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Magnetically-Driven Ferroelectric Atomic Displacements in perovskite like YMnO3

Strongly Correlated Electrons 2011-08-12 v1

Abstract

Magnetically-driven ferroelectric atomic displacements of the order of 103Angstromhavebeenobservedinorthorhombic(perovskitelike)YMnO^{-3} Angstrom have been observed in orthorhombic (perovskite like) YMnO_3byasinglecrystalsynchrotronxraydiffraction.TherefinedpolarstructureshowsthecharacteristicbondalternationdrivenbytheexchangestrictioninstaggeredMnOMnarrayswith by a single-crystal synchrotron x-ray diffraction. The refined polar structure shows the characteristic bond alternation driven by the exchange striction in staggered Mn-O-Mn arrays with \uparrow\uparrow\downarrow\downarrow$ type ordering, giving rise to a spontaneous polarization along a-axis. First-principles calculations based on the Berry phase method as well as on the experimentally refined crystal structure can reproduce the observed polarization value.

Keywords

Cite

@article{arxiv.1107.2467,
  title  = {Magnetically-Driven Ferroelectric Atomic Displacements in perovskite like YMnO3},
  author = {D. Okuyama and S. Ishiwata and Y. Takahashi and K. Yamauchi and S. Picozzi and K. Sugimoto and H. Sakai and M. Takata and R. Shimano and Y. Taguchi and T. Arima and Y. Tokura},
  journal= {arXiv preprint arXiv:1107.2467},
  year   = {2011}
}

Comments

8 pages, 5 figures, 2 tables

R2 v1 2026-06-21T18:35:56.815Z