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We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

We study the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Ge. We measure RIXS spectra with systematically varying momenta in the final state. The spectra are a measure of exciting an electron-hole pair. We find a single…

材料科学 · 物理学 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi , Hironobu Shoji , Toshiaki Iwazumi

We develop a formalism to calculate the L-edge resonant x-ray scattering (RIXS) spectra from transition-metal compounds. Using a multi-orbital tight-binding model, we derive useful formulas to calculate the spectra by collecting up the…

强关联电子 · 物理学 2015-06-16 Jun-ichi Igarashi , Tatsuya Nagao

We analyze theoretically the resonant inelastic x-ray scattering (RIXS) at the Ni K edge in the stripe-ordered state of La_{2-x}Sr_xNiO_4 at x=1/3. In the calculation of RIXS spectra, the stripe-ordered ground state is described within the…

强关联电子 · 物理学 2012-01-18 Takuji Nomura , Eiji Kaneshita

We present calculations for resonant inelastic x-ray scattering (RIXS) in edge-shared copper oxide systems, such as CuGeO$_{3}$ and Li$_{2}$CuO$_{2}$, appropriate for hard x-ray scattering where the photoexcited electron lies above oxygen…

强关联电子 · 物理学 2009-11-13 F. Vernay , B. Moritz , I. Elfimov , J. Geck , D. Hawthorn , T. P. Devereaux , G. A. Sawatzky

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender x-ray range and have recently become available for…

材料科学 · 物理学 2014-01-08 K. O. Kvashnina , S. M. Butorin

Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…

强关联电子 · 物理学 2015-11-11 Kenji Tsutsui , Eiji Kaneshita , Takami Tohyama

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

The study of elementary bosonic excitations is essential toward a complete description of quantum electronic solids. In this context, resonant inelastic X-ray scattering (RIXS) has recently risen to becoming a versatile probe of electronic…

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

强关联电子 · 物理学 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

The Cu K-edge resonant inelastic x-ray scattering (RIXS) spectrum in one-dimensional insulating cuprates is theoretically examined by using the exact diagonalization technique for the extended one-dimensional Hubbard model with nearest…

强关联电子 · 物理学 2016-08-31 K. Tsutsui , T. Tohyama , S. Maekawa

We study resonant inelastic x-ray scattering (RIXS) peaks corresponding to low energy particle-hole excited states of metallic FeTe and semi-metallic TiSe$_2$ for photon incident energy tuned near the $L_{3}$ absorption edge of Fe and Ti…

材料科学 · 物理学 2014-07-04 B. Barbiellini , J. N. Hancock , C. Monney , Y. Joly , G. Ghiringhelli , L. Braicovich , T. Schmitt

We have used high-resolution resonant inelastic x-ray scattering (RIXS) to study a thin film of NdNiO$_3$, a compound whose unusual spin- and bond-ordered electronic ground state has been of long-standing interest. Below the magnetic…

Element- and site-specific resonant inelastic x-ray scattering spectroscopy (RIXS) is employed to investigate electron correlation effects in {$\rm NaV_2O_5$}. In contrast to single photon techniques, RIXS at the vanadium $L_3$ edge is able…

强关联电子 · 物理学 2009-11-07 G. P. Zhang , T. A. Callcott , G. T. Woods , L. Lin , Brian Sales , D. Mandrus , J. He

We theoretically investigate the origin of the resonant x-ray scattering (RXS) signal near the Ce $L_{III}$ absorption edge in the quadrupolar ordering phase of CeB$_6$, considering the intersite interaction between the $\Gamma_8$ states in…

强关联电子 · 物理学 2009-11-07 Tatsuya Nagao , Jun-ichi Igarashi

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu $K$-edge resonant inelastic X-ray scattering (RIXS) from La$_{2}$CuO$_{4}$. The model includes…

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

强关联电子 · 物理学 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux

This paper makes a comparison between x-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) in the rare earths. Atomic calculations are given for 2p -> 4f and 2p -> 5d XAS. The latter calculation includes the contraction and…

材料科学 · 物理学 2009-10-30 Michel van Veenendaal , Robert Benoist

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

强关联电子 · 物理学 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš
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