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We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…

In previous studies of spin-to-orbital angular momentum (AM) conversion in laser high harmonic generation (HHG) using a plasma target, one unit of spin AM is always converted into precisely one unit of OAM [1, 2]. Here we show, through…

等离子体物理 · 物理学 2023-05-22 R. M. G. M. Trines , H. Schmitz , M. King , P. McKenna , R. Bingham

Although solid-state platforms underpin modern electronics, little is known about how intense ultrashort light pulses carrying orbital angular momentum (OAM) interact with solids. This gap persists even though, for more conventional…

High-harmonic generation by a laser-driven solid slab is simulated using time-dependent density functional theory. Multiple harmonic plateaus up to very high harmonic orders are observed already at surprisingly low field strengths. The full…

原子物理 · 物理学 2017-11-29 Kenneth K. Hansen , Tobias Deffge , Dieter Bauer

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

High-harmonic generation (HHG), a typical nonlinear optical effect, has been actively studied in electron systems such as semiconductors and superconductors. As a natural extension, we theoretically study HHG from electric polarization,…

强关联电子 · 物理学 2020-03-10 Tatsuhiko N. Ikeda , Masahiro Sato

Competition and cooperation among orders is at the heart of many-body physics in strongly correlated materials and leads to their rich physical properties. It is crucial to investigate what impact many-body physics has on extreme nonlinear…

强关联电子 · 物理学 2022-04-06 K. Uchida , G. Mattoni , S. Yonezawa , F. Nakamura , Y. Maeno , K. Tanaka

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

原子物理 · 物理学 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

A fully electrically interfaced chip-scale Micro-Electro-Mechanical System based higher-order harmonic generator has multitudes of applications as it can simultaneously facilitate monolithic integration with on-chip electronics and offer…

应用物理 · 物理学 2019-10-03 Gayathri Pillai , Sheng-Shian Li

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

量子物理 · 物理学 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

原子物理 · 物理学 2026-04-23 Aaron T. Bondy , Klaus Bartschat

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

原子物理 · 物理学 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

We present a theoretical study of high-order harmonic generation (HHG) driven by ultrashort optical pulses with different kind of chirps. The goal of the present work is perform a detailed study to clarify the relevant parameters in the…

原子物理 · 物理学 2016-12-21 E Neyra , F Videla , J A Pérez-Hernández , M F Ciappina , L Roso , G A Torchia

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

A new physical mechanism to achieve spin-to-orbital angular momentum conversion based on the interaction of an intense circularly polarized (CP) laser beam with a plane foil is presented and studied for the first time. It has been verified…

等离子体物理 · 物理学 2019-03-13 Shasha Li , Xiaomei Zhang , Weifeng Gong , Zhigang Bu , Baifei Shen

Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

光学 · 物理学 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

We investigate the non linear mixing of orbital angular momentum in type II second harmonic generation with arbitrary topological charges imprinted on two orthogonally polarized beams. Starting from the basic nonlinear equations for the…

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

原子物理 · 物理学 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

原子物理 · 物理学 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

原子物理 · 物理学 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin