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We report the synthesis, crystal structure, and magnetic properties of two new quantum antiferromagnets A3ReO5Cl2 (A = Sr and Ba). The crystal structure is isostructural with the mineral pinalite Pb3WO5Cl2, in which the Re6+ ion is…

强关联电子 · 物理学 2021-04-06 Daigorou Hirai , Takeshi Yajima , Kazuhiro Nawa , Mitsuaki Kawamura , Zenji Hiroi

The spin-1/2 Heisenberg antiferromagnet on an anisotropic triangular lattice (ATL) is an archetypal spin system hosting exotic quantum magnetism and dimensional crossover. However, the progress in experimental research on this field has…

材料科学 · 物理学 2023-11-13 M. Gen , D. Hirai , K. Morita , S. Kogane , N. Matsuyama , T. Yajima , M. Kawamura , K. Deguchi , A. Matsuo , K. Kindo , Y. Kohama , Z. Hiroi

We determined the crystal structure of Cs$_2$LiRuCl$_6$, which was synthesized first in this work, and investigated its magnetic properties. Cs$_2$LiRuCl$_6$ has a hexagonal structure composed of linear chains of face-sharing RuCl$_6$ and…

The Re5+(5d2) compounds possess large spin-orbital interaction which urges for large anisotropy, non-collinear structures and other phenomena. Here we present ReCl5 composed by separate Re2Cl10 units formed by edge-shared chlorine…

A structural and thermodynamic study of the newly synthesized single crystal Sr5Rh4O12 is reported. Sr5Rh4O12 consists of a triangular lattice of spin chains running along the c-axis. It is antiferromagnetically ordered below 23 K with the…

强关联电子 · 物理学 2015-06-25 G. Cao , S. Parkin , P. Schlottmann

The observation of spinon excitations in the $S=\frac{1}{2}$ triangular antiferromagnet Ca$_3$ReO$_5$Cl$_2$ reveals a quasi-one-dimensional (1D) nature of magnetic correlations, in spite of the nominally 2D magnetic structure. This…

强关联电子 · 物理学 2022-10-31 S. A. Zvyagin , A. N. Ponomaryov , J. Wosnitza , D. Hirai , Z. Hiroi , M. Gen , Y. Kohama , A. Matsuo , Y. H. Matsuda , K. Kindo

Motivated by the observation of a gapless spin liquid state in $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$, we analyze the anisotropic triangular lattice $S=1/2$ Heisenberg model with the resonating valence bond mean-field approximation. Paying…

强关联电子 · 物理学 2007-06-13 Yuta Hayashi , Masao Ogata

We present a theoretical and experimental study of a quasi-one-dimensional zigzag antiferromagnet (N_2H_5)CuCl_3, which can be viewed as weakly coupled Heisenberg chains with a frustrated interaction. We first discuss generic features of…

强关联电子 · 物理学 2009-11-07 N. Maeshima , M. Hagiwara , Y. Narumi , K. Kindo , T. C. Kobayashi , K. Okunishi

Spin liquids occuring in 2D frustrated spin systems were initially assumed to appear at strongest frustration, but evidence grows that they more likely intervene at transitions between two different types of order. To identify if this is…

强关联电子 · 物理学 2013-01-30 Philipp Hauke

Non-collinear two-dimensional triangular lattice antiferromagnets (2D TLAF) are currently an area of very active research due to their unique magnetic properties, which lead to non-trivial quantum effects that experimentally manifest…

Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…

We report a structural, thermodynamic and transport study of the newly synthesized Sr5Rh4O12, Ca5Ir3O12 and Ca4IrO6 single crystals. These quasi-one-dimensional insulators consist of a triangular lattice of spin chains running along the…

强关联电子 · 物理学 2015-06-25 G. Cao , V. Durairaj , S. Chikara , S. Parkin , P. Schlottmann

Ca3Co2O6 is a system exhibiting a series of fascinating properties, including magnetization plateaus and remarkably slow dynamics at low-T. These properties are intimately related to the geometrical frustration, which results from a…

强关联电子 · 物理学 2007-05-23 Vincent Hardy , Delphine Flahaut , Raymond Fresard , Antoine Maignan

We investigate the anisotropic triangular lattice that interpolates from decoupled one-dimensional chains to the isotropic triangular lattice and has been suggested to be relevant for various quasi-two-dimensional materials, such as…

强关联电子 · 物理学 2009-07-17 Dariush Heidarian , Federico Becca , Sandro Sorella

The S=2 anisotropic triangular lattice alpha-NaMnO2 is studied by neutron inelastic scattering. Antiferromagnetic order occurs at T ~ 45 K with opening of a spin gap. The spectral weight of the magnetic dynamics above the gap (Delta ~ 7.5…

强关联电子 · 物理学 2015-05-13 C. Stock , L. C. Chapon , O. Adamopoulos , A. Lappas , M. Giot , J. W. Taylor , M. A. Green , C. M. Brown , P. G. Radaelli

The $1/4$-filled organic compound, $\delta$-(EDT-TTF-CONMe$_{2}$)$_{2}$AsF$_6$ is a frustrated two-dimensional triangular magnetic system as shown by high-frequency (111.2 and 222.4 GHz) electron spin resonance (ESR) and structural data in…

强关联电子 · 物理学 2016-11-22 B. Náfrádi , A. Antal , T. Fehér , L. F. Kiss , C. Mézière , P. Batail , L. Forró , A. Jánossy

The quantum spin-1/2 antiferromagnetic Heisenberg model on a two dimensional triangular lattice geometry with spatial anisotropy is relevant to describe materials like ${\rm Cs_2 Cu Cl_4}$ and organic compounds like…

强关联电子 · 物理学 2011-11-09 Seiji Yunoki , Sandro Sorella

We study the quasi-one-dimensional limit of the spin-1/2 quantum Heisenberg antiferromagnet on the kagome lattice. The lattice is divided into antiferromagnetic spin-chains (exchange J) that are weakly coupled via intermediate "dangling"…

强关联电子 · 物理学 2008-11-20 Andreas P. Schnyder , Oleg A. Starykh , Leon Balents

We present a model compound with a spin-1/2 spatially anisotropic frustrated square lattice, in which three antiferromagnetic interactions and one ferromagnetic interaction are competing. We observe an unconventional gradual increase in the…

强关联电子 · 物理学 2021-06-24 H. Yamaguchi , Y. Iwasaki , Y. Kono , T. Okubo , S. Miyamoto , Y. Hosokoshi , A. Matsuo , T. Sakakibara , T. Kida , M. Hagiwara

The compounds $Ln$AuAl$_4$Ge$_2$ ($Ln$ $=$ lanthanide) form in a structure that features two-dimensional triangular lattices of $Ln$ ions that are stacked along the crystalline $c$ axis. Together with crystal electric field effects,…

强关联电子 · 物理学 2024-01-03 Keke Feng , Caleb Bush , Olatunde Oladehin , Minhyea Lee , Ryan Baumbach
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