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We show that the Weyl phase in $\rm Sm_2Ir_2O_7$ is protracted up to at least 2~\% alloying with Bi by an anomalous negative lattice expansion with $\rm \Delta a \sim- 0.01$\AA. With further doping, the magnetic ordering disappears and…

强关联电子 · 物理学 2021-06-28 Prachi Telang , Surjeet Singh

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

强关联电子 · 物理学 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

The oxide pyrochlore Bi$_2$Ti$_2$O$_7$ is in some ways analogous to perovskite PbTiO$_3$, in that Bi$_2$Ti$_2$O$_7$ has two cations, Bi$^{3+}$ and Ti$^{4+}$ in oxidation states that are normally associated with a propensity to off-center.…

材料科学 · 物理学 2007-12-13 Craig J. Fennie , Ram Seshadri , Karin M. Rabe

The crystal lattice of Sr$_2$IrO$_4$ is investigated with synchrotron X-ray powder diffraction under hydrostatic pressures up to $P=43$ GPa and temperatures down to $20$ K. The tetragonal unit cell is maintained over the whole investigated…

强关联电子 · 物理学 2020-02-26 K. Samanta , R. Tartaglia , U. F. Kaneko , N. M. Souza-Neto , E. Granado

We study the electronic properties of strongly spin-orbit coupled electrons on the elastic pyrochlore lattice. Akin to the Peierls transition in one-dimensional systems, the coupling of the lattice to the electronic degrees of freedom can…

介观与纳米尺度物理 · 物理学 2015-04-16 Tomáš Bzdušek , Andreas Rüegg , Manfred Sigrist

Eu2Ir2O7, a candidate Weyl semimetal, shows an insulator-to-metal transition as a function of Bi substitution at the Eu site. In this work, we investigate the (Eu_1-xBi_x)2Ir2O7 series via Hard X-ray Photoemission Spectroscopy (HAXPES),…

强关联电子 · 物理学 2021-01-29 Prachi Telang , Kshiti Mishra , Rabindranath Bag , A. Gloskovskii , Yu. Matveyev , Surjeet Singh

Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

强关联电子 · 物理学 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

强关联电子 · 物理学 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

强关联电子 · 物理学 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher

We report on the epitaxial growth, structural and electrical properties of metallic pyrochlore bismuth ruthenate heterostructures grown along both the [001] and [111] directions. Ordered pyrochlore thin films were obtained with highly…

Pyrochlore systems ($A_{2}B_{2}O_{7}$) with $A$-site rare-earth local moments and $B$-site $5d$ conduction electrons offer excellent material platforms for the discovery of exotic quantum many-body ground states. Notable examples include…

强关联电子 · 物理学 2019-05-01 Hanbit Oh , Sangjin Lee , Yong Baek Kim , Eun-Gook Moon

$\rm Sr_2IrO_4$ is an archetypal spin-orbit-coupled Mott insulator and has been extensively studied in part because of a wide range of predicted novel states. Limited experimental characterization of these states thus far brings to light…

强关联电子 · 物理学 2020-09-14 Feng Ye , Christina Hoffmann , Wei Tian , Hengdi Zhao , G. Cao

The XY pyrochlore antiferromagnet Er$_2$Ti$_2$O$_7$ exhibits a rare case of $Z_6$ discrete symmetry breaking in its $\psi_2$ magnetic ground state. Despite being well-studied theoretically, systems with high discrete symmetry breakings are…

强关联电子 · 物理学 2017-02-15 J. Gaudet , A. M. Hallas , J. Thibault , N. P. Butch , H. A. Dabkowska , B. D. Gaulin

In the search for topological phases in correlated electron systems, iridium-based pyrochlores A2Ir2O7 -- materials with 5d transition-metal ions -- provide fertile grounds. Several novel topological states have been predicted but the…

The pyrochlore Eu$_2$Ir$_2$O$_7$ has recently attracted significant attention as a candidate Weyl semimetal. The previous reports on this compound unanimously show a thermally induced metal to insulator (MI) transition, concomitant with…

强关联电子 · 物理学 2018-06-27 Prachi Telang , Kshiti Mishra , A. K. Sood , Surjeet Singh

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

We investigate a lattice of interacting anharmonic oscillators by using a mean field theory and exact diagonalization. We construct an effective five-state hopping model with intersite repulsions as a model for beta-pyrochlore AOs_2O_6(A=K,…

强关联电子 · 物理学 2009-11-13 Kazumasa Hattori , Hirokazu Tsunetsugu

Magnetic materials with pyrochlore crystal structure form exotic magnetic states due to the high lattice frustration. In this work we follow the effects of coupling of the lattice and electronic and magnetic degrees of freedom in two…

We study the physics of hard-core bosons with unfrustrated hopping (t) and nearest-neighbor repulsion (V) on the three dimensional pyrochlore lattice. At half-filling, we demonstrate that the small V/t superfluid state eventually becomes…

强关联电子 · 物理学 2009-11-13 Argha Banerjee , Sergei V. Isakov , Kedar Damle , Yong Baek Kim

Motivated by the proposal of a Weyl-semimetal phase in pyrochlore iridates, we consider a Hubbard-type model on the pyrochlore lattice. To shed light on the question as to why such a state has not been observed experimentally, its…

强关联电子 · 物理学 2018-05-23 Christoph Berke , Paolo Michetti , Carsten Timm
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