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Frequency up-conversion, enabled by molecular optomechanical coupling, has recently emerged as a promising approach for converting infrared signals into the visible range through quantum coherent conversion of signals. However, detecting…

量子物理 · 物理学 2024-04-17 Fen Zou , Lei Du , Yong Li , Hui Dong

Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity…

光学 · 物理学 2017-01-17 Maxim V. Gorkunov , Alexander N. Darinskii , Alexey V. Kondratov

In the context of the quantum-mechanical description of single-molecule surface-enhanced Raman scattering, intensity-field correlation measurements of photons emitted from a plasmonic cavity are explored, theoretically, using the technique…

量子物理 · 物理学 2019-07-10 Octavio de los Santos Sánchez

The spectral properties of a variety of improved staggered operators are studied in quenched QCD. The systematic dependence of the infrared eigenvalue spectrum on i) improvement in the staggered operator, ii) improvement in the gauge field…

高能物理 - 格点 · 物理学 2009-11-10 Kit Yan Wong , R. M. Woloshyn

In this review, we discuss the use of continuous variable spectroscopy techniques for investigating quantum coherence and light-matter interactions in semiconductor systems with ultrafast dynamics. We focus on multichannel homodyne…

介观与纳米尺度物理 · 物理学 2023-06-05 Carolin Lüders , Franziska Barkhausen , Matthias Pukrop , Elena Rozas , Jan Sperling , Stefan Schumacher , Marc Aßmann

We theoretically investigate a scheme in which backward coherent anti-Stokes Raman scattering (CARS) is significantly enhanced by using slow light. Specifically, we reduce the group velocity of the Stokes excitation pulse by introducing a…

光学 · 物理学 2017-01-03 Li Gong , Haifeng Wang

Time-resolved Raman spectroscopy techniques offer various ways to study the dynamics of molecular vibrations in liquids or gases and optical phonons in crystals. While these techniques give access to the coherence time of the vibrational…

量子物理 · 物理学 2021-04-06 Santiago Tarrago Velez , Vivishek Sudhir , Nicolas Sangouard , Christophe Galland

The homochirality of biomolecules remains one of the outstanding puzzles concerning the beginning of life. Chiral amplification of a randomly perturbed racemic mixture of chiral molecules is a well-accepted prerequisite for all routes to…

化学物理 · 物理学 2022-10-12 Uri Hananel , Assaf Ben-Moshe , Haim Diamant , Gil Markovich

Coherent Raman scattering microscopy is a fast, label-free and chemically specific imaging technique that has a high potential for future in-vivo optical histology. However, its imaging depth into tissues is limited to the sub-millimeter…

Surface Enhanced Raman Spectroscopy (SERS) is a highly sensitive and selective technique that greatly enhances the signal of an analyte, compared with its signal from classical Raman Spectroscopy, due to its interaction with a substrates…

材料科学 · 物理学 2025-10-20 Jan Komeda , Antonio Cammarata , Tomas Polcar

Spin-polarised atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that…

量子物理 · 物理学 2022-05-11 Alexander Roth , Klemens Hammerer , Kirill S. Tikhonov

We discuss layout and performance of a high-resolution Stimulated Raman Loss spectrometer that has been newly developed for accurate studies of spectral lineshapes and line center frequencies of hydrogen isotopologues and in general of…

光学 · 物理学 2023-04-06 M. Lamperti , L. Rutkowski , D. Gatti , R. Gotti , L. Moretti , D. Polli , G. Cerullo , M. Marangoni

Locally chiral light is an emerging tool for probing and controlling molecular chirality. It can generate large and freely adjustable enantioselectivities in purely electric-dipole effects, offering its major advantages over traditional…

光学 · 物理学 2023-10-19 Chong Ye , Yifan Sun , Libin Fu , Xiangdong Zhang

The average Raman signal power obtained in a modulated optical trap is dependent on the Brownian motion - therefore hydrodynamic properties of the trapped particle. Hence, in addition to the molecular properties obtained from the Raman…

光学 · 物理学 2023-11-27 Rohin Sharma , Anusa Thapa , Rijan Maharjan , Ashim Dhakal

To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…

材料科学 · 物理学 2024-09-04 Akihito Kato , Nobuhiko Yokoshi

Combined frequency-resolved techniques are suitable to study electrochromic (EC) materials. We present an experimental setup for simultaneous electrochemical and color impedance studies of EC systems in transmission mode and estimate its…

应用物理 · 物理学 2020-01-22 Edgar A. Rojas-González , Gunnar A. Niklasson

Chiral light matter interaction enables new fundamental researches and applications of light. The interaction has traditionally faced challenges in low directionality and efficiency based on spin orbit interaction of light in microscopic…

应用物理 · 物理学 2019-12-10 Liang Fang , Haozhi Luo , Xiaoping Cao , Shuang Zheng , Xinlun Cai , Jian Wang

Chiral objects typically exhibit a different extinction for the two circular polarizations of light. Researchers often detect the chirality of objects by measuring this extinction difference employing Circular Dichroism (CD) spectroscopy.…

We report on the first demonstration of nonlinear dual-frequency-comb spectroscopy. In multi-heterodyne femtosecond Raman-induced Kerr-effect spectroscopy, the Raman gain resulting from the coherent excitation of molecular vibrations by a…

Optical coherence tomography is state-of-the-art in non-invasive imaging of biological structures. Spectral Domain Optical Co-herence Tomography is the popularly used variation of this technique, but its performance is limited by the…

光学 · 物理学 2023-03-01 Prabhav Gaur , Andrew Grieco , Yeshaiahu Fainman