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Our previous work show that in the molecular cluster regime, the band blue shift associated with cluster growth can be understood by a model that assume electrons are confined to a spherical potential well and the clusters are made of some…

化学物理 · 物理学 2019-08-27 John Hongguang Zhang

Based on the theory of the optical properties of fractal clusters, which is an operator-based modification of the coupled-dipole method, an alternate solution is proposed for the problem of adequately describing the evolution of optical…

光学 · 物理学 2007-05-23 S. V. Karpov , A. L. Bas'ko , A. K. Popov , V. V. Slabko , Thomas F. George

Electronic and optical properties of silver clusters were calculated using two different \textit{ab initio} approaches: 1) based on all-electron full-potential linearized-augmented plane-wave method and 2) local basis function…

介观与纳米尺度物理 · 物理学 2016-11-28 John T. Titantah , Mikko Karttunen

The localized surface-plasmon resonances (LSPRs) of coinage-metal clusters and nanoparticles provide the basis for a great number of applications, the conception and necessary optimization of which require precise theoretical description…

材料科学 · 物理学 2024-12-09 Mohit Chaudhary , Hans-Christian Weissker

Electrical properties of multilayer arrays of germanium nanoclusters grown on the silicon (001) surface at low temperature have been studied. A correlation between the quantum dot (QD) density estimated from STM and the charge accumulated…

介观与纳米尺度物理 · 物理学 2009-11-16 O. V. Feklisova , E. B. Yakimov , L. V. Arapkina , V. A. Chapnin , K. V. Chizh , V. P. Kalinushkin , V. A. Yuryev

We have performed systematic large-scale all-electron correlated calculations on boron Bn, aluminum Aln and magnesium Mgn clusters (n=2--5), to study their linear optical absorption spectra. Several possible isomers of each cluster were…

原子与分子团簇 · 物理学 2016-07-26 Ravindra Shinde

Zero-dimensional nanocrystals, as obtained by chemical synthesis, offer a broad range of applications, as their spectrum and thus their excitation gap can be tailored by variation of their size. Additionally, nanocrystals of the type ABC…

介观与纳米尺度物理 · 物理学 2015-05-20 Daniel Mourad , Gerd Czycholl

It is found out that there are physical effects, typical of small metal clusters deposited on a non-adsorbing support, that cause a difference between the adsorption properties of sites at the metal cluster surface and those of sites at the…

统计力学 · 物理学 2007-05-23 Maria K. Koleva , L. A. Petrov

Using classical electrodynamics we determine the angular dependence of the light intensities radiated in second and third harmonic generation by spherical metal clusters. Forward and backward scattering is analyzed in detail. Also resonance…

凝聚态物理 · 物理学 2007-05-23 J. Dewitz , W. Hubner , K. H. Bennemann

Magic-size clusters are ultra-small colloidal semiconductor systems that are intensively studied due to their monodisperse nature and sharp UV-vis absorption peak compared with regular quantum dots. However, the small size of such clusters…

Motivated by recent scanning tunneling microscope (STM) experiments on cobalt clusters adsorbed on single wall metallic nanotubes [Odom {\em et al.}, Science {\bf 290}, 1549 (2000)], we study theoretically the size dependence of STM spectra…

强关联电子 · 物理学 2009-11-07 Gregory A. Fiete , Gergely Zarand , Bertrand I. Halperin , Yuval Oreg

Assemblies of closely separated gold nanoparticles exhibit a strong collective plasmonic response due to coupling of the plasmon modes of the individual nanostructures. In the context of self-assembly of nanoparticles, closed packed 2D…

材料科学 · 物理学 2021-08-05 Rituraj Borah , Sammy W. Verbruggen

Transition-metal nanoclusters exhibit structural and electronic properties that depend on their size, often making them superior to bulk materials for heterogeneous catalysis. However, their performance can be limited by sulfur poisoning.…

The atomic and electronic structure of a set of proposed thin (1.6 nm in diameter) silicon/silica quantum nanodots and nanowires with narrow interface, as well as parent metastable silicon structures (1.2 nm in diameter), was studied in…

The size-dependent structures and optical properties of CdSeS nanoclusters in water medium are investigated. The stability of different size-dependent Cd$_n$Se$_m$S$_p$ nanoclusters (up to n=6) is studied using density functional…

材料科学 · 物理学 2020-11-10 Meenakshi Rana , Papia Chowdhury

Colloidal semiconductor nanocrystals are nanomaterials synthesized in solution. Below a certain size, these nanocrystals acquire quantum confinement properties: their optoelectronic properties depend on the nanoparticle size. In the visible…

应用物理 · 物理学 2019-08-26 Bertille Martinez

Asymmetric double tunnel barriers with the center electrode being a metal cluster in the quantum regime are studied. The zero dimensionality of the clusters used and the associated quantized energy spectra are manifest in well-defined steps…

其他凝聚态物理 · 物理学 2009-11-11 A. Iovan , D. B. Haviland , V. Korenivski

The ground-state electronic, structural, and magnetic properties of small silver clusters, Ag$_n$ (2$\le$n$\le$22), have been studied using a linear combination of atomic Gaussian-type orbitals within the density functional theory. The…

原子与分子团簇 · 物理学 2009-11-11 M. Pereiro , D. Baldomir , J. E. Arias

The fluorescence of silicon clusters is reviewed. Atomic clusters of silicon have been at the focus of research for several decades because of the relevance of size effects for material properties, the importance of silicon in electronics…

原子与分子团簇 · 物理学 2017-09-19 Klaus von Haeften

We develop a quantitative description of giant asymmetry in reflectance, recently observed in semicontinuous metal films. The developed scaling-theory based technique reproduces the spectral properties of semicontinuous composites, as well…

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