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Recent experiments on vesicles formed from block copolymers with liquid-crystalline side-chains reveal a rich variety of vesicle morphologies. The additional internal order ("structure") developed by these self-assembled block copolymer…

软凝聚态物质 · 物理学 2012-05-21 Xiangjun Xing , Homin Shin , Mark J. Bowick , Zhenwei Yao , Lin Jia , Min-Hui Li

Polymer vesicles are stable robust vesicles made from block copolymer amphiphiles. Recent progress in the chemical design of block copolymers opens up the exciting possibility of creating a wide variety of polymer vesicles with varying fine…

软凝聚态物质 · 物理学 2009-09-02 Lin Jia , Amin Cao , Daniel Levy , Bing Xu , Pierre-Antoine Albouy , Xiangjun Xing , Mark J. Bowick , Min-Hui Li

We investigate experimentally and numerically the defect configurations emerging when a cholesteric liquid crystal is confined to a spherical shell. We uncover a rich scenario of defect configurations, some of them non-existent in nematic…

软凝聚态物质 · 物理学 2017-09-13 Alexandre Darmon , Michael Benzaquen , Simon Čopar , Olivier Dauchot , Teresa Lopez-Leon

Polyhedral vesicles with a large bending modulus of the membrane such as the gel phase lipid membrane were studied using a Brownian dynamics simulation. The vesicles exhibit various polyhedral morphologies such as tetrahedron and cube…

软凝聚态物质 · 物理学 2009-11-07 Hiroshi Noguchi

The phase behavior of the system of parallel rigid triblock copolymers is examined using the second-virial density functional theory. The triblock particle consists of two identical infinitely thin hard rods of finite lengths on the…

软凝聚态物质 · 物理学 2007-10-15 Szabolcs Varga , Seth Fraden

The dynamics of active smectic liquid crystals confined on a spherical surface is explored through an active phase field crystal model. Starting from an initially randomly perturbed isotropic phase, several types of topological defects are…

软凝聚态物质 · 物理学 2025-03-11 Michael Nestler , Simon Praetorius , Zhi-Feng Huang , Hartmut Löwen , Axel Voigt

We study the organization of topological defects in a system of nematogens confined to the two-dimensional sphere (S^2). We first perform Monte Carlo simulations of a fluid system of hard rods (spherocylinders) living in the tangent plane…

软凝聚态物质 · 物理学 2009-11-13 Homin Shin , Mark J. Bowick , Xiangjun Xing

Smectic liquid crystals are charcterized by layers that have a preferred uniform spacing and vanishing curvature in their ground state. Dislocations in the smectics play an important role in phase nucleation, layer reorientation, and…

软凝聚态物质 · 物理学 2017-06-28 Hillel Aharoni , Thomas Machon , Randall D. Kamien

Grain boundaries in extremely confined colloidal smectics possess a topological fine structure with coexisting nematic and tetratic symmetry of the director field. An alternative way to approach the problem of smectic topology is via the…

软凝聚态物质 · 物理学 2024-04-24 René Wittmann

The interplay between geometry, topology and order can lead to geometric frustration that profoundly affects the shape and structure of a curved surface. In this commentary we show how frustration in this context can result in the faceting…

软凝聚态物质 · 物理学 2016-02-02 Mark Bowick , Rastko Sknepnek

We study the topology of smectic defects in two and three dimensions. We give a topological classification of smectic point defects and disclination lines in three dimensions. In addition we describe the combination rules for smectic point…

软凝聚态物质 · 物理学 2019-11-19 Thomas Machon , Hillel Aharoni , Yichen Hu , Randall D. Kamien

We study the phase behaviour of cholesteric liquid crystal shells with different geometries. We compare the cases of tangential and no anchoring at the surface, focussing on the former case, which leads to a competition between the…

软凝聚态物质 · 物理学 2023-03-01 Giuseppe Negro , Livio Nicola Carenza , Giuseppe Gonnella , Davide Marenduzzo , Enzo Orlandini

A theoretical study of vesicles of topological genus zero is presented. The bilayer membranes forming the vesicles have various degrees of intrinsic (tangent-plane) orientational order, ranging from smectic to hexatic, frustrated by…

凝聚态物理 · 物理学 2009-10-28 R. M. L. Evans

Liquid crystals can self-organize into a layered smectic phase. While the smectic layers are typically straight forming a lamellar pattern in bulk, external confinement may drastically distort the layers due to the boundary conditions…

Smectic liquid crystals are materials formed by stacking deformable, fluid layers. Though smectics prefer to have flat, uniformly-spaced layers, boundary conditions can impose curvature on the layers. Since the layer spacing and curvature…

微分几何 · 数学 2007-05-23 Randall D. Kamien , Christian D. Santangelo

We study the phase behaviour of a quasi-two dimensional cholesteric liquid crystal shell. We characterise the topological phases arising close to the isotropic-cholesteric transition, and show that they differ in a fundamental way from…

软凝聚态物质 · 物理学 2022-08-25 Livio Nicola Carenza , Giuseppe Gonnella , Davide Marenduzzo , Giuseppe Negro , Enzo Orlandini

Using computer simulations we investigate the microscopic structure of the singular director field within a nematic droplet. As a theoretical model for nematic liquid crystals we take hard spherocylinders. To induce an overall topological…

软凝聚态物质 · 物理学 2009-10-31 J. Dzubiella , M. Schmidt , H. Loewen

A series of amphiphilic LC block copolymers, in which the hydrophobic block is a smectic polymer poly(4-methoxyphenyl 4-(6-acryloyloxy-hexyloxy)-benzoate) (PA6ester1) and the hydrophilic block is polyethyleneglycol (PEG), were synthesized…

软凝聚态物质 · 物理学 2009-09-04 B. Xu , R. Pinol , M. Nono-Djamen , S. Pensec , P. Keller , P. -A. Albouy , D. Levy , M. -H. Li

The known ground state of ultrathin smectic films confined to the surface of a sphere is described by four +1/2 defects assembled on a great circle and a director which follows geodesic lines. Using a simple perturbative approach we show…

软凝聚态物质 · 物理学 2016-01-12 O. V. Manyuhina , M. J. Bowick

Topological defects play a central role in the formation and organization of various biological systems. Historically, such nonequilibrium defects have been mainly studied in the context of homogeneous active nematics. Phase-separated…

软凝聚态物质 · 物理学 2023-07-13 Timo Krüger , Ivan Maryshev , Erwin Frey
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