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We explore pump-probe high harmonic generation (HHG) from monolayer hexagonal-Boron-Nitride, where a terahertz pump excites coherent optical phonons that are subsequently probed by an intense infrared pulse that drives HHG. We find, through…

材料科学 · 物理学 2022-06-22 Ofer Neufeld , Jin Zhang , Umberto De Giovannini , Hannes Hubener , Angel Rubio

High-order harmonic generation (HHG) has become a standard technique for producing attosecond XUV pulses in the laboratory, yet the high flux necessary for nonlinear XUV photoionization remains accessible to only a few research groups.…

Ultrafast laser driven, single-cycle THz pulsed sources hold immense potential for scientific and industrial applications; however, their limited average power hinders their widespread application. In particular, applications where high…

An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…

化学物理 · 物理学 2019-10-23 Baoning Wang , Lixin He , Yanqing He , Yinfu Zhang , Renzhi Shao , Pengfei Lan , Peixiang Lu

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

原子物理 · 物理学 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel

Chiral (highly helical) extreme ultraviolet (XUV) sources are pivotal for investigating chiroptical phenomena on the ultrafast electronic timescale. Table-top, coherent High Harmonic Generation (HHG)-based sources are particularly…

光学 · 物理学 2025-03-07 Eran Ben Arosh , Eldar Ragonis , Lev Merensky , Avner Fleischer

High-harmonic generation (HHG), the hallmark effect of attosecond science, is a nonperturbative nonlinear process leading to the emission of high-harmonic light from gases and solids. In gases, extreme driving laser pulse intensities can…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

强关联电子 · 物理学 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

光学 · 物理学 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

We describe how active feedback routines can be applied at limited repetition rate (5 Hz) to optimize high-power $>10$ TW) laser interactions with clustered gases. Optimization of x-ray production from an argon cluster jet, using a genetic…

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

光学 · 物理学 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

The combination of electronic sources operating at high frequencies and modern microwave instrumentation has enabled the recent development of chirped-pulse spectrometers for the millimetre and THz bands. This type of instrument can operate…

Plasma surface high-order harmonics generation (SHHG) driven by intense laser pulses on plasma targets enables a high-quality extreme ultraviolet source with high pulse energy and outstanding spatiotemporal coherence. Optimizing the…

等离子体物理 · 物理学 2024-11-01 Lili Fan , Ziwei Wang , Chenfei Liao , Jingwei Wang

We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…

光学 · 物理学 2025-07-15 Boyan Obreshkov , Tzveta Apostolova

Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…

Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…

光学 · 物理学 2022-07-21 Xiyuan Lu , Gregory Moille , Ashutosh Rao , Daron Westly , Kartik Srinivasan

We present a laser source delivering waveform-controlled 1.5-cycle pulses that can be focused to relativistic intensity at 1 kHz repetition rate. These pulses are generated by nonlinear compression of high-temporal-contrast sub-25\,fs…

High-order harmonic generation (HHG) from crystals offers a new source of coherent extreme ultraviolet (XUV) attosecond radiation.

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

光学 · 物理学 2016-08-02 David T. Lloyd , Kevin O'Keeffe , Patrick N. Anderson , Simon M. Hooker