degrees of freedom induce a spontaneous dimerization of spins and drive them into…

强关联电子 · 物理学 2008-04-12 G. Jackeli , D. I. Khomskii

Motivated by recent experiments on the spin-3/2 frustrated bilayer honeycomb antiferromagnet Bi$_3$Mn$_4$O$_{12}$(NO$_3$), we study the spin-S Heisenberg model on the honeycomb lattice with various additional exchange interactions which…

强关联电子 · 物理学 2013-05-29 R. Ganesh , D. N. Sheng , Young-June Kim , A. Paramekanti

Evidence for multiple magnetic transitions and unconventional spin exchange interactions in the ilmenite insulator MnTiO3 is provided via neutron scattering. On cooling, while G-type antiferromagnetic (AFM) order sets in first at 63 K with…

强关联电子 · 物理学 2026-03-09 Srimal Rathnayaka , Luke Daemen , Despina Louca

Sr$_{3}$ZnIrO$_{6}$ is an effective spin one-half Mott insulating iridate belonging to a family of magnets which includes a number of quasi-one dimensional systems as well as materials exhibiting three dimensional order. Here we present the…

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

强关联电子 · 物理学 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

We have combined single crystal neutron and x-ray diffractions to investigate the magnetic and crystal structures of the honeycomb lattice $\rm Na_2IrO_3$. The system orders magnetically below $18.1(2)$ K with Ir$^{4+}$ ions forming zigzag…

We employ density functional theory within a non-collinear framework to investigate the magnetic properties of the octanuclear molecular rings Cr$_8$ and V$_8$. Our aim is to generalize the evaluation of the effective magnetic interactions…

材料科学 · 物理学 2026-04-28 Maria Barbara Maccioni , Elia Stocco , Luca Binci , Andrea Floris , Matteo Cococcioni

We report thermodynamic properties, magnetic ground state, and microscopic magnetic model of the spin-1 frustrated antiferromaget Li$_{2}$NiW$_{2}$O$_{8}$ showing successive transitions at $T_{\rm N1}\simeq 18$ K and $T_{\rm N2}\simeq 12.5$…

Iridates are characterized by a fascinating interplay of spin-orbit and electron-electron interactions. The honeycomb-lattice materials A2IrO3 (A=Na,Li) have been proposed to realize pseudospin-1/2 Mott insulating states with strongly…

强关联电子 · 物理学 2014-11-11 Eric C. Andrade , Matthias Vojta

The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…

In the Van der Waal material $\rm NiPS_3$, Ni atoms have spin S=1 and realize a honeycomb lattice. Six sulfur atoms surround each Ni and split their d manifold into three filled and two unfilled bands. Aimed to determine the spin…

强关联电子 · 物理学 2023-12-14 Paula Mellado

Motivated by the recent activities on the Ni-based diamond lattice antiferromagnet NiRh$_2$O$_4$, we theoretically explore on a general ground the unique spin and orbital physics for the Ni$^{2+}$ ions with a $3d^8$ electron configuration…

强关联电子 · 物理学 2019-07-10 Fei-Ye Li , Gang Chen

We study the interplay of strong electron correlations and intra-triangle spin exchange at two-thirds filling of the single-orbital Hubbard model on the decorated honeycomb lattice using rotationally invariant slave bosons. We find that the…

强关联电子 · 物理学 2021-08-06 H. L. Nourse , Ross H. McKenzie , B. J. Powell

Recent interest in honeycomb lattice materials has focused on their potential to host quantum spin liquid (QSL) states. Variations in bond angles and spin allow a range of interesting behaviors on this lattice, from the predicted QSL ground…

强关联电子 · 物理学 2021-09-15 Veronica J. Stewart , Juan R. Chamorro , Tyrel M. McQueen

Ni$_{2}$Mo$_{3}$O$_{8}$ is a pyroelectric honeycomb antiferromagnet exhibiting peculiar changes of its electric polarization at magnetic transitions. Ni$_{2}$Mo$_{3}$O$_{8}$ stands out from the isostructural magnetic compounds, showing an…

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