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A systematic study using neutron diffraction and magnetic susceptibility are reported on Mn substituted ferrimagnetic inverse spinel Ti$_{1-x}$Mn$_{x}$Co$_2$O$_4$ in the temperature interval 1.6 K $\leq$ $T$ $\leq$ 300 K. Our neutron…

强关联电子 · 物理学 2020-03-23 P. Pramanik , D. C. Joshi , M. Reehuis , A. Hoser , J. U. Hoffmann , R. S. Manna , T. Sarkar , S. Thota

We investigate the quasiparticle dynamics in MnBi2Te4 single crystal using the ultrafast optical spectroscopy. Our results show that there exist anomalous dynamical optical responses below the antiferromagnetic (AFM) ordering temperature…

材料科学 · 物理学 2023-08-24 Liang Cheng , Tian Xiang , Jingbo Qi

muSR experiments on the geometrically frustrated spinel oxide, Li2Mn2O4, show the development of spin correlations over a range of length scales with decreasing temperature. Increased relaxation below 150 K is consistent with the onset of…

强关联电子 · 物理学 2009-11-11 C. R. Wiebe , P. L. Russo , A. T. Savici , Y. J. Uemura , G. J. MacDougall , G. M. Luke , S. Kuchta , J. E. Greedan

We report detailed Raman spectroscopic and magnetic susceptibility studies on the spin-driven ferroelectric compounds Mn4Nb2O9 (MNO) and Mn4Ta2O9 (MTO). Both systems exhibit strong spin-phonon coupling below the short-range magnetic…

材料科学 · 物理学 2026-02-09 Rajesh Jana , Alka Garg , Rekha Rao , Thomas Meier

We report on the temperature dependent Raman spectroscopic studies of orthorombic distorted perovskite YCrO3 in the temperature range of 20-300K. Temperature dependence of DC-magnetization measurement under field cooled and zero field…

材料科学 · 物理学 2013-09-30 Yogesh Sharma , Satyaprakash Sahoo , W. Perez , Ram S. Katiyar

The magnon dispersion in the charge, orbital and spin ordered phase in La(0.5)Sr(1.5)MnO(4) has been studied by means of inelastic neutron scattering. We find an excellent agreement with a magnetic interaction model basing on the CE-type…

强关联电子 · 物理学 2009-11-11 D. Senff , F. Krueger , S. Scheidl , M. Benomar , Y. Sidis , F. Demmel , M. Braden

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

材料科学 · 物理学 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

强关联电子 · 物理学 2017-08-23 Santanu Pal , Siddhartha Lal

The breakdown of magnons, the quasiparticles of magnetic systems, has rarely been seen. By using an inelastic neutron scattering technique we report the observation of spontaneous magnon decay in multiferroic LuMnO$_3$, a simple…

Inelastic neutron scattering measurements on the molecular dimer-Mott insulator $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl reveal a phonon anomaly in a wide temperature range. Starting from $T_{\rm ins}\sim50$-$60$ K where the charge gap…

From low-temperature Synchrotron X-ray diffraction, a precise thermal characterization of octahedral distortions in single phase Ruddlesden-Popper Ca3Mn2O7 is performed. Highly sensitive close-steps temperature dependences of Mn-O-Mn bond…

材料科学 · 物理学 2020-04-24 Pooja Sahlot , A. K. Sinha , A. M. Awasthi

Quantum spin liquid (QSL), a state characterized by exotic low energy fractionalized excitations and statistics is still elusive experimentally and may be gauged via indirect experimental signatures. Remnant of QSL phase may reflect in the…

Layered antiferromagnetic materials have emerged as a novel subset of the two-dimensional family providing a highly accessible regime with prospects for layer-number-dependent magnetism. Furthermore, transition metal phosphorous…

The lattice dynamic properties and spin-phonon coupling in DyMn$_2$O$_5$ are studied by using the density-functional theory. The calculated phonon frequencies are in very good agreement with experiments. We then compare the phonon modes…

材料科学 · 物理学 2009-11-13 Tianqi Shen , Kun Cao , Guang-Can Guo , Lixin He

Two distinct ferromagnetic phases of LaMn$_{0.5}$Co$_{0.5}$O$_{3}$ having monoclinic structure with distinct physical properties have been studied. The ferromagnetic ordering temperature $\textit{T}_{c}$ is found to be different for both…

Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view, the combination of the high-frequency of spin manipulations offered by…

Structural, electronic, and magnetic properties of modified cubic spinel compound LiNi$_{0.5}$Mn$_{1.5}$O$_{4}$ are studied via x-ray diffraction, resistivity, DC and AC magnetization, heat capacity, neutron diffraction, $^7$Li nuclear…

材料科学 · 物理学 2020-12-02 S. S. Islam , Vikram Singh , K Somesh , Prashanta K Mukharjee , A. Jain , S. M. Yusuf , R. Nath

The breaking of chiral and time-reversal symmetries provides a pathway to exotic quantum phenomena and topological phases. In particular, the breaking of chiral (mirror) symmetry in quantum materials has been shown to have important…

强关联电子 · 物理学 2023-02-13 Anjishnu Bose , Arijit Haldar , Erik S. Sørensen , Arun Paramekanti

Neutron scattering has been used to study the structure and spin dynamics of La$_{0.85}$Sr$_{0.15}$MnO$_3$. The magnetic structure of this system is ferromagnetic below T_C = 235 K. We see anomalies in the Bragg peak intensities and new…

强关联电子 · 物理学 2009-10-31 L. Vasiliu-Doloc , J. W. Lynn , A. H. Moudden , A. M. de Leon-Guevara , A. Revcolevschi

We report low-temperature Raman signatures of the Heisenberg quantum magnet Ca$_{10}$Cr$_7$O$_{28}$, showing clear anomalies in phonon mode frequencies and linewidths below $\sim$100 K. This crossover temperature lies in between the…

强关联电子 · 物理学 2023-12-12 Srishti Pal , Arnab Seth , Anzar Ali , Yogesh Singh , D. V. S. Muthu , Subhro Bhattacharjee , A. K. Sood