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A theory of electronic transport through molecular wires is applied to analyze characteristics of a long-range electron transfer (ET) through molecular bridges in macromolecules with complex donor/acceptor subsystems. Assuming a coherent…

软凝聚态物质 · 物理学 2007-05-23 Natalya A. Zimbovskaya

The Planar Model of the Electrode-Vacuum-Electrode configuration for STM in which electrode surfaces are assumed to be infinite parallel planes, with atomic size separation and vacuum between them, is used to calculate tunneling current…

其他凝聚态物理 · 物理学 2023-01-04 Malati Dessai , Arun V. Kulkarni

This thesis investigates the mechanically controlled break junctions, with a particular emphasis on elucidating the behaviour of molecular currents at room temperature. The core of this experimental investigation involves a detailed…

介观与纳米尺度物理 · 物理学 2024-09-17 Giovanna Angelis Schmidt

We developed the theory of elastic electron tunneling through a potential barrier driven by a strong high-frequency electromagnetic field. It is demonstrated that the driven barrier can be considered as a stationary two-barrier potential…

介观与纳米尺度物理 · 物理学 2023-11-13 M. V. Boev , V. M. Kovalev , O. V. Kibis

We demonstrate that a simple phenomenological approach can be used to simulate electronic conduction in molecular wires under thermal effects induced by the surrounding environment. This "Landauer-B\"uttiker's probe technique" can properly…

化学物理 · 物理学 2015-08-25 Michael Kilgour , Dvira Segal

We investigate the time-dependent, coherent, and dissipative dynamics of bound particles in single multilevel quantum dots in the presence of sequential tunnelling transport. We focus on the nonequilibrium regime where several channels are…

介观与纳米尺度物理 · 物理学 2010-02-11 Eduardo Vaz , Jordan Kyriakidis

The transport properties of a tunnel barrier in a one-dimensional wire are investigated at finite voltages and temperatures. We generalize the Luttinger model to account for finite ranges of the interaction. This leads to deviations from…

介观与纳米尺度物理 · 物理学 2009-10-30 Margit Steiner , Wolfgang Häusler

In this work we theoretically study steady state thermoelectric transport through a single-molecule junction with a long chain-like bridge. Electron transmission through the system is computed using a tight-binding model for the bridge. We…

介观与纳米尺度物理 · 物理学 2018-03-02 Natalya A. Zimbovskaya , Abraham Nitzan

The traditional transmission coefficient present in the original Landauer formulation, which is valid for quasi-static scenarios with working frequencies below the inverse of the electron transit time, is substituted by a novel…

介观与纳米尺度物理 · 物理学 2021-03-24 Matteo Villani , Simone Clochiatti , Werner Prost , Nils Weimann , Xavier Oriols

Inspired by recent experimental findings that will be presented elsewhere, we formulate and investigate a model of a superconducting junction that combines the electron propagation in a quantum channel with an arbitrary transmission, and…

介观与纳米尺度物理 · 物理学 2022-01-21 Hristo Barakov , Yuli V. Nazarov

This paper extends the modern theory of tunneling transport to finite temperatures. The extension enables applications to molecular electronic devices connected to semiconducting leads. The paper presents an application of the theory to…

介观与纳米尺度物理 · 物理学 2010-02-08 Emil Prodan , Amy LeVee

We consider exciton effects on current in molecular nanojunctions, using a model comprising a two two-level sites bridge connecting free electron reservoirs. Expanding the density operator in the many-electron eigenstates of the uncoupled…

强关联电子 · 物理学 2015-05-14 GuangQi Li , Boris D. Fainberg , Abraham Nitzan , Sigmund Kohler , Peter Hänggi

Understanding electron transport processes in molecular wires connected between contacts is a central focus in the field of molecular electronics. Especially, the dephasing effect causing tunneling-to-hopping transition has great importance…

介观与纳米尺度物理 · 物理学 2012-06-26 Daijiro Nozaki , Claudia Gomes da Rocha , Horacio M. Pastawski , Gianaurelio Cuniberti

A review of the present state of investigations of the pseudospin-electron model (PEM), which is used in the theory of strongly correlated electron systems, is given. The model is used to describe the systems with the locally anharmonic…

强关联电子 · 物理学 2016-11-23 Ihor Stasyuk

Modeling of electron transport through organic molecules is presented in order to interpret the experimental data of Rosink et al. [PRB 62, 10459 (2000)]. Such results are understand as coherent off-resonance tunneling through the junction…

软凝聚态物质 · 物理学 2007-05-23 Kamil Walczak

On the basis of the Keldysh method of non-equilibrium systems, we develop a theory of electron tunneling in normal-metal/superconductor junctions. By using the tunneling Hamiltonian model (being appropriate for the tight-binding systems),…

超导电性 · 物理学 2009-10-31 Xin-Zhong Yan , Hongwei Zhao , Chia-Ren Hu

Redox molecular junctions are molecular conduction junctions that involve more than one oxidation state of the molecular bridge. This property is derived from the ability of the molecule to transiently localize transmitting electrons,…

介观与纳米尺度物理 · 物理学 2013-06-21 Agostino Migliore , Abraham Nitzan

Work is devoted to physics of current transport in a wide class of the hetero-phase granulated mediums and similar systems with set of metal or semi-conductor granules, quantum dots or potential wells in which the exit from Coulomb blockade…

介观与纳米尺度物理 · 物理学 2013-08-13 E. S. Demidov , N. E. Demidova

Quantitative description of charge transport across tunneling and break-junction devices with novel superconductors encounters some problems not present, or not as severe for traditional superconducting materials. In this work, we explain…

超导电性 · 物理学 2016-08-11 E. Zhitlukhina , I. Devyatov , O. Egorov , M. Belogolovskii , P. Seidel

We consider the conductance of a one-dimensional wire interrupted by a double-barrier structure allowing for a resonant level. Using the electron-electron interaction strength as a small parameter, we are able to build a non-perturbative…

介观与纳米尺度物理 · 物理学 2009-11-07 Yu. V. Nazarov , L. I. Glazman