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A theory describing the forces governing the self-assembly of nanoparticles at the solid-liquid interface is developed. In the process, new theoretical results are derived to describe the effect that the field penetration of a point-like…

介观与纳米尺度物理 · 物理学 2017-09-19 Ryan-Rhys Griffiths

The directed self-assembly of colloidal nanoparticles (NPs) using external fields guides the formation of sophisticated hierarchical materials but becomes less effective with decreasing particle size. As an alternative, electron-beam-driven…

软凝聚态物质 · 物理学 2024-09-13 Jonathan G. Raybin , Ethan J. Dunsworth , Veronica Guo , Naomi S. Ginsberg

Self-assembly processes provide the means to achieve scalable and versatile metamaterials by "bottom-up" fabrication. Despite their enormous potential, especially as a platform for energy materials, self-assembled metamaterials are often…

应用物理 · 物理学 2023-03-09 Jelena Wohlwend , Georg Haberfehlner , Henning Galinski

Studies of nanoparticle-based optical matter have only considered spherical constituents. Yet nanoparticles with other shapes are expected to have different local electromagnetic field distributions and therefore interactions with neighbors…

介观与纳米尺度物理 · 物理学 2018-08-01 Delphine Coursault , Nishant Sule , John Parker , Ying Bao , Norbert F. Scherer

The spontaneous assembly of particles in suspension provides a strategy for inexpensive fabrication of devices with nanometer-scale control, such as single-electron transistors for memory or logic applications. A scaleable and robust method…

We use numerical simulations to show how noninteracting hard particles binding to a deformable elastic shell may self-assemble into a variety of linear patterns. This is a result of the nontrivial elastic response to deformations of shells.…

软凝聚态物质 · 物理学 2011-02-25 Andela Šarić , Angelo Cacciuto

Elastic sheets with macroscopic dimensions are easy to deform by bending and stretching. Yet shaping nanometric sheets by mechanical manipulation is hard. Here we show that nanoparticle self-assembly could be used to this end. We…

软凝聚态物质 · 物理学 2015-05-20 Josep C. Pàmies , Angelo Cacciuto

Self-assembly processes allow us to design and create complex nanostructures using molecules as building blocks and surfaces as scaffolds. This autonomous driven construction is possible due to a complex thermodynamic balance of…

介观与纳米尺度物理 · 物理学 2017-09-06 Sabrina Simoncelli , Yi Li , Emiliano Cortés , Stefan A. Maier

Colloidal particles can self-assemble into various ordered structures in fluid flows that have potential applications in biomedicine, materials synthesis and encryption. These dynamic processes are also of fundamental interest for probing…

软凝聚态物质 · 物理学 2017-01-31 Yu Abe , Bo Zhang , Leonardo Gordillo , Alireza Mohammad Karim , Lorraine F. Francis , Xiang Cheng

We discuss two aspects of the plasmofluidic assembly of plasmonic nanostructures at the metal fluid interface. First, we experimentally show how three and four spot evanescent wave excitation can lead to unconventional assembly of plasmonic…

A multiple-image method is developed to accurately calculate the electrostatic interaction between neutral dielectric particles and a uniformly charged dielectric substrate. The difference in dielectric constants between the particle and…

软凝聚态物质 · 物理学 2024-12-18 Xin Li , Changhao Li , Xiangui Chen , Zaixin Wang , Sun Min , Decai Huang

We report experiments, modeling and numerical simulations of the self--assembly of particle patterns obtained from a nanometric metallic square grid. Initially, nickel filaments of rectangular cross section are patterned on a SiO$_2$ flat…

The combination of soft responsive particles, such as microgels, with nanoparticles (NPs) yields highly versatile complexes of great potential for applications, from ad-hoc plasmonic sensors to controlled protocols for loading and release.…

Engineered nanoparticles made from noble metals, rare-earth oxides or semiconductors are emerging as the central constituents of future nanotech developments. In this review, a survey of the complexing strategies between nanoparticles and…

材料科学 · 物理学 2011-08-25 J. -P. Chapel , J. -F. Berret

Self-assembly of nanoparticles at fluid-fluid interfaces is a promising route to fabricate functional materials from the bottom-up. However, directing and controlling particles into highly tunable and predictable structures -- while…

软凝聚态物质 · 物理学 2019-09-25 Qingguang Xie , Gary B. Davies , Jens Harting

Hierarchical self-assembly arranges nanostructures at different length scales. It gradually becomes an effective method of fabricating artificial metamaterials from composite nanostructures tailored for a particular response. Hierarchical…

Despite tremendous progress in the research on self-assembled nanotechnological building blocks such as macromolecules, nanowires, and two-dimensional materials, synthetic self-assembly methods bridging nanoscopic to macroscopic dimensions…

During the last 3 years, our group has investigated extensively the complexation mechanism between neutral-polyelectrolyte block copolymers with oppositely charged species. These species are surfactant micelles, multivalent counterions and…

软凝聚态物质 · 物理学 2007-05-23 J. -F. Berret , P. Herve , M. Morvan , K. Yokota , M. Destarac , J. Oberdisse , I. Grillo , R. Schweins

We develop equilibrium and kinetic theories that describe the assembly of viral capsid proteins on a charged central core, as seen in recent experiments in which brome mosaic virus (BMV) capsids assemble around nanoparticles functionalized…

生物大分子 · 定量生物学 2009-05-06 Michael F. Hagan

Based on experimental and simulation methods we helped develop, we are advancing mechanistic understanding of how self-assembled NC metamaterials can produce distinctive near- and far-field optical properties not readily achievable in…

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