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Buildings are responsible for a considerable fraction of the energy wasted globally every year, and as a result, excess carbon emissions. While heat is lost directly in colder months and climates, resulting in increased heating loads, in…

The bottleneck in modern thermoelectric power generation and cooling is the low energy conversion efficiency of thermoelectric materials. The detrimental effects of lattice phonons on performance can be mitigated, but achieving a high…

Cross-plane superlattices composed of nanoscale layers of alternating potential wells and barriers have attracted great attention for their potential to provide thermoelectric power factor improvements and higher ZT figure of merit.…

材料科学 · 物理学 2015-12-16 Mischa Thesberg , Mahdi Pourfath , Hans Kosina , Neophytos Neophytou

Bipolar carrier transport is often a limiting factor in the thermoelectric efficiency of narrow bandgap materials (such as Bi2Te3 and PbTe) at high temperatures due to the introduction of an additional term to the thermal conductivity and a…

材料科学 · 物理学 2019-04-12 Samuel Foster , Neophytos Neophytou

We investigate the low-temperature electrical and thermal transport properties in atomically precise metallic heterostructures involving strongly-correlated electron systems. The model of the Mott-insulator/ band-insulator superlattice was…

强关联电子 · 物理学 2008-06-19 Andreas Ruegg , Sebastian Pilgram , Manfred Sigrist

We study the thermoelectric effect of two-dimensional metals on a square lattice within semiclassical Boltzmann transport theory with particular focus on electron-electron scattering. We compute the electrical conductivity and the Seebeck…

强关联电子 · 物理学 2013-09-17 Jonathan M. Buhmann , Manfred Sigrist

Thermoelectric materials intrigue much interest due to their wide range of application such as power generators and refrigerators. The efficiency of thermoelectric materials is quantified by the figure of merit, and a figure greater than…

介观与纳米尺度物理 · 物理学 2022-02-16 Masashi Hosoi , Ikuma Tateishi , Hiroyasu Matsuura , Masao Ogata

We performed Boltzmann transport calculation to obtain the Seebeck coefficient, electrical conductivity, electronic thermal conductivity, and thermoelectric figure of merit (ZT) for Dirac systems. We found an enhancement of ZT due to the…

介观与纳米尺度物理 · 物理学 2018-10-04 Eddwi H. Hasdeo , Lukas P. A. Krisna , Ahmad R. T. Nugraha

The Seebeck coefficient and electrical conductivity are two critical quantities to optimize simultaneously in designing thermoelectric materials, and they are determined by the dynamics of carrier scattering. We uncover a new regime where…

材料科学 · 物理学 2022-11-17 Natalya S. Fedorova , Andrea Cepellotti , Boris Kozinsky

With the goal of maximizing the thermoelectric (TE) figure of merit $ZT$, Mahan and Sofo [Proc. Natl. Acad. Sci. U.S.A. 93, 7436 (1996)] found that the optimal transport distribution (TD) is a delta function. Materials, however, have TDs…

材料科学 · 物理学 2022-09-13 Jesse Maassen

Thermoelectric materials can be used to construct devices which recycle waste heat into electricity. However, the best known thermoelectrics are based on rare, expensive or even toxic elements, which limits their widespread adoption. To…

材料科学 · 物理学 2022-12-14 Luis M. Antunes , Keith T. Butler , Ricardo Grau-Crespo

Thermoelectric (TE) materials are useful for applications such as waste heat harvesting or efficient and targeted cooling. While various strategies towards superior thermoelectrics through a reduction of the lattice thermal conductivity…

In this Letter, we show thermoelectric conversion efficiency is \emph{exactly} determined by \emph{three} independent material parameters $Z_{\rm gen}$, $\tau$, and $\beta$. Each parameter is a figure of merit hence improving $\tau$ or…

材料科学 · 物理学 2019-10-25 Byungki Ryu , Jaywan Chung , SuDong Park

Thermoelectric devices that utilize the Seebeck effect convert heat flow into electrical energy and are highly desirable for the development of portable, solid state, passively-powered electronic systems. The conversion efficiencies of such…

材料科学 · 物理学 2015-01-06 Ruixiang Fei , Alireza Faghaninia , Ryan Soklaski , Jia-An Yan , Cynthia Lo , Li Yang

Recent discovery of new materials for thermoelectric energy conversion is enabled by efficient prediction of materials' performance from first-principles, without empirically fitted parameters. The novel simplified approach for computing…

材料科学 · 物理学 2018-05-02 Georgy Samsonidze , Boris Kozinsky

We propose a model describing Seebeck effect on a weak link between two quantum systems with fine-tunable ground states of Fermi and Non-Fermi liquid origin. The experimental realization of the model can be achieved by utilizing the quantum…

介观与纳米尺度物理 · 物理学 2018-02-06 T. K. T. Nguyen , M. N. Kiselev

Using the tools of random matrix theory we develop a statistical analysis of the transport properties of thermoelectric low-dimensional systems made of two electron reservoirs set at different temperatures and chemical potentials, and…

介观与纳米尺度物理 · 物理学 2016-08-23 Adel Abbout , Henni Ouerdane , Christophe Goupil

Following demands for materials with peculiar transport properties, e.g. in magnetoelectronics or thermoelectrics, there is a need for materials modeling at the quantum-mechanical level. We combine density-functional with various…

材料科学 · 物理学 2010-11-02 Peter Kratzer , Vladimir M. Fomin , B. Hülsen , M. Scheffler

In order to improve the thermoelectric performance of TiCoSb we have substituted 50% of Ti equally with Zr and Hf at Ti site and Sb with Sn and Se equally at Sb site. The electronic structure of Ti0.5Zr0.25Hf0.25CoSn0.5Se0.5 is investigated…

材料科学 · 物理学 2018-05-09 Mukesh K. Choudhary , P Ravindran

In the work, a modified effective medium theory is constructed for calculating the effective properties of thermoelectric composites with different values of percolation thresholds. It is shown that even at concentrations beyond the…

材料科学 · 物理学 2020-06-23 Snarskii Andrei , Yuskevich Pavel