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The mechanical properties of soft matter are of great importance in countless applications, in addition of being an active field of academic research. Given the relative ease with which soft materials can be deformed, their non-linear…

软凝聚态物质 · 物理学 2020-05-25 Luca Cipelletti , Kirsten Martens , Laurence Ramos

Colloidal gel networks are disordered elastic solids that can form even in extremely dilute particle suspensions. With interaction strengths comparable to the thermal energy, their stress-bearing network can locally restructure via breaking…

软凝聚态物质 · 物理学 2014-06-18 Jader Colombo , Asaph Widmer-Cooper , Emanuela Del Gado

By means of molecular dynamics, we study the structure and the dynamics of a microscopic model for colloidal gels at low volume fractions. The presence of directional interactions leads to the formation of a persistent interconnected…

软凝聚态物质 · 物理学 2010-01-02 Emanuela Del Gado , Walter Kob

Hydrogels have had a profound impact in the fields of tissue engineering, drug delivery, and materials science as a whole. Due to the network architecture of these materials, imbibement with water often results in uniform swelling and…

Colloidal gels have unique mechanical and transport properties that stem from their bicontinous nature, in which a colloidal network is intertwined with a viscous solvent, and have found numerous applications in foods, cosmetics,…

软凝聚态物质 · 物理学 2021-08-12 Hideyo Tsurusawa , Mathieu Leocmach , John Russo , Hajime Tanaka

Attractive colloidal dispersions, suspensions of fine particles which aggregate and frequently form a space spanning elastic gel are ubiquitous materials in society with a wide range of applications. The colloidal networks in these…

流体动力学 · 物理学 2018-11-14 Zsigmond Varga , Jennifer L. Hofmann , James W. Swan

Motivated by recent experiments studying the creep and breakup of a protein gel under stress, we introduce a simple mesoscopic model for the irreversible failure of gels and fibrous materials, and demonstrate it to capture much of the…

软凝聚态物质 · 物理学 2024-02-16 Henry A. Lockwood , Molly H. Agar , Suzanne M. Fielding

Repeated loading of a solid leads to microstructural damage that ultimately results in catastrophic material failure. While posing a major threat to the stability of virtually all materials, the microscopic origins of fatigue, especially…

软凝聚态物质 · 物理学 2018-05-23 Jan Maarten van Doorn , Joanne E. Verweij , Joris Sprakel , Jasper van der Gucht

Attractive colloidal particles can form a disordered elastic solid or gel when quenched into a two-phase region, if the volume fraction is sufficiently large. When the interactions are comparable to thermal energies the stress-bearing…

软凝聚态物质 · 物理学 2014-03-13 Lisa J. Teece , James M. Hart , Kerry Yen Ni Hsu , Stephen Gilligan , Malcolm A. Faers , Paul Bartlett

We study creep flow and yielding of particulate depletion gels under constant shear stress, combining data on different length and time scales. We characterise the breakage of meso-scale strands in the gel. Breakage events are distributed…

软凝聚态物质 · 物理学 2024-08-14 Himangsu Bhaumik , Tanniemola B. Liverpool , C. Patrick Royall , Robert L. Jack

We predict a phenomenon of catastrophic material failure arising suddenly within an amorphous material, with an extremely long delay time since the material was last deformed. By simulating a mesoscopic soft glassy rheology model in one…

软凝聚态物质 · 物理学 2025-07-15 Henry A. Lockwood , Emily S. Carrington , Suzanne M. Fielding

Colloidal gels consist of percolating networks of interconnected arms. Their mechanical properties depend on the individual arms, and on their collective behaviour. We use numerical simulations to pull on a single arm, built from a model…

软凝聚态物质 · 物理学 2023-01-31 Kristian Thijssen , T. B. Liverpool , C. Patrick Royall , Robert L. Jack

We investigate the delayed rupture of biopolymer gels under a constant shear load by simultaneous dynamic light scattering and rheology measurements. We unveil the crucial role of normal stresses built up during gelation: all samples that…

软凝聚态物质 · 物理学 2021-01-05 Angelo Pommella , Luca Cipelletti , Laurence Ramos

Colloidal gels are formed through the aggregation of attractive particles, whose size ranges from 10~nm to a few micrometers, suspended in a liquid. Such gels are ubiquitous in everyday life applications, from food products to paints or…

软凝聚态物质 · 物理学 2020-11-16 Thomas Gibaud , Thibaut Divoux , Sébastien Manneville

We deform, in pure shear, a thin sample of Cu$_{50}$Zr$_{50}$ metallic glass using a molecular dynamics simulation up to, and including, failure. The experiment is repeated ten times in order to have average values and standard deviations.…

材料科学 · 物理学 2020-02-19 Matias Sepulveda-Macias , Gonzalo Gutierrez , Fernando Lund

Metastable gels formed by weakly attractive colloidal particles display a distinctive two-stage time-dependent settling behavior under their own weight. Initially a space-spanning network is formed that for a characteristic time, which we…

软凝聚态物质 · 物理学 2015-05-30 Paul Bartlett , Lisa J. Teece , Malcolm A. Faers

The elastic coupling between plastic events is generally invoked to interpret plastic properties and failure of amorphous soft glassy materials. We report an experiment where the emergence of a self-organized plastic flow is observed well…

软凝聚态物质 · 物理学 2014-05-21 Le Bouil Antoine , Amon Axelle , McNamara Sean , Crassous Jérôme

We present experiments and simulations on cyclically sheared colloidal gels, and probe their behaviour on several different length scales. The shearing induces structural changes in the experimental gel, changing particles' neighborhoods…

The competition of depletion attractions and longer-ranged repulsions between colloidal particles in colloid-polymer mixtures leads to the formation of heterogeneous gel-like structures. For instance, gel networks, i.e., states where the…

软凝聚态物质 · 物理学 2021-06-24 Matthias Gimperlein , Michael Schmiedeberg

We present an experimental study of the deformation inside a granular material that is progressively tilted. We investigate the deformation before the avalanche with a spatially resolved Diffusive Wave Spectroscopy setup. At the beginning…

软凝聚态物质 · 物理学 2015-06-12 Axelle Amon , Roman Bertoni , Jérôme Crassous
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