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We have carried out temperature-dependent x-ray diffraction and Raman scattering experiments on powder $Cs_3Bi_2Br_9$. Trigonal to monoclinic structural transition at around 95 K is discussed and shown to be driven by the softening of the…

Using multiscale modelling we investigate layer-breathing phonons in MX$_2$ bilayers (M=Mo,W; X=S,Se) containing dislocations specific for lattice-relaxed moir\'e superlattices. The dislocations, forming in the bilayers with parallel and…

介观与纳米尺度物理 · 物理学 2025-07-14 V. V. Enaldiev

Twisted stacked few layer black phosphorus heterostructures were successfully fabricated in this work. Abnormal blue shifts in their Ag1 and Ag2 Raman peaks and unique optical reflections were observed in these samples. The phonon behavior…

材料科学 · 物理学 2018-05-04 Tao Fang , Teren Liu , Zenan Jiang , Rui Yang , Peyman Servati , Guangrui , Xia

Resonant Raman spectra of single layer WS$_{2}$ flakes are presented. A second order Raman peak (2LA) appears under resonant excitation with a separation from the E$^{1}_{2g}$ mode of only $4$cm$^{-1}$. Depending on the intensity ratio and…

介观与纳米尺度物理 · 物理学 2014-06-30 A. A. Mitioglu , P. Plochocka , G. Deligeorgis , S. Anghel , L. Kulyuk , D. K. Maude

Bound quasiparticles, negatively charged trions and neutral excitons, are associated with the direct optical transitions at the K-points of the Brillouin zone for monolayer MoS$_2$. The change in the carrier concentration, surrounding…

材料科学 · 物理学 2017-08-01 Achintya Bera , D V S Muthu , A K Sood

For conventional materials, the thermal conductivity of thin film is usually suppressed when the thickness decreases due to phonon-boundary scattering. However, this is not necessarily true for the van der Waals solids if the thickness is…

材料科学 · 物理学 2016-03-01 Xiaokun Gu , Baowen Li , Ronggui Yang

We report ultra-strong high-order nonlinear multiphoton processes in monolayer MoS$_2$ (1L-MoS$_2$): the third harmonic is thirty times stronger than the second harmonic, and the fourth harmonic is comparable to the second harmonic. We find…

We present a Raman study of ZrAs_{2} single crystals, a nodal line semimetal with symmetry-enforced Dirac-like band crossings. We identified the symmetry of phonon modes by polarized light measurements and comparison with calculated phonon…

材料科学 · 物理学 2024-05-16 R. Bacewicz , C. Jastrzębski , K. Zberecki , A. S. Wadge , D. Jastrzębski , A. Wiśniewski

We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…

光学 · 物理学 2018-05-25 Yu Song , Ruijuan Tian , Jiulong Yang , Rui Yin , Jianlin Zhao , Xuetao Gan

Under homogeneous uniaxial strains, the Raman 2D band of graphene involving two-phonon double-resonance scattering processes splits into two peaks and they altogether redshift strongly depending on the direction and magnitude of the strain.…

介观与纳米尺度物理 · 物理学 2015-03-19 Duhee Yoon , Young-Woo Son , Hyeonsik Cheong

The Raman selection rules arise from the crystal symmetry and then determine the Raman activity and polarization of scattered phonon modes. However, these selection rules can be broken in resonant process due to the strong electron-phonon…

材料科学 · 物理学 2021-02-09 Qing-Hai Tan , Kai-Xuan Xu , Yu-Jia Sun , Xue-Lu Liu , Yuan-Fei Gao , Shu-Liang Ren , Ping-Heng Tan , Jun Zhang

Based on ab initio calculations and metadynamics simulations, we predict that 2H-MoS$_2$, a layered insulator, will metallize under pressures in excess of 20-30 GPa. In the same pressure range, simulations and enthalpy optimization predict…

材料科学 · 物理学 2015-06-12 Liliana Hromadová , Roman Martoňák , Erio Tosatti

The effects of phonon anharmonicity, phonon-magnon and electron-phonon interactions on the temperature dependence of Raman optical phonon modes are theoretically investigated. Besides of the Klemens result for the phonon width due to…

强关联电子 · 物理学 2015-06-16 L. A. Falkovsky

Crystals of tetracene have been studied by means of lattice phonon Raman spectroscopy as a function of temperature and pressure. Two different phases (polymorphs I and II) have been obtained, depending on sample preparation and history.…

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

超导电性 · 物理学 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

The experimental Raman spectra of graphene exhibit a few intense two-phonon bands, which are enhanced through double-resonant scattering processes. Though there are many theoretical papers on this topic, none of them predicts the spectra…

介观与纳米尺度物理 · 物理学 2014-12-17 Valentin N. Popov , Philippe Lambin

We explore the Fano resonance in ZrTe5, using Raman scattering measurements. We identified two closely spaced B2g phonon modes, B2g I and B2g II, around 9 meV and 10 meV, respectively. Interestingly, only B2g I exhibited the Fano resonance,…

Anisotropic two-dimensional (2D) semiconductors recently have emerged as a promising platform for polarization-controlled Raman amplification. In this study, we probe energy-dependent resonant Raman scattering in few layer ReS2 under…

光学 · 物理学 2025-07-22 Pritam Das , Devarshi Chakrabarty , Neha Gill , Sajal Dhara

The asymmetric peak at 212 - 218 cm-1 occurring in InAs micro-nano wires is investigated using spatially resolved Raman spectroscopy (SRRS) of uniform, bent and long tapered MNWs grown on a Si (001) substrate. It is attributed to…

材料科学 · 物理学 2016-05-25 Vandna Kumari Gupta , Alka A. Ingale , Suparna Pal , R. Aggarwal , V. Sathe

Understanding interfacial interactions in two-dimensional (2D) heterostructures is essential for advancing optoelectronic and quantum technologies. We investigate metal-organic chemical vapor deposition (MOCVD)-grown WSe$_2$ films (one to…