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Nuclear magnetic resonance (NMR) study of the high magnetic field (H) part of the Bose-Einstein condensed (BEC) phase of the quasi-onedimensional (quasi-1D) antiferromagnetic quantum spin-chain compound NiCl2-4SC(NH2)2 (DTN) was performed.…

Quasi-one-dimensional magnet NiCl$_2\cdot$4SC(NH$_2$)$_2$, usually abbreviated as DTN, does not order at zero field down to $T=0$: due to the strong single-ion anisotropy of the "easy plane" type acting on $S=1$ Ni$^{2+}$ ions, the $S_z=0$…

强关联电子 · 物理学 2021-02-24 V. N. Glazkov

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

Magnetic adatoms on a superconducting substrate undergo a quantum phase transition as their exchange coupling to the conduction electrons increases. For quantum spins, this transition is accompanied by screening of the adatom spin. Here, we…

介观与纳米尺度物理 · 物理学 2022-06-22 Harald Schmid , Jacob F. Steiner , Katharina J. Franke , Felix von Oppen

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

We investigate various types of quantum entanglement in the octanuclear heterometallic $3d/4f$ complexes denoted as Ni$^{2+}_4$Gd$^{3+}_4$ under an external magnetic field, using the exact diagonalization approach. These molecular magnets,…

材料科学 · 物理学 2025-09-15 Hamid Arian Zad , Michal Jaščur , Azam Zoshki , Ralph Kenna , Nerses Ananikian

In Mott insulators, the strong electron-electron Coulomb repulsion prevents metallicity and charge excitations are gapped. In dimensions greater than one, their spins are usually ordered antiferromagnetically at low temperatures.…

Geometric frustration among competing spin exchanges can give rise to novel quantum phases by enhancing fluctuations that drive magnetic systems beyond the classical regime. We investigate the frustrated array of strongly correlated spin…

We report on terahertz spectroscopic measurements of quantum spin dynamics on single crystals of a spin-1/2 frustrated spin-ladder antiferromagnet BiCu$_2$PO$_6$ as a function of temperature, polarization, and applied external magnetic…

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Quantum-disordered magnetic ground states are challenging to identify in three-dimensional (3D) oxides, where strong exchange pathways typically favour long-range magnetic order or spin freezing. The quadruple perovskite…

A quantum magnetic state due to magnetic charges is never observed, even though they are treated as quantum mechanical variable in theoretical calculations. Here, we demonstrate the occurrence of a novel quantum disordered state of magnetic…

介观与纳米尺度物理 · 物理学 2021-02-25 George Yumnam , Yiyao Chen , Jiasen Guo , Jong K. Keum , Valeria Lauter , Deepak K. Singh

Competing interactions in Quantum Materials induce novel states of matter such as frustrated magnets, an extensive field of research both from the theoretical and experimental perspectives. Here, we show that competing energy scales present…

强关联电子 · 物理学 2020-07-16 J. Herbrych , J. Heverhagen , G. Alvarez , M. Daghofer , A. Moreo , E. Dagotto

In condensed matter systems, the formation of long range order (LRO) with broken symmetry is often accompanied by new types of excitations. However, in many magnetic pyrochlore oxides, geometrical frustration suppresses conventional LRO…

The 3$d^7$ Co$^{2+}$-based insulating magnet \NCTO{} has recently been reported to have strong Kitaev interactions on a honeycomb lattice, and is thus being considered as a Kitaev quantum spin liquid candidate. However, due to the existence…

The honeycomb magnet Na$_3$Co$_2$SbO$_6$ recently emerged as a promising candidate for realizing Kitaev quantum spin liquid with relatively low levels of structural disorder. While the precise spin Hamiltonian remains controversial, the…

强关联电子 · 物理学 2025-07-16 Rongsheng Li , Liyu Shi , Yuchen Gu , Yue Chen , Xintong Li , Qiong Wu , Shuxiang Xu , Dong Wu , Yuan Li , Fa Wang , Tao Dong , Nanlin Wang

We present specific-heat and neutron-scattering results for the \emph{S}=1/2 quantum antiferromagnet (dimethylammonium)(3,5-dimethylpyridinium)CuBr$_4$. The material orders magnetically at \emph{T}$_N$=1.99(2)\,K, and magnetic excitations…

Spin-orbit coupling (SOC), the intrinsic interaction between a particle spin and its motion, is responsible for various important phenomena, ranging from atomic fine structure to topological condensed matter physics. The recent experimental…

量子气体 · 物理学 2013-07-05 Yongping Zhang , Gang Chen , Chuanwei Zhang

The quantum magnetism in a three-singlet model (TSM) with singlet crystalline electric field (CEF) states interacting on a lattice is investigated, motivated by its appearance in compounds with 4f^2 and 5f^2 electronic structure. Contrary…

强关联电子 · 物理学 2021-05-04 Peter Thalmeier
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