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The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman…

光学 · 物理学 2010-08-27 V. P. Yashchuk , E. A. Tikhonov , O. A. Prygodiuk

Surface lattice resonance (SLR) lasers, where gain is supplied by a thin film active material and the feedback comes from multiple scattering by plasmonic nanoparticles, have shown both low threshold lasing and tunability of the angular and…

We revisit laser intensity noise in the context of stimulated Raman scattering (SRS), which has recently proved to be a key technique to provide label free images of chemical bonds in biological and medical samples. Contrary to most…

仪器与探测器 · 物理学 2019-10-29 Xavier Audier , Sandro Heuke , Peter Volz , Ingo Rimke , Hervé Rigneault

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

光学 · 物理学 2020-08-26 Andre Kovach , Arynn Gallegos , Jinghan He , Hyungwoo Choi , Andrea M. Armani

The range of stimulated Raman scattering (SRS) frequencies covers a domain which at the low end abuts half the laser frequency, omega_0 / 2, according to the simplest SRS theories, corresponding to scatter from electron densities near 1/4…

等离子体物理 · 物理学 2015-05-20 Harvey A. Rose , Philippe Mounaix

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

Raman spectroscopy is an appealing technique that probes molecular vibrations in a wide variety of materials with virtually no sample preparation. However, accurate and reliable Raman measurements are still a challenge and require more…

光学 · 物理学 2020-02-14 Hugo Kerdoncuff , Mikael Lassen , Jan C. Petersen

Raman scattering experiments from silver nanocrystals embedded in films of amorphous silica are reported. In addition to the low-frequency peak due to vibrational quadrupolar modes, a broadband is observed in the high-frequency range, with…

凝聚态物理 · 物理学 2007-05-23 H. Portales , E. Duval , L. Saviot , M. Fujii , M. Sumitomo , S. Hayashi

Stimulated globular scattering (SGS) characteristics (frequency shifts, threshold, conversion efficiency) have been studied in photonic crystals (synthetic opal matrices and opal nanocomposites) at different temperatures. Results have been…

光学 · 物理学 2007-09-18 V. S. Gorelik , A. D. Kudryavtseva , N. V. Tcherniega , A. I. Vodchits

In stimulated Raman scattering, two incident optical waves induce a force oscillating at the difference of the two light frequencies. This process has enabled important applications such as the excitation and coherent control of phonons and…

材料科学 · 物理学 2017-09-27 Sebastian Maehrlein , Alexander Paarmann , Martin Wolf , Tobias Kampfrath

In this study, we combined the surface-enhanced Raman scattering (SERS) with density functional theory (DFT) calculations to investigate the SERS spectra of lanthanide (Ln)-citrate complexes (Ln = La, Ce, Pr, Nd, Sm, Eu, and Gd) under 488,…

化学物理 · 物理学 2025-03-25 Hao Jin , Tamitake Itoh , Yuko S. Yamamoto

Lead sulfide is an important semiconductor that has found technological applications for over a century. Raman spectroscopy, a standard tool for the investigation and characterization of semiconductors, has limited application to this…

材料科学 · 物理学 2015-05-13 P. G. Etchegoin , M. Cardona , R. Lauck , R. J. H. Clark , J. Serrano , A. H. Romero

As shown in the early 1960s, the gain in stimulated Raman scattering (SRS) is drastically suppressed when the rate of creation of phonons (via pump-to-Stokes conversion) is exactly balanced by the rate of phonon annihilation (via…

A coherent microwave radiation, concomitant with experiments of stimulated Raman scattering (SRS) in weakly compressed hydrogen, had been observed; qualitative and quantitative results had been obtained, and are given in this article. .An…

光学 · 物理学 2007-05-23 Boris Oksengorn

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

量子物理 · 物理学 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

We report multiphonon Raman scattering in graphene samples. Higher order combination modes involving 3 phonons and 4 phonons are observed in single-layer (SLG), bi-layer (BLG), and few layer (FLG) graphene samples prepared by mechanical…

介观与纳米尺度物理 · 物理学 2015-05-30 Rahul Rao , Derek Tishler , Jyoti Katoch , Masa Ishigami

Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…

The recently discovered layered BiS2-based superconductors have attracted a great deal of interest due to their structural similarity to cuprate and iron-pnictide superconductors. We have performed Raman scattering measurements on two…

The symmetry group analysis is applied to classify the phonon modes of $N$-stacked graphene layers (NSGL's) with AB- and AA-stacking, particularly their infra-red and Raman properties. The dispersions of various phonon modes are calculated…

材料科学 · 物理学 2008-06-30 Jin-Wu Jiang , Hui Tang , Bing-Shen Wang , Zhao-Bin Su

Surface enhanced Raman scattering (SERS) effects on tin dioxide in the form of bulk material, nanostructured thin films and colloidal solutions were investigated. Raman spectra are characterized by the three Raman scattering peaks at 478,…

材料科学 · 物理学 2015-06-03 Enza Fazio , Fortunato Neri , Salvatore Savasta , Salvatore Spadaro , Sebastiano Trusso