相关论文: Multipolar polarizabilities and hyperpolarizabilit…
We address the problem of lattice light shifts in the Sr clock caused by multipolar M1 and E2 atom-field interactions. We presented a simple but accurate formula for the magnetic-dipole polarizability that takes into account both the…
In neutral atom optical clocks, the higher-order atomic polarizability terms lead to the clock transition frequency shift which is motion-state dependent and nonlinear with the optical lattice depth. We propose to use an auxiliary optical…
The progress in optical clock with uncertainty at a level of $10^{-18}$ requires unprecedented precision in estimating the contribution of multipolar and higher-order effects of atom-field interactions. Current theoretical and experimental…
We experimentally investigate the lattice-induced light shift by the electric-quadrupole ($E2$) and magnetic-dipole ($M1$) polarizabilities and the hyperpolarizability in Sr optical lattice clocks. Precise control of the axial as well as…
The hyperpolarizability of an atom is a property that describes the nonlinear interaction between an atom and an external electric field leading to a higher-order Stark shift. Accurate evaluations of these coefficients for various systems…
We report the observation of the higher order frequency shift due to the trapping field in a $^{87}$Sr optical lattice clock. We show that at the magic wavelength of the lattice, where the first order term cancels, the higher order shift…
With the improvement of high-precision optical clock, the higher-order multipolar interaction between atoms and light needs quantitative evaluation. However for the Sr clock, the differential dynamic E2-M1 polarizability at the magic…
A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. We present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an…
Progress in atomic optical clocks with total uncertainty of $10^{-18}$ or below requires a precise estimation of multipolar and higher-order effects due to atom-field interactions. Magnesium is an attractive candidate for optical lattice…
To operate an optical lattice clock at a fractional uncertainty below $10^{-17}$, one must typically consider not only electric-dipole (E1) interaction between an atom and the lattice light field when characterizing the resulting lattice…
Molecular lattice clocks enable the search for new physics, such as fifth forces or temporal variations of fundamental constants, in a manner complementary to atomic clocks. Blackbody radiation (BBR) is a major contributor to the systematic…
The energy levels and electric dipole ($E1$) matrix elements of the ground state and low-lying excited states of Be atoms are calculated using the relativistic configuration interaction plus core polarization (RCICP) method. The static and…
Recent progress in optical lattice clocks requires unprecedented precision in controlling systematic uncertainties at $10^{-18}$ level. Tuning of nonlinear light shifts is shown to reduce lattice-induced clock shift for wide range of…
Despite being a canonical example of quantum mechanical perturbation theory, as well as one of the earliest observed spectroscopic shifts, the Stark effect contributes the largest source of uncertainty in a modern optical atomic clock…
In state-of-the-art optical lattice clocks, beyond-electric-dipole polarizability terms lead to a break-down of magic wavelength trapping. In this Letter, we report a novel approach to evaluate lattice light shifts, specifically addressing…
The light-induced frequency shift due to the hyperpolarizability (i.e. terms of second-order in intensity) is studied for a forbidden optical transition, $J$=0$\to$$J$=0. A simple universal dependence on the field ellipticity is obtained.…
We present a detailed experimental and theoretical study of the effect of nuclear spin on the performance of optical lattice clocks. With a state-mixing theory including spin-orbit and hyperfine interactions, we describe the origin of the…
We evaluated the static and dynamic polarizabilities of the 5s^2 ^1S_0 and 5s5p ^3P_0^o states of Sr using the high-precision relativistic configuration interaction + all-order method. Our calculation explains the discrepancy between the…
We present a comprehensive study of the frequency shifts associated with the lattice potential for a Sr lattice clock. By comparing two such clocks with a frequency stability reaching $5\times 10^{-17}$ after a one hour integration time,…
The theoretical calculations of the dynamic E2-M1 polarizability at the magic wavelength of the Sr optical clock are inconsistent with experimental results. We investigate role of negative-energy states in the E2 and M1 polarizabilities.…