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X-ray reflectivity (XRR) measurements of femtosecond laser-induced transient gratings are applied to demonstrate the spatio-temporal coherent control of thermally induced surface deformations on ultrafast timescales. Using gracing incidence…

We demonstrate full control of acoustic and thermal periodic deformations at solid surfaces down to sub-nanosecond time scales and few-micrometer length scales via independent variation of the temporal and spatial phase of two optical…

应用物理 · 物理学 2019-08-28 J. -E. Pudell , M. Sander , R. Bauer , M. Bargheer , M. Herzog , P. Gaal

Diffraction imaging of non-equilibrium dynamics at atomic resolution is becoming possible with X-ray free-electron lasers. However, there are unresolved problems with applying this method to objects that are confined in only one dimension.…

强关联电子 · 物理学 2018-02-19 Kenneth R. Beyerlein

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

The dynamics of thermal and non-thermal lattice deformation of nanometer thick polycrystalline aluminum film has been studied by means of femtosecond (fs) time-resolved electron diffraction. We utilized two different pump wavelengths: 800…

材料科学 · 物理学 2017-09-13 Runze Li , Pengfei Zhu , Jie Chen , Jianming Cao , Peter M. Rentzepis , Jie Zhang

Laser with high spectral purity plays a crucial role in high-precision optical metrology and coherent communication. Thanks to the rapid development of laser frequency stabilization, the laser phase noise can be remarkably compensated,…

仪器与探测器 · 物理学 2020-04-22 Liang Zhang , Liang Chen , Xiaoyi Bao

We have developed an improved method of time-resolved x-ray reflectivity (XRR) using monochromatic synchrotron radiation. Our method utilizes a polycapillary x-ray optic to create a range of incident angles and an area detector to collect…

材料科学 · 物理学 2019-03-27 Howie Joress , Shane Quinlan Arlington , Timothy P. Weihs , Joel D. Brock , Arthur Woll

Proposed, justified and tested measuring of beam spatial coherence, based on the detection of an interference visibility of the equal to intensity of beam replicas emerging under reflection from the rotated plane-parallel plate. The method…

光学 · 物理学 2015-10-20 E. A. Tikhonov , A. K. Lyamets

We present a unified elucidation for the role temporal coherence properties of x-rays in surface x-ray standing wave analysis, under total external reflection condition. Analytical formulas have been derived that provide a direct relation…

介观与纳米尺度物理 · 物理学 2014-06-16 M K Tiwari , Gangadhar Das

Coherent diffractive imaging is unique as the only route for achieving diffraction-limited spatial resolution in the extreme ultraviolet and X-ray regions, limited only by the wavelength of the light. Recently, advances in coherent short…

We present time-resolved X-ray diffraction measurements using advanced timing schemes that provide high temporal resolution while also maintaining a high flux in the X-ray probe beam. The method employs patterned probe pulse sequences that…

Pump-probe time-resolved x-ray diffraction of allowed and nearly forbidden reflections in InSb is used to follow the propagation of a coherent acoustic pulse generated by ultrafast laser-excitation. The surface and bulk components of the…

We discuss the potential creation and measurement of coherences in both dispersive solids and qubit-like single levels using current generation time- and angle-resolved photoemission technology. We show that in both cases, when both the…

介观与纳米尺度物理 · 物理学 2020-05-22 Alexander F. Kemper , Avinash Rustagi

X-ray diffraction is ideal for probing sub-surface state during complex or rapid thermomechanical loading of crystalline materials. However, challenges arise as the size of diffraction volumes increases due to spatial broadening and…

材料科学 · 物理学 2025-01-10 Rachel E. Lim , Shun-Li Shang , Chihpin Chuang , Thien Q. Phan , Zi-Kui Liu , Darren C. Pagan

The Fourier inversion of phased coherent diffraction patterns offers images without the resolution and depth-of-focus limitations of lens-based tomographic systems. We report on our recent experimental images inverted using recent…

A broadband detection method with coherent laser pulses exciting surface plasmons is investigated. The intensity and phase characteristics of the reflected light in Kretschmann configuration are calculated. It is shown that by mixing…

仪器与探测器 · 物理学 2018-11-14 Alexandre Kolomenskii , Elizabeth Surovic , Hans Schuessler

In coherent X-ray diffraction microscopy the diffraction pattern generated by a sample illuminated with coherent x-rays is recorded, and a computer algorithm recovers the unmeasured phases to synthesize an image. By avoiding the use of a…

The formation of permanent laser-induced periodic surface structures (LIPSS) on solid surfaces under impulsive laser irradiation above the damage threshold has been subject of extensive research. We demonstrate the formation of transient…

We describe an optical method to directly measure position-dependent thermal diffusivity of reflective single crystal samples across a broad range of temperatures for condensed matter physics research. Two laser beams are used, one as a…

The properties of artificially grown thin films are often strongly affected by the dynamic relationship between surface growth processes and subsurface structure. Coherent mixing of X-ray signals promises to provide an approach to better…

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