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We have detected a second-order nonlinear optical response from aggregates of the ampholytic megamolecular polysaccharide sacran extracted from cyanobacterial biomaterials, by using optical second harmonic generation (SHG) microscopy. The…

Second-harmonic generation (SHG) is a fundamental nonlinear optical process widely used in photonics; however, it is strictly forbidden in the bulk of centrosymmetric materials due to their inversion symmetry. Nevertheless, applying an…

光学 · 物理学 2025-07-15 Hangkai Fan , Alexey Proskurin , Mingzhao Song , Yuri Kivshar , Andrey Bogdanov

The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…

介观与纳米尺度物理 · 物理学 2015-06-17 Godfrey Gumbs , Yonatan Abranyos , Upali Aparajita , Oleksiy Roslyak

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

强关联电子 · 物理学 2021-03-17 G. van der Laan , S. W. Lovesey

We report on the optical second harmonic generation (SHG) on the 1S exciton-polariton resonance in bulk ZnSe that is subject to an external magnetic field applied perpendicular to the light wave vector $\mathbf k$ (Voigt geometry). For the…

介观与纳米尺度物理 · 物理学 2025-07-18 J. Mund , D. R. Yakovlev , A. Farenbruch , N. V. Siverin , M. A. Semina , M. M. Glazov , E. L. Ivchenko , M. Bayer

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

软凝聚态物质 · 物理学 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…

光学 · 物理学 2019-03-27 Raksha Singla , W. Luis Mochán

Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

光学 · 物理学 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

介观与纳米尺度物理 · 物理学 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

适应与自组织系统 · 物理学 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

凝聚态物理 · 物理学 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…

光学 · 物理学 2011-03-16 Alessandro Ciattoni

The demand for nonlinear effects within a silicon platform to support photonic circuits requiring phase-only modulation, frequency doubling, and/or difference frequency generation, is becoming increasingly clear. However, the symmetry of…

光学 · 物理学 2017-04-05 E. Timurdogan , Christopher V. Poulton , M. R. Watts

For centrosymmetric materials such as monolayer graphene, no optical second harmonic generation (SHG) is generally expected because it is forbidden under the electric-dipole approximation. Yet we observed a strong, doping induced SHG from…

介观与纳米尺度物理 · 物理学 2019-02-12 Yu Zhang , Di Huang , Yuwei Shan , Tao Jiang , Zhihong Zhang , Kaihui Liu , Lei Shi , Jinluo Cheng , John E. Sipe , Wei-Tao Liu , Shiwei Wu

Nonlinear optics of semiconductors is an important field of fundamental and applied research, but surprisingly the role of excitons in the coherent processes leading to harmonics generation has remained essentially unexplored. Here we…

介观与纳米尺度物理 · 物理学 2015-06-17 M. Lafrentz , D. Brunne , A. V. Rodina , V. V. Pavlov , R. V. Pisarev , D. R. Yakovlev , A. Bakin , M. Bayer

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

Optical second harmonic generation (SHG) is studied from multilayer graphene films in the presence of DC electric current flowing in the sample plane. Graphene layers are manufactured by chemical vapour deposition (CVD) technique and…

介观与纳米尺度物理 · 物理学 2015-06-04 Anton Y. Bykov , Tatiana V. Murzina , Maxim G. Rybin , Elena D. Obraztsova

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

原子物理 · 物理学 2025-03-31 Xinhua Xie
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