相关论文: Stimulated low-frequency Raman scattering in album…
Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…
Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…
Noise can play an important role in nonlinear pulse propagation. It is not only the origin of fluctuations in supercontinuum but can also determine the generated signal amplitude and phase, as seen in phenomena such as noise-seeded…
Raman spectroscopy enables non-destructive, label-free molecular analysis with high specificity, making it a powerful tool for biomedical diagnostics. However, its application to biological tissues is challenged by inherently weak Raman…
Composition-spread La1-xSrxMnO3 thin films were prepared by pulsed laser deposition technique from LaMnO3 and SrMnO3 targets. The films were epitaxial with a continuous variation of the out of plane lattice parameter along the direction of…
We investigated interlayer phonon modes of mechanically exfoliated few-layer 2H-SnS2 samples by using room temperature low-frequency micro-Raman spectroscopy. Raman measurements were performed using laser wavelength of 441.6, 514.4, 532 and…
Lattice structure and symmetry of two-dimensional (2D) layered materials are of key importance to their fundamental mechanical, thermal, electronic and optical properties. Raman spectroscopy, as a convenient and nondestructive tool, however…
Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour…
Stimulated Raman scattering is a well-known nonlinear process that can be harnessed to produce optical gain in a wide variety of media. This effect has been used to produce the first silicon-based lasers and high-gain amplifiers.…
The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…
Molybdenum sulfides are in the spotlight of materials science thanks to their interesting properties for applications in optoelectronics, nanocomposites, lubricants, and catalysis. The structural characterization of Molybdenum sulfides is a…
This work presents how first-principles simulations validated through experimental measurements lead to a new accurate prediction of the expected Raman shift as a function of strain in silicon. Structural relaxation of a strained primitive…
The Raman shifts of nanocrystalline GaSb excited by an Ar+ ion laser of wavelengths 514.5, 496.5, 488.0, 476.5, and 457.9 nm are studied by experiment and explained by phonon confinement, tensile stress, resonance Raman scattering and…
We present the first experimental evidence of stimulated Raman re-scattering of a laser in plasma: The scattered light produced by the Raman instability is intense enough to scatter again through the same instability. Although never…
The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…
Soliton microcombs are evolving towards octave-spanning for $f$-$2f$ self-referencing and expanding applications in spectroscopy and timekeeping. As spectra broaden and pulses shorten, the Raman-induced soliton self-frequency shift (SSFS)…
Stimulated Raman scattering (SRS) in its strongly nonlinear, kinetic regime is controlled by a technique of deterministic, strong temporal modulation and spatial scrambling of laser speckle patterns, called Spike Trains of Uneven Duration…
Hydrogen detection is of great importance in chemical and energy industries. Optical fiber hydrogen sensors show flexibility and compactness and have the potential for distributed analysis. However, traditional fiber sensors encounter a…
We have measured the spectral correlations and intensity statistics of random lasing modes in weakly scattering systems, and compared them to those of the amplified spontaneous emission spikes. Their dramatic differences revealed the…
Raman transitions are used in quantum simulations with ultracold atoms for cooling, spectroscopy and creation of artificial gauge fields. Spatial shaping of the Raman fields allows local control of the effective Rabi frequency, which can be…