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We measured two magnetic modes with finite and discrete energies in an antiferromagnetic ordered phase of a geometrically frustrated magnet MgCr2O4 by single-crystal inelastic neutron scattering, and clarified the spatial spin correlations…

强关联电子 · 物理学 2008-10-22 K. Tomiyasu , H. Suzuki , M. Toki , S. Itoh , M. Matsuura , N. Aso , K. Yamada

In quantum materials, charge orders typically stabilize in specific crystallographic orientations, though their formation mechanisms may vary. Here, using low-temperature scanning tunneling microscopy (STM), we discover a lattice-decoupled…

Strong correlations within a symmetry-unbroken ground-state wavefunction can show up in approximate density functional theory as symmetry-broken spin-densities or total densities, which are sometimes observable. They can arise from soft…

强关联电子 · 物理学 2021-04-28 John P. Perdew , Adrienn Ruzsinszky , Jianwei Sun , Niraj K. Nepal , Aaron D. Kaplan

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

强关联电子 · 物理学 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

强关联电子 · 物理学 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

In this letter we investigated the temperature-dependent Raman spectra of CaMn7O12 helimagnet from room temperature down to 10 K. The temperature dependence of the Raman mode parameters show remarkable anomalies for both antiferromagnetic…

At room temperature, the normal oxide spinels NiCr_2O_4 and CuCr_2O_4 are tetragonally distorted and crystallize in the I4_1/amd space group due to cooperative Jahn-Teller ordering driven by the orbital degeneracy of tetrahedral Ni$^{2+}$…

Intriguing lattice dynamics has been predicted for aperiodic crystals that contain incommensurate substructures. Here we report inelastic neutron scattering measurements of phonon and magnon dispersions in Sr14Cu24O41, which contains…

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

强关联电子 · 物理学 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

Utilizing magnetic susceptibility, specific heat, thermal expansion and IR spectroscopy we provide experimental evidence that the two subsequent antiferromagnetic transitions in ZnCr_2S_4 at T_N1 = 15 K and T_N2= 8 K are accompanied by…

强关联电子 · 物理学 2009-11-11 J. Hemberger , T. Rudolf , H. -A. Krug von Nidda , F. Mayr , A. Pimenov , V. Tsurkan , A. Loidl

We investigate the superconducting properties of Sc$_{5}$Co$_{4}$Si$_{10}$ using low-temperature resistivity, magnetization, heat capacity, and muon-spin rotation and relaxation ($\mu$SR) measurements. We find that Sc$_{5}$Co$_{4}$Si$_{10}$…

The phonon dispersion was measured at room temperature along (0,0,L) in the tetragonal phase of LaFeAsO using inelastic x-ray scattering. Spin-polarized first-principles calculations imposing various types of antiferromagnetic order are in…

The dynamics of electrons, spins and phonons induced by optical femtosecond pulses has been simulated for the polaronic crystal $\rm{Pr_{1/2}Ca_{1/2}MnO_3}$. The model used for the simulation has been derived from first-principles…

强关联电子 · 物理学 2021-06-15 Sangeeta Rajpurohit , Christian Jooss , Peter E. Blöchl

We report a detailed magnetic, dielectric and Raman studies on partially disordered and biphasic double perovskite La2NiMnO6. DC and AC magnetic susceptibility measurements show two magnetic anomalies at TC1 ~ 270 K and TC2 ~ 240 K, which…

材料科学 · 物理学 2015-06-18 Pradeep Kumar , S. Ghara , B. Rajeswaran , D. V. S. Muthu , A. Sundaresan , A. K. Sood

We report a novel crossover behavior in the long-range-ordered phase of a prototypical spin-$1/2$ Heisenberg antiferromagnetic ladder compound $\mathrm{(C_7H_{10}N)_2CuBr_4}$. The staggered order was previously evidenced from a continuous…

强关联电子 · 物理学 2017-04-21 M. Jeong , H. Mayaffre , C. Berthier , D. Schmidiger , A. Zheludev , M. Horvatić

We have analyzed the experimental evidence of charge and orbital ordering in La0.5Sr1.5MnO4 using first principles band structure calculations. Our results suggest the presence of two types of Mn sites in the system. One of the Mn sites…

强关联电子 · 物理学 2009-11-07 Priya Mahadevan , K. Terakura , D. D. Sarma

The recent discovery of altermagnetism has sparked growing interest in compensated magnetic systems as promising platforms for highly scalable spintronics. Altermagnetism is a distinct magnetic order where opposite spin sublattices are…

We report inelastic light scattering measurements of lattice dynamics related to the incommensurate orbital order in $\mathrm{CaMn_7O_{12}}$. Below the ordering temperature $T_\mathrm{o} \approx 250 \,\mathrm{K}$, we observe extra phonon…

强关联电子 · 物理学 2015-06-22 Xinyu Du , Renliang Yuan , Lian Duan , Chong Wang , Yuwen Hu , Yuan Li

Electron spins are amongst the most coherent solid-state systems known, however, to be used in devices for quantum sensing and information processing applications, they must be typically placed near interfaces. Understanding and mitigating…