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Recently, there has been a growing interest in the usage of mm-scale composites of plasmonic nanoparticles for enhancing the rates of chemical reactions; the effect was shown recently to be predominantly associated with the elevated…

应用物理 · 物理学 2023-03-31 Ieng-Wai Un , Yonatan Sivan

We report a novel behavior of the surface plasmon linewidth in sodium nanospheres Na$_{1760}$ changing with the electron temperature, which monotonically decreases and bears a discontinuous sudden drop at high electron temperatures. Our…

介观与纳米尺度物理 · 物理学 2014-08-15 Guozhong Wang , Yizhuang Zheng , Jian Zi

Following the lifespan of optical excitations from their creation to decay into photons is crucial in understanding materials optical properties. Macroscopically, techniques such as the photoluminescence excitation spectroscopy provide…

We demonstrate that plasmonic helical gratings consisting of metallic nanowires imprinted with helical grooves or ridges can be used efficiently to generate plasmonic vortices with radius much smaller than the operating wavelength. In our…

We extend de concept of Compton scattering to the case of plasmons. This concept was originally applied to electrons in vacuum. Here, we consider electrons in a plasma, and study the scattering properties of photon-plasmon interactions. We…

等离子体物理 · 物理学 2023-10-18 José Tito Mendonça , Fernando Haas

Tremendous enhancement of light-matter interaction in plasmon-excited molecular hybrid devices allows for non-linearities on the level of single emitters and few photons. This promises a plethora of novel applications like single photon…

We use excited-state quantum chemistry techniques to investigate the intraband absorption of doped semiconductor nanoparticles as a function of doping density, nanoparticle radius, and material properties. The excess electrons are modeled…

介观与纳米尺度物理 · 物理学 2019-07-29 Bryan T. G. Lau , Timothy C. Berkelbach

Relaxation dynamics of embedded metal nanoparticles after ultrafast laser pulse excitation is driven by thermal phenomena of different origins the accurate description of which is crucial for interpreting experimental results: hot electron…

材料科学 · 物理学 2009-11-13 Majid Rashidi-Huyeh , Sebastian Volz , Bruno Palpant

We show that the dynamics of the surface plasmon in metallic nanoparticles damped by its interaction with particle-hole excitations can be modelled by a single degree of freedom coupled to an environment. In this approach, the fast decrease…

介观与纳米尺度物理 · 物理学 2011-11-09 Cesar Seoanez , Guillaume Weick , Rodolfo A. Jalabert , D. Weinmann

Atomic and single-molecule junctions represent the ultimate limit to the miniaturization of electrical circuits. They are also ideal platforms to test quantum transport theories that are required to describe charge and energy transfer in…

介观与纳米尺度物理 · 物理学 2013-08-01 Woochul Lee , Kyeongtae Kim , Wonho Jeong , Linda Angela Zotti , Fabian Pauly , Juan Carlos Cuevas , Pramod Reddy

The physical mechanisms of periodic separation and relaxation of electric charges within aerosol particles possessing the properties the short-circuited batteries can be extremely diverse. With use of appropriate materials and dispersing…

综合物理 · 物理学 2012-04-16 Oleg Meshcheryakov

Quantum emitters coupled to plasmonic resonators are known to allow enhanced broadband Purcell factors, and such systems have been recently suggested as possible candidates for on-demand single photon sources, with fast operation speeds.…

Crystals of plasmonic metal nanoparticles have intriguing optical properties. They reach the regimes of ultrastrong and deep strong light-matter coupling, where the photonic states need to be included in the simulation of material…

Isolating single molecules in the solid state has allowed fundamental experiments in basic and applied sciences. When cooled down to liquid helium temperature, certain molecules show transition lines, that are tens of megahertz wide,…

The hot electron generation in plasmonic nanoparticles is the key to efficient plasmonic photocatalysis. In the paper, we study theoretically for the first time the effect of Tamm states (TSs) at the interface metal-semiconductor on hot…

Understanding the spectral and temporal dynamics of charge transfer plasmon resonances that emerge in conductively connected plasmonic nanoparticles is crucial for exploiting their potentials for enhanced infrared spectroscopy and optical…

光学 · 物理学 2024-12-25 Alemayehu Nana Koya , Longnan Li , Wei Li

Plasmonic nanocavities are known for their extreme field enhancement and sub-wavelength light confinement in gaps of just a few nanometers. Pairing this with the ability to host quantum emitters, they form highly promising platforms to…

量子物理 · 物理学 2024-02-26 Kalun Bedingfield , Benjamin Yuen , Angela Demetriadou

Plasmonic nanoparticles (NPs) hold tremendous promise for catalyzing light-driven chemical reactions. The conventionally assumed detrimental absorption loss from plasmon damping can now be harvested to drive chemical transformations of the…

Lasers are ubiquitous for information storage, processing, communications, sensing, biological research, and medical applications [1]. To decrease their energy and materials usage, a key quest is to miniaturize lasers down to nanocavities…

By using the real-space method, switching of a single plasmon interacting with a hybrid nanosystem composed of a semiconductor quantum dot (SQD) and a metallic nanoparticle (MNP) coupled to one-dimensional surface plasmonic waveguide is…

介观与纳米尺度物理 · 物理学 2016-01-13 Myong-Chol Ko , Nam-Chol Kim , Zhong-Hua Hao , Li Zhou , Jian-Bo Li , Qu-Quan Wang