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We demonstrate spectroscopy and thermometry of individual motional modes in a mesoscopic 2D ion array using entanglement-induced decoherence as a method of transduction. Our system is a $\sim$400 $\mu$m-diameter planar crystal of several…

We present static and dynamical properties of linear vortices in 4He droplets obtained from Density Functional calculations. By comparing the adsorption properties of different atomic impurities embedded in pure droplets and in droplets…

软凝聚态物质 · 物理学 2009-11-10 Francesco Ancilotto , Manuel Barranco , Marti Pi

Non-planar aromatic molecules are interesting systems for organic electronics and optoelectronics applications due to their high stability and electronic properties. By using scanning tunneling microscopy and spectroscopy, we investigated…

K$_3$-picene is a superconducting molecular crystal with critical temperature T$_c=7$K or 18K, depending on preparation conditions. Using density functional theory we show that electron-phonon interaction accounts for T$_c ~ 3-8$ K. The…

超导电性 · 物理学 2015-05-28 Michele Casula , Matteo Calandra , Gianni Profeta , Francesco Mauri

Tip-enhanced photoluminescence (TEPL) measurements are performed with sub-nanometer spatial resolution on individual molecules decoupled from a metallic substrate by a thin NaCl layer. TEPL spectra reveal progressive fluorescence quenching…

介观与纳米尺度物理 · 物理学 2024-03-18 Katharina Kaiser , Michelangelo Romeo , Fabrice Scheurer , Guillaume Schull , Anna Rosławska

Experimental and theoretical studies are presented on the reactivity of methanimine and aminomethylene cations with ethene. Selective isomer generation is performed via dissociative photoionization of suitable neutral precursors and…

Graphene has vast promising applications on the nanoelectronics and spintronics because of its unique magnetic and electronic properties. Making use of an ab initio spin-polarized density functional theory, implemented by the method of…

材料科学 · 物理学 2016-11-26 Zongguo Wang , Shaojing Qin , Chuilin Wang

A theoretical study is made on He scattering from three fundamental classes of disordered ad-layers: (a) Translationally random adsorbates, (b) disordered compact islands and (c) fractal submonolayers. The implications of the results to…

We theoretically demonstrate the ability of electron beams to probe the nonlinear photonic response with nanometer spatial resolution, well beyond the capabilities of existing optical techniques. Although the interaction of electron beams…

介观与纳米尺度物理 · 物理学 2020-12-30 Andrea Konečná , Valerio Di Giulio , Vahagn Mkhitaryan , Claus Ropers , F. Javier García de Abajo

Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

化学物理 · 物理学 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

$ $An experiment has been carried out for studying the cluster structure of $^9$Be induced by the $^3$He ions at the energy of 30 MeV. As results of the nuclear reaction $^3$He + $^9$Be the differential cross sections for the exit channels…

Rotationally resolved infrared spectra are reported for the X-HCN (X = Cl, Br, I) binary complexes solvated in helium nanodroplets. These results are directly compared with that obtained previously for the corresponding X-HF complexes [J.…

原子与分子团簇 · 物理学 2016-07-06 Jeremy M. Merritt , Jochen Küpper , Roger E. Miller

Magnesium atoms embedded in superfluid helium nanodroplets have been identified to arrange themselves in a metastable network, refered to as foam. In order to investigate the ionization dynamics of this unique structure with respect to a…

原子与分子团簇 · 物理学 2015-06-12 S. Göde , R. Irsig , J. Tiggesbäumker , K. -H. Meiwes-Broer

Chemical processes on the surface of icy grains play an important role in the chemical evolution in molecular clouds. In particular, reactions involving non-energetic hydrogen atoms accreted from the gaseous phase have been extensively…

星系天体物理 · 物理学 2022-07-20 Masashi Tsuge , Akira Kouchi , Naoki Watanabe

Benzene, with its sea of delocalized $\pi$-electrons in the valence orbitals, is identified as an example of a class of molecules that enable establishment of the correspondence between intense ion-induced and laser-light-induced fields in…

原子物理 · 物理学 2009-11-06 D. Mathur

Graphene hosts a unique electron system in which electron-phonon scattering is extremely weak but electron-electron collisions are sufficiently frequent to provide local equilibrium above liquid nitrogen temperature. Under these conditions,…

We calculate the photoionization cross-section of a molecular endohedral. We limit ourselves to two-atomic molecules. The consideration is much more complex than for atomic endohedrals because the system even for almost spherical fullerenes…

原子与分子团簇 · 物理学 2019-09-04 M. Ya. Amusia , L. V. Chernysheva , S. K. Semenov

We investigate here the fast electron scattering upon endohedral atoms that present a fullerene CN staffed by an atom A, A@CN. We calculate the inelastic scattering cross-section expressing it via generalized oscillator strengths (GOS)…

原子与分子团簇 · 物理学 2012-03-06 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We perform laser spectroscopy at liquid helium temperatures (T=2 K) to investigate single dibenzoterrylene (DBT) molecules doped in anthracene crystals of nanoscopic height fabricated by electrohydrodynamic dripping. Using high-resolution…

We study the potential of graphene plasmons for spectrometer-free sensing based on surface-enhanced infrared absorption and Raman scattering. The large electrical tunability of these excitations enables an accurate identification of…

介观与纳米尺度物理 · 物理学 2018-06-08 Andrea Marini , Iván Silveiro , F. Javier García de Abajo
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