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Strong coupling between light and matter in an optical cavity provides a pathway to giant polariton nonlinearity, where effective polariton-polariton interactions are mediated by materials' nonlinear responses. The pursuit of such enhanced…

光学 · 物理学 2024-11-26 Zhi Wang , Li He , Bumho Kim , Bo Zhen

We theoretically designed and experimentally demonstrated a mechanism to protect a spatially segregated mixed light-matter state, known as intercavity exciton-polariton in strongly coupled optical cavities. This excitation, shared across…

This thesis studies light-matter interactions in strong and weak coupling regimes. In the first part, we study the formation and propagation of exciton-polariton condensates in different microcavities in the strong coupling regime.…

介观与纳米尺度物理 · 物理学 2024-01-19 Dogyun Ko

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

Enhancement and active control of light-matter interactions at the atomic scale is important for developing next-generation nanophotonic and quantum optical devices. Here, we demonstrate electric control of both excitonic strong coupling…

Simultaneous photoluminescence and photocurrent measurements on individual single-walled carbon nanotubes reveal spontaneous dissociation of excitons into free electron-hole pairs. Correlation of luminescence intensity and photocurrent…

介观与纳米尺度物理 · 物理学 2014-03-19 Y. Kumamoto , M. Yoshida , A. Ishii , A. Yokoyama , T. Shimada , Y. K. Kato

Light emission from carbon nanotubes is expected to be dominated by excitonic recombination. Here we calculate the properties of excitons in nanotubes embedded in a dielectric, for a wide range of tube radii and dielectric environments. We…

材料科学 · 物理学 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

Polariton emission from optical cavities integrated with various luminophores has been extensively studied recently due to the wide variety of possible applications in photonics, particularly promising in terms of fabrication of…

介观与纳米尺度物理 · 物理学 2021-07-28 Dmitriy Dovzhenko , Maksim Lednev , Konstantin Mochalov , Ivan Vaskan , Pavel Samokhvalov , Yury Rakovich , Igor Nabiev

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

介观与纳米尺度物理 · 物理学 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

We present a comprehensive investigation of the light-matter interaction dynamics in two-dimensional materials coupled with a spectrally isolated cavity mode in the strong coupling regime. The interaction between light and matter breaks the…

介观与纳米尺度物理 · 物理学 2023-12-18 Maria Vittoria Gurrieri , Emil V. Denning , Kristian Seegert , Philip T. Kristensen , Jesper Mørk

Strong exciton-plasmon interaction between the layered two-dimensional (2D) semiconductors and gap plasmons shows a great potential to implement cavity quantum-electrodynamics in ambient condition. However, achieving a robust…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

材料科学 · 物理学 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

Achieving strong coupling between light and matter is usually a challenge in Cavity Quantum Electrodynamics (cQED), especially in solid state systems. For this reason is useful taking advantage of alternative approaches to reach this…

介观与纳米尺度物理 · 物理学 2018-03-07 J. E. Ramírez-Muñoz , J. P. Restrepo Cuartas , H. Vinck-Posada

We demonstrate control over optical coupling between air-suspended carbon nanotubes and air-mode nanobeam cavities by spectral tuning. Taking advantage of the large dielectric screening effects caused by adsorbed molecules, laser heating is…

介观与纳米尺度物理 · 物理学 2018-08-24 H. Machiya , T. Uda , A. Ishii , Y. K. Kato

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

介观与纳米尺度物理 · 物理学 2015-05-13 I. V. Bondarev , L. M. Woods , K. Tatur

We investigate plasmon-emitter interactions in a nanoparticle-on-a-mirror cavity. We consider two different sorts of emitters, those that sustain dipolar transitions, and those hosting only quadrupolar, dipole-inactive, excitons. By means…

介观与纳米尺度物理 · 物理学 2020-01-15 A. Cuartero-González , A. I. Fernández-Domínguez

Strong coupling of excitonic resonances with a cavity gives rise to exciton-polaritons which possess a modified energy landscape compared to the uncoupled emitter. However, due to the femtosecond lifetime of the so-called bright polariton…

介观与纳米尺度物理 · 物理学 2022-05-19 Jan M. Lüttgens , Zhuoran Kuang , Nicolas F. Zorn , Tiago Buckup , Jana Zaumseil

The coherent strong coupling of molecules with confined light fields to create polaritons - part matter, part light - is opening exciting opportunities ranging from extended exciton transport and inter-molecular energy transfer to modified…

Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…

介观与纳米尺度物理 · 物理学 2025-07-11 Giuseppe Fumero , Jagannath Paul , Jared K. Wahlstrand , Alan D. Bristow