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We use ab initio electronic structure calculations in combination with Monte Carlo simulations to investigate the magnetic and ferroelectric properties of bulk orthorhombic HoMnO$_3$ and ErMnO$_3$. Our goals are to explain the…

材料科学 · 物理学 2018-12-12 Natalya S. Fedorova , Amadé Bortis , Christoph Findler , Nicola A. Spaldin

The crystal and magnetic structure of polycrystalline $La{}_{0.5-x}Nd{}_{x}Ca_{0.5}MnO{}_{3}$ (0.0 \ensuremath{\le} x \ensuremath{\le} 0.5) samples have been investigated using magnetization, resistivity, transmission electron microscope,…

材料科学 · 物理学 2010-11-01 Indu Dhiman , A. Das , P. K. Mishra , N. P. Lalla , A. Kumar

Controlling material properties by modulating the crystalline structure has been attempted using various techniques, e.g., hydrostatic pressure, chemical pressure, and epitaxy. These techniques succeed to improve properties and achieve…

The magnetic correlations in double perovskites La2Mn2-xNixO6 (x = 0.5, 0.75, 1.0, 1.25 and 1.5) have been systematically investigated across macroscopic, mesoscopic, and microscopic length scales using temperature-dependent bulk DC…

材料科学 · 物理学 2025-10-14 A. K. Bera , K. S. Chikara , B. Saha , S. M. Yusuf , Mohd. Nasir , S. Sen

Strain is a leading candidate for controlling magnetoelectric coupling in multiferroics. Here, we use x-ray diffraction to study the coupling between magnetic order and structural distortion in epitaxial films of the orthorhombic (o-)…

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

强关联电子 · 物理学 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Complex oxide thin films and heterostructures offer a wide range of properties originating from the intrinsic coupling between lattice strain and magnetic/electronic ordering. This article reviews experimental, phenomenological, and…

强关联电子 · 物理学 2023-10-20 Surendra Singh

The crystal and magnetic structures of the specified CMR manganite system have been studied as a function of $y=(0.2-1)$ across the metal-insulator (MI) transition, and of the oxygen mass ($^{16}$O, $^{18}$O). We quantitatively show how the…

强关联电子 · 物理学 2011-04-12 V. Yu. Pomjakushin , D. V. Sheptyakov , K. Conder , E. V. Pomjakushina , A. M. Balagurov

We use first-principles calculations based on density functional theory to investigate the interplay between oxygen vacancies, A-site cation size / tolerance factor, epitaxial strain, ferroelectricity and magnetism in the perovskite…

We use ab initio electronic structure calculations within the generalized gradient approximation (GGA+U) to density functional theory (DFT) to determine the microscopic exchange interactions in the series of orthorhombic rare-earth…

材料科学 · 物理学 2015-04-22 Natalya S. Fedorova , Claude Ederer , Nicola A. Spaldin , Andrea Scaramucci

We study how strain affects orbital ordering and magnetism at the interface between SrMnO$_3$ and LaMnO$_3$ from density-functional calculations and interpret the basic results in terms of a three-site Mn-O-Mn model. Magnetic interaction…

材料科学 · 物理学 2010-03-10 B. R. K. Nanda , S. Satpathy

Rare-earth manganites are fascinating, because they display a wide variety of fundamental properties from magnetism to ferroelectricity, from colossal magnetoresistance to semi-metallicity, and because they can be used in a number of…

其他凝聚态物理 · 物理学 2007-05-23 V. Lovchinov , A. Apostolov , D. Dimitrov , I. Radulov , Ph. Vanderbemden

Orthorhombically distorted perovskite manganites, RMnO3 with R being a trivalent rare-earth ion, exhibit a variety of magnetic and electric phases including multiferroic (i.e. concurrently magnetic and ferroelectric) phases and fascinating…

强关联电子 · 物理学 2016-09-08 Masahito Mochizuki , Nobuo Furukawa

By combining dielectric, specific heat, and magnetization measurements and high-resolution neutron powder diffraction, we have investigated the thermodynamic and magnetic/structural properties of the metastable orthorhombic perovskite…

强关联电子 · 物理学 2007-08-02 F. Ye , B. Lorenz , Q. Huang , Y. Q. Wang , Y. Y. Sun , C. W. Chu , J. A. Fernandez-Baca , Pengcheng Dai , H. A. Mook

The single phase polycrystalline Ba1/4Sr3/4MnO3 layered perovskite manganite has been synthesized by combustion method having various crystallite sizes. The room temperature X-ray diffraction patterns reveal that Ba1/4Sr3/4MnO3 crystallizes…

材料科学 · 物理学 2018-11-30 Dinesh Kumar , Monika Singh , Akhilesh Kumar Singh

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

强关联电子 · 物理学 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

We report a x-ray resonant diffraction study of the perovskite Pr0.6Ca0.4MnO3. At the Mn K-edge, this technique is sensitive to details of the electronic structure of the Mn atoms. We discuss the resonant x-ray spectra measured above and…

Magnetically-driven ferroelectric atomic displacements of the order of 10$^{-3} Angstrom have been observed in orthorhombic (perovskite like) YMnO$_3$ by a single-crystal synchrotron x-ray diffraction. The refined polar structure shows the…

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

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