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Adsorption of small amphiphilic molecules occurs in various biological and technological processes, sometimes desired, the other times unwanted (e.g., contamination). Surface-active molecules preferentially bind to interfaces and affect…

软凝聚态物质 · 物理学 2022-11-24 Fabio Staniscia , Horacio V. Guzman , Matej Kanduč

We show that an electro-osmotic flow near the slippery hydrophobic surface depends strongly on the mobility of surface charges, which are balanced by counter-ions of the electrostatic diffuse layer. For a hydrophobic surface with immobile…

流体动力学 · 物理学 2015-04-03 S. R. Maduar , A. V. Belyaev , V. Lobaskin , O. I. Vinogradova

A binary mixture of oppositely charged components confined to a plane such as cationic and anionic lipid bilayers may exhibit local segregation. The relative strength of the net short range interactions, which favors macroscopic…

软凝聚态物质 · 物理学 2009-11-11 Sharon M. Loverde , Yury S. Velichko , Monica Olvera de la Cruz

Many key industrial processes, from electricity production, conversion and storage to electrocatalysis or electrochemistry in general, rely on physical mechanisms occurring at the interface between a metallic electrode and an electrolyte…

计算物理 · 物理学 2021-09-03 Laura Scalfi , Mathieu Salanne , Benjamin Rotenberg

The surface tension of monolayers with mixtures of anionic and nonionic surfactant at the liquid/vapour interface is studied. Previous works have observed that calculations of the surface tension of simple fluids show artificial…

Over the past few decades the experimental literature has consistently reported observations of attraction between like-charged colloidal particles and macromolecules in solution. Examples include nucleic acids and colloidal particles in…

软凝聚态物质 · 物理学 2020-04-22 Alzbeta Kubincova , Philippe H. Hunenberger , Madhavi Krishnan

We construct a mean-field formulation of the thermodynamics of ion solvation in immiscible polar binary mixtures. Assuming an equilibrium planar interface separating two semi-infinite regions of different constant dielectric medium, we…

软凝聚态物质 · 物理学 2007-10-03 William Kung , Francisco J. Solis , Monica Olvera de la Cruz

Understanding the response of the surface of metallic solids to external electric field sources is crucial to characterize electrode-electrolyte interfaces. Continuum electrostatics offer a simple description of the induced charge density…

化学物理 · 物理学 2021-12-14 Giovanni Pireddu , Laura Scalfi , Benjamin Rotenberg

The closed integral equations for the interfacial tension as a function of external polarization at the liquid metal - ionic melt interface are derived. The version of Popel'-Pavlov isotherm is applied to the analysis of electrocapillary…

化学物理 · 物理学 2007-05-23 Oleg A. Kobelev , Alexandr V. Kobelev

We consider the atomistic origin and the main mechanisms determining the energy of a liquid interface after relaxation. A simple theory is constructed for the monatomic densely packed liquids that allows calculation of the surface tension…

统计力学 · 物理学 2025-08-11 Dmitry M. Naplekov , Vladimir V. Yanovsky

Nonequilibrium interfacial thermodynamics is formulated in the presence of surface reactions for the study of diffusiophoresis in isothermal systems. As a consequence of microreversibility and Onsager-Casimir reciprocal relations,…

化学物理 · 物理学 2018-12-24 Pierre Gaspard , Raymond Kapral

Surface sensitive synchrotron-X-ray scattering studies reveal the distributions of monovalent ions next to highly charged interfaces. A lipid phosphate (dihexadecyl hydrogen-phosphate) was spread as a monolayer at the air-water interface,…

软凝聚态物质 · 物理学 2009-11-11 Wei Bu , David Vaknin , Alex Travesset

In the presence of surfactants, the interfacial tension (IFT) of microscopic droplets differs significantly from IFT of macroscopic drops for the same surfactant solutions. As a result, IFT between two immiscible liquids can strongly depend…

软凝聚态物质 · 物理学 2007-05-23 J. Tothova , M. Richterova , V. Lisy

Surface tension plays a ubiquitous role in phase transitions including condensation or evaporation of atmospheric liquid droplets. Especially, understanding of interfacial thermodynamics of the critical nucleus of 1 nm scale is important…

软凝聚态物质 · 物理学 2020-04-28 QHwan Kim , Wonho Jhe

Strongly interacting electrons in clean two-dimensional devices are theorized to exhibit many distinct transport regimes, such as ballistic, hydrodynamic, or diffusive. Realistic samples often lie in crossover regimes between these…

介观与纳米尺度物理 · 物理学 2026-05-14 Jack H. Farrell , Andrew Lucas

Surface sensitive synchrotron x-ray scattering studies were performed to obtain the distribution of monovalent ions next to a highly charged interface. A lipid phosphate (dihexadecyl hydrogen-phosphate) was spread as a monolayer at the…

软凝聚态物质 · 物理学 2007-05-23 Wei Bu , David Vaknin , Alex Travesset

The interface of a cholesteric liquid crystal with an isotropic fluid can display a range of unusual properties, such as a layer of topological defects close to an undulated interface. These properties have been know for a long time and…

软凝聚态物质 · 物理学 2014-07-02 N. R. Bernardino , M. C. F. Pereira , N. M. Silvestre , M. M. Telo da Gama

The origin of the apparent negative charge at hydrophobic-water interfaces has fueled one of the biggest debates in physical chemistry for several decades. The most common interpretation given to explain this observation is that negatively…

化学物理 · 物理学 2020-03-25 Emiliano Poli , Kwang H. Jong , Ali Hassanali

We present an overview of our understanding of electrostatic interactions between charged macromolecular surfaces mediated by mobile counter- and coions. The dichotomy between the weak and the strong coupling regimes is described in detail…

软凝聚态物质 · 物理学 2016-12-21 Ali Naji , Matej Kanduc , Roland R. Netz , Rudolf Podgornik

Osmotic transport in nanoconfined aqueous electrolytes provides new venues for water desalination and "blue energy" harvesting; the osmotic response of nanofluidic systems is controlled by the interfacial structure of water and electrolyte…

化学物理 · 物理学 2022-08-16 Laurent Joly , Robert H. Meißner , Marcella Iannuzzi , Gabriele Tocci