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We have investigated the electronic excitations in bulk 2H-MoS2 using electron energy-loss spectroscopy. The electron energy-loss spectra in the {\Gamma}M and {\Gamma}K directions were measured for various momentum transfer values. The…

介观与纳米尺度物理 · 物理学 2015-06-18 Carsten Habenicht , Martin Knupfer , Bernd Büchner

We have investigated indirect excitons in bulk $2H$-MoS$_2$ using transmission electron energy-loss spectroscopy. The electron energy-loss spectra were measured for various momentum transfer values parallel to the $\Gamma$K and $\Gamma$M…

介观与纳米尺度物理 · 物理学 2018-05-07 Carsten Habenicht , Roman Schuster , Martin Knupfer , Bernd Büchner

In this letter we report a thorough analysis of the exciton dispersion in bulk hexagonal boron nitride. We solve the ab initio GW Bethe-Salpeter equation at finite $\mathbf{q}\parallel \Gamma K$, and we compare our results with recent…

介观与纳米尺度物理 · 物理学 2018-02-22 Lorenzo Sponza , Hakim Amara , Claudio Attaccalite , François Ducastelle , Annick Loiseau

We combine electron energy-loss spectroscopy (EELS) and density functional theory (DFT) calculations to study the dispersion and effective mass of excitons in the bulk of WSe$_2$. Our EELS data suggest substantial deviations from the…

介观与纳米尺度物理 · 物理学 2016-08-10 R. Schuster , Y. Wan , M. Knupfer , B. Büchner

Using first-principles GW plus Bethe-Salpeter equation calculations, we identify anomalously strong excitonic effects in several vacancy-ordered double perovskites Cs2MX6 (M = Ti, Zr; X = I, Br). Giant exciton binding energies about 1 eV…

计算物理 · 物理学 2023-06-21 Fan Zhang , Weiwei Gao , Greis J. Cruz , Yi-yang Sun , Peihong Zhang , Jijun Zhao

Bose condensation has shaped our understanding of macroscopic quantum phenomena, having been realized in superconductors, atomic gases, and liquid helium. Excitons are bosons that have been predicted to condense into either a superfluid or…

Atomically precise lateral heterojunctions based on transition metal dichalcogenides provide a new platform for exploring exciton Mott transition in one-dimension. To investigate the intrinsically non-equilibrium Mott transition, we…

介观与纳米尺度物理 · 物理学 2021-11-16 Long Yuan , Biyuan Zheng , Qiuchen Zhao , Roman Kempt , Thomas Brumme , Agnieszka Beata Kuc , Chao Ma , Shibin Deng , Anlian Pan , Libai Huang

There are conflicting predictions and reports on the character of the exciton Mott transition (EMT) in monolayer transition metal dichalcogenides. It could be either a discontinuous or a continuous transition from the excitonic to the…

材料科学 · 物理学 2026-01-27 Subhadra Mohapatra , Samuel Palato , Nicholas Olsen , Julia Stähler , Lukas Gierster

Moir\'e superlattices of transition-metal dichalcogenides (TMDs) host strongly interacting Bose-Fermi mixtures in which bosonic excitons coexist with correlated electron lattices. Using ultrafast, time- and energy-resolved photoluminescence…

Excitons -- elementary excitations formed by bound electron-hole pairs -- govern the optical properties and excited-state dynamics of materials. In two-dimensions (2D), excitons are theoretically predicted to have a linear energy-momentum…

材料科学 · 物理学 2025-03-14 Luna Y. Liu , Steffi Y. Woo , Jinyuan Wu , Bowen Hou , Cong Su , Diana Y. Qiu

Photoluminescence spectra measured on a type-II GaSb/GaAs quantum dot ensemble at high excitation power indicate a Mott transition from the low density state comprising of spatially-indirect excitons to a high density electron-plasma state.…

其他凝聚态物理 · 物理学 2009-11-13 Bhavtosh Bansal , M. Hayne , M. Geller , D. Bimberg , V. V. Moshchalkov

Several theoretical predictions have claimed that the neutral exciton of TMDCs splits into a transversal and longitudinal exciton branch, with the longitudinal one, which is the upper branch, exhibiting an extraordinary strong dispersion in…

介观与纳米尺度物理 · 物理学 2020-05-29 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Excitonic effects due to the correlation of electrons and holes in excited states of matter dominate the optical spectra of many interesting materials. They are usually studied in the long-wavelength limit. Here we investigate excitons at…

材料科学 · 物理学 2023-04-18 Vitaly Gorelov , Lucia Reining , Matteo Gatti

When electron-hole pairs are excited in a semiconductor, it is a priori not clear if they form a fermionic plasma of unbound particles or a bosonic exciton gas. Usually, the exciton phase is associated with low temperatures. In atomically…

Transition metal dichalcogenides layered nano-crystals are emerging as promising candidates for next-generation optoelectronic and quantum devices. In such systems, the interaction between excitonic states and atomic vibrations is crucial…

介观与纳米尺度物理 · 物理学 2023-12-29 Jianbo Hu , Yang Xiang , Beatrice Matilde Ferrari , Emilio Scalise , Giovanni Maria Vanacore

Exciton Mott physics in two-dimensional electron-hole (e-h) systems is studied in the quasiequilibrium, which is the crossovers or phase transitions between the insulating exciton gas and the metallic e-h plasma. By developing a…

量子气体 · 物理学 2014-07-08 Kenichi Asano , Takuya Yoshioka

Understanding and controlling the way excitons propagate in solids is a key for tailoring materials with improved optoelectronic properties. A fundamental step in this direction is the determination of the exciton energy-momentum…

Spontaneous condensation of excitons is a long sought phenomenon analogous to the condensation of Cooper pairs in a superconductor. It is expected to occur in a semiconductor at thermodynamic equilibrium if the binding energy of the…

强关联电子 · 物理学 2021-03-25 S. Samaneh Ataei , Daniele Varsano , Elisa Molinari , Massimo Rontani

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

材料科学 · 物理学 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

We present a unified description of the excitonic properties of four monolayer transition-metal dichalcogenides (TMDC's) using an equation of motion method for deriving the Bethe-Salpeter equation in momentum space. Our method is able to…

介观与纳米尺度物理 · 物理学 2017-08-08 A. J. Chaves , R. M. Ribeiro , T. Frederico , N. M. R. Peres
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