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An influence of multi-line CO laser focusing on spectral characteristics of broadband sum-frequency generation in ZnGeP2 nonlinear crystal was experimentally and numerically studied. Maximal frequency conversion was experimentally observed…

Comparative study of nonlinear crystals for picosecond difference frequency generation in mid-IR is presented. Nonlinear crystals of AgGaS$_2$, BaGa$_4$Se$_7$, LiGaSe$_2$, and LiGaS$_2$ were studied. Samples of AgGaS$_2$, BaGa$_4$Se$_7$,…

We report on extensive experimental investigation of novel barium chalcogenides (BaGa4Se7, BaGa2GeSe6 and BaGa2GeS6) for generation of a strong narrowband terahertz (THz) radiation. The Ba-containing compounds demonstrate the large bandgap…

光学 · 物理学 2026-03-03 D. Z. Suleimanova , E. A. Migal , D. V. Badikov , F. V. Potemkin

Infrared laser systems are vital for applications in spectroscopy, communications, and biomedical devices, where infrared nonlinear optical (NLO) crystals are required for broadband frequency down-conversion. Such crystals need to have high…

High-power infrared laser systems with broadband tunability are of great importance due to their wide range of applications in spectroscopy and free-space communications. These systems require nonlinear optical (NLO) crystals for wavelength…

Proposed is a new laser material for the making of active elements of tunable lasers for mid IR region (4-5 mkm) - Zn1-xMgxSe (0.11<x<0.42) single crystals doped with Fe2+ ions. The optical transmission spectra of Fe2+:Zn0.89Mg0.11Se and…

材料科学 · 物理学 2010-12-03 Yu. A. Zagoruiko , N. O. Kovalenko , O. A. Fedorenko , A. S. Gerasimenko

Since de discovery of graphene, the family of 2-dimensional materials has attracted much recent attention. In this work, the nonlinear optical properties of few-layer MoS2 two-dimensional crystals are studied using femtosecond laser pulses.…

介观与纳米尺度物理 · 物理学 2013-06-20 Leandro M. Malard , Thonimar V. Alencar , Ana Paula M. Barboza , Kin Fai Mak , Ana M. de Paula

BGGSe is a newly developed nonlinear material that is attractive for ultrabroad frequency mixing and ultrashort pulse generation due to its comparably low dispersion and high damage threshold.In a first experiment, we show that a long…

We demonstrate enhanced second harmonic generation in a gallium phosphide photonic crystal waveguide with a measured external conversion efficiency of 5$\times10^{-7}$/W. Our results are promising for frequency conversion of on-chip…

光学 · 物理学 2015-05-28 Kelley Rivoire , Sonia Buckley , Fariba Hatami , Jelena Vuckovic

The Z-scan measurements for the non-centrosymmetric optical crystals {\beta}-BaTeMo2O9 (BTMO) were performed. The corresponding experiments were carried out using the 5 ns pulses of the second harmonic of a nanosecond Nd:YAG laser at the…

We report optical second-harmonic generation (SHG) in reflection from GaSe crystals of 1 to more than 100 layers using a fundamental picosecond pulsed pump at 1.58 eV and a supercontinuum white light pulsed laser with energies ranging from…

介观与纳米尺度物理 · 物理学 2017-10-10 Yanhao Tang , Krishna C. Mandal , John A. McGuire , Chih Wei Lai

We report on the fabrication of what we believe is the first example of a two dimensional nonlinear periodic crystal\cite{berger}, where the refractive index is constant but in which the 2nd order nonlinear susceptibility is spatially…

Nonlinear frequency conversion provides essential tools for light generation, photon entanglement, and manipulation. Transition metal dichalcogenides (TMDs) possess huge nonlinear susceptibilities and 3R-stacked TMD crystals further combine…

The resonant nonlinear refraction of 4-5 $\mu$m light in CO and CO$_2$ gas at a peak intensity of 15 MW/cm$^2$ was demonstrated using time- and frequency-resolved measurements of self-focusing and self-defocusing. The nonlinearity of these…

We demonstrate the post-induction of high-quality microcavity on silicon photonic crystal (PC) waveguide by integrating few-layer GaSe crystal, which promises highly efficient on-chip optical frequency conversions. The integration of GaSe…

We report on frequency tripling of high energy, high repetition rate ns pulses from a cryogenically gas cooled multi-slab Yb:YAG laser system Bivoj/DiPOLE, using a type-I phase matched LBO crystal for second harmonic generation and type-II…

The 4-bar crystal symmetry in materials such as GaAs can enable quasi-phasematching for efficient frequency conversion without poling, twinning or other engineered domain inversions. 4-bar symmetry means that a 90 degree rotation is…

介观与纳米尺度物理 · 物理学 2012-10-09 Paulina S. Kuo , Glenn S. Solomon

We present a systematic experimental comparison of single-pass second-harmonic generation (SHG) in bismuth triborate (BiBO) and lithium triborate (LBO) nonlinear crystals, driven by a 1.3 ps, 91 kHz laser at 1030 nm with up to 57 W of…

The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a…

光学 · 物理学 2017-04-05 Henning Kurzke , Jan Kiethe , Axel Heuer , Andreas Jechow

We present a study of second harmonic generation (SHG) and third harmonic generation (THG) in lithium triborate (LBO) crystals using a high-energy, 10-J-class, 10 Hz Yb:YAG laser system. We achieved high conversion efficiencies of 75% for…

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