相关论文: Cu$_2$O Microcrystals Grown on Silicon as Platform…
Cuprous oxide (Cu${}_2$O) has recently been proposed as a promising solid-state host for excitonic Rydberg states with large principal quantum numbers ($n$), whose exaggerated wavefunction sizes ($\propto n^2)$ facilitate gigantic…
Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide ($\text{Cu}_{2}\text{O}$) has recently…
High-lying Rydberg states of Mott-Wannier excitons are receiving considerable interest due to the possibility of adding long-range interactions to the physics of exciton-polaritons. Here, we study Rydberg excitation in bulk synthetic…
Highly excited atoms with an electron moved into a level with large principal quantum number are fascinating hydrogen-like objects. The giant extension of these Rydberg atoms leads to huge interaction effects. Monitoring these interactions…
Rydberg states of excitons can reach microns in size and require extremely pure crystals. We introduce an experimental method for the rapid and spatially-resolved characterization of Rydberg excitons in copper oxide (Cu2O) with sub-micron…
Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…
We theoretically investigate the nonlinear optical transmission through a cuprous oxide crystal for wavelengths that cover the series of highly excited excitons, observed in recent experiments. Since such Rydberg excitons have strong van…
Rydberg excitons in Cu2O can be an emergent platform for solid-state quantum information processing by utilizing the exaggerated properties of high-lying excited states within the material. To develop practical quantum systems,…
The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4]…
Microwave-optical conversion is key to future networks of quantum devices, such as those based on superconducting technology. Conversion at the single quantum level requires strong nonlinearity, high bandwidth, and compatibility with a…
We report exciton-mediated coupling between microwave and optical fields in cuprous oxide (Cu$_2$O) at low temperatures. Rydberg excitonic states with principal quantum number up to $n=12$ were observed at 4~K using both one-photon…
The shape-controlled synthesis of cuprous oxide (Cu$_2$O) photocatalysts with both low or high index crystal planes has received increasing attention due to their unique facet-dependent properties. Since they are cheap and earth abundant,…
Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…
We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…
The recent observation of high-lying Rydberg states of excitons in semiconductors with relatively high binding energy motivates exploring their applications in quantum nonlinear optics and quantum information processing. Here, we study…
Excitons, i.e. the bound states of an electron and a positively charged hole are the solid state analogue of the hydrogen atom. As such they exhibit a Rydberg series, which in cuprous oxide has been observed up to high principal quantum…
The quantum confinement of Rydberg excitons is an important step towards exploiting their large nonlinearities for quantum applications. We observe Rydberg excitons in natural nanoparticles of Cu$_2$O. We resolve up to the principal quantum…
Hosting giant Rydberg excitons with principal quantum numbers up to n = 30, cuprous oxide (Cu2O) provides a rare solid-state setting for exploring Rydberg physics, as exemplified by the blockade effect. Here we access the strongly…
Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…
Highly-excited states of excitons in cuprous oxide have recently been observed at a record quantum number of up to $n=25$. Here, we evaluate the long-range interactions between pairs of Rydberg excitons in Cu$_2$O, which are due to direct…