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The diffusion Monte Carlo method with symmetry-based state selection is used to calculate the quantum energy states of H$_2^+$ confined into potential barriers of atomic dimensions (a model for these ions in solids). Special solutions are…

化学物理 · 物理学 2019-04-03 Gaia Micca Longo , Savino Longo , Domenico Giordano

In this paper the Diffusion Monte Carlo (DMC) method is applied to the confined hydrogen atom with different confinement geometries. This approach is validated using the much studied spherical and cylindrical confinements and then applied…

化学物理 · 物理学 2019-03-20 Gaia Micca Longo , Savino Longo , Domenico Giordano

Computational codes based on the Diffusion Monte Carlo method can be used to determine the quantum state of two-electron systems confined by external potentials of various nature and geometry. In this work, we show how the application of…

化学物理 · 物理学 2021-02-24 Gaia Micca Longo , Carla Maria Coppola , Domenico Giordano , Savino Longo

Ground state energies for confined hydrogen (H) and helium (He) atoms, inside a penetrable/impenetrable compartment have been calculated using Diffusion Monte Carlo (DMC) method. Specifically, we have investigated spherical and ellipsoidal…

其他凝聚态物理 · 物理学 2009-11-13 M. Neek-Amal , G. Tayebirad , M. Molayem , M. E. Foulaadvand , L. Esmaeili Sereshki , A. Namiranian

The variational Monte Carlo method is used to evaluate the ground-state energy of the confined hydrogen molecule, H_2. Accordingly, we considered the case of hydrogen molecule confined by a hard prolate spheroidal cavity when the nuclear…

原子与分子团簇 · 物理学 2015-09-10 S. B. Doma , F. N. El-Gammal , A. A. Amer

The Diffusion Monte Carlo (DMC) method is applied to compute the ground state energies of the water monomer and dimer and their D 2 O isotopomers using MB-pol; the most recent and most accurate ab inito- based potential energy surface…

化学物理 · 物理学 2015-10-28 Joel Mallory , Vladimir Mandelshtam

The molecular ion H$_2^+$ is studied under strong confinement conditions produced by a spherical barrier centered in the gravity center of the molecule. Results for the potential curves are obtained by diffusion Monte Carlo methods for the…

化学物理 · 物理学 2019-04-03 Gaia Micca Longo , Savino Longo , Domenico Giordano

We present ground and excited state energies obtained from Diffusion Monte Carlo (DMC) calculations, using accurate multiconfiguration wave functions, for $N$ electrons ($N\le13$) confined to a circular quantum dot. We analyze the…

凝聚态物理 · 物理学 2009-10-31 F. Pederiva , C. J. Umrigar , E. Lipparini

We study beryllium dihydride (BeH$_2$) and acetylene (C$_2$H$_2$) molecules using real-space diffusion Monte Carlo (DMC) method. The molecules serve as perhaps the simplest prototypes that illustrate the difficulties with biases in the…

We have carried out theoretical investigations of electron correlation effects on the atomic properties of the Ca atom trapped inside an attractive spherically symmetric potential well of an endohedral fullerene C$_{60}$ cluster.…

原子物理 · 物理学 2018-07-24 S. Bharti , L. Sharma , B. K. Sahoo , P. Malkar , R. Srivastava

We report results of both Diffusion Quantum Monte Carlo(DMC) method and Reptation Quantum Monte Carlo(RMC) method on the potential energy curve of the helium dimer. We show that it is possible to obtain a highly accurate description of the…

化学物理 · 物理学 2015-05-18 Xuebin Wu , Xianru Hu , Chenlei Du , Yunchuan Dai , Shibin Chu , Leibo Hu , Jianbo Deng , Yuanping Feng

A faithful description of chemical processes requires exploring extended regions of the molecular potential energy surface (PES), which remains challenging for strongly correlated systems. Transferable deep-learning variational Monte Carlo…

化学物理 · 物理学 2026-03-27 P. Bernát Szabó , Zeno Schätzle , Frank Noé

The ground state energy of hydrogen molecular ion H2+ confined by a hard prolate spheroidal cavity is calculated. The case in which the nuclear positions are clamped at the foci is considered. Our calculations are based on using the…

原子与分子团簇 · 物理学 2016-05-25 S. B. Doma , F. N. El-Gammal , A. A. Amer

The feasibility of shell-model calculations is radically extended by the Quantum Monte Carlo Diagonalization method with various essential improvements. The major improvements are made in the sampling for the generation of shell-model basis…

核理论 · 物理学 2008-11-26 Michio Honma , Takahiro Mizusaki , Takaharu Otsuka

We report results of both the Diffusion Quantum Monte Carlo (DMC) and Reptation Quantum Monte Carlo (RMC) methods on the potential energy curve of the helium dimer. We show that it is possible to obtain a highly accurate description of the…

化学物理 · 物理学 2010-05-07 Xuebin Wu , Chenlei Du , Jianbo Deng

A many-flavor electron gas (MFEG) in a semiconductor with a valley degeneracy ranging between 6 and 24 was analyzed using diffusion Monte Carlo (DMC) calculations. The DMC results compare well with an analytic expression derived by one of…

强关联电子 · 物理学 2009-11-13 G. J. Conduit , P. D. Haynes

The effects of quantum confinement on the momentum distribution of electrons confined within a cylindrical potential well have been analyzed. The motivation is to understand specific features of the momentum distribution of electrons when…

原子物理 · 物理学 2016-05-04 A. S. Baltenkov , A. Z. Msezane

We investigate Monte Carlo simulation strategies for determining the effective ("depletion") potential between a pair of hard spheres immersed in a dense sea of much smaller hard spheres. Two routes to the depletion potential are…

软凝聚态物质 · 物理学 2015-06-16 D. J. Ashton , V. Sanchez-Gil , N. B. Wilding

The ground-state properties of two-dimensional liquid $^4$He at zero temperature are studied by means of a quadratic diffusion Monte Carlo method. As interatomic potential we use a revised version of the HFDHE2 Aziz potential which is…

凝聚态物理 · 物理学 2009-10-28 S. Giorgini , J. Boronat , J. Casulleras

We have used diffusion Monte Carlo (DMC) simulations to calculate the energy barrier for H$_2$ dissociation on the Mg(0001) surface. The calculations employ pseudopotentials and systematically improvable B-spline basis sets to expand the…

材料科学 · 物理学 2009-11-13 M. Pozzo , D. Alfe`
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