相关论文: Chirp Mixing
We propose a method to break the chiral symmetry of light in traveling wave resonators by coupling the optical modes to a lossy channel. Through the engineered dissipation, an indirect dissipative coupling between two oppositely propagating…
A broad effort is underway to improve the sensitivity of nuclear magnetic resonance through the use of dynamic nuclear polarization. Nitrogen-vacancy (NV) centers in diamond offer an appealing platform because these paramagnetic defects can…
We present an efficient scheme which couples any designated pair of spins in heteronuclear spin systems. The scheme is based on the existence of Hadamard matrices. For a system of $n$ spins with pairwise coupling, the scheme concatenates…
The first step in the coherent control of a photoinduced binary reaction is bond making or photoassociation. We have recently demonstrated coherent control of bond making in multi-photon femtosecond photoassociation of hot magnesium atoms,…
Single-shot supercontinuum spectral interferometry (SSSI) is an optical technique that can measure ultrafast transients in the complex index of refraction. This method uses chirped supercontinuum reference/probe pulses that need to be…
The outlook for producing useful practical devices within the paradigm of magnonics rests on our ability to emit, control and detect coherent exchange spin waves on the nanoscale. Here, we argue that all these key functionalities can be…
Four-wave mixing in resonant atomic vapors based on maximum coherence induced by Stark-chirped rapid adiabatic passage (SCRAP) is investigated theoretically. We show the advantages of a coupling scheme involving maximum coherence and…
We describe how the semiclassical theory of radical pair recombination reactions recently introduced by two of us [D. E. Manolopoulos and P. J. Hore, J. Chem. Phys. 139, 124106 (2013)] can be generalised to allow for different singlet and…
We introduce a theoretical framework for computaions of anisotropic multipolar exchange interactions found in many spin--orbit coupled magnetic systems and propose a method to extract these coupling constants using a density functional…
In the superradiance phenomenon, a collection of non-interacting atoms exhibits collective dissipation due to interaction with a common radiation field, resulting in a non-monotonic decay profile. This work shows that dissipative…
The theory of inter-spin-subband electric dipole spin resonance in transition metal dichalcogenide heterobilayers is proposed. Our symmetry analysis demonstrates that, in contrast to monolayers, the reduced symmetry of heterobilayers…
We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…
Frequent polarization reversals, or spin-flips, of a stored polarized beam in a high energy scattering asymmetry experiments may greatly reduce systematic errors of spin asymmetry measurements. A spin-flipping technique is being developed…
Squeezed states of spin systems are an important entangled resource for quantum technologies, particularly quantum metrology and sensing. Here we consider the generation of spin squeezed states by interacting the spins with a dissipative…
The synthesis of single-cycle, compressed optical and microwave pulses sparked novel areas of fundamental research. In the field of acoustics, however, such a generation has not been introduced yet. For numerous applications, the large…
Artificial spin ice (ASI) systems exhibit fascinating phenomena, such as frustration and the formation of magnetic monopole states, and Dirac strings. However, exploring the wave phenomena in these systems is elusive due to the weak dipolar…
We demonstrate that judicious shaping of a nanosecond-time-scale frequency chirp can dramatically enhance the formation rate of ultracold $^{87}$Rb$_{2}$ molecules. Starting with ultracold $^{87}$Rb atoms, we apply pulses of…
In chiral magnets with intrinsic inversion symmetry breaking, it has been known that two spin waves moving in opposite directions can propagate at different velocities, exhibiting a phenomenon called magnetochiral nonreciprocity which…
We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $\pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that…
A unified model of molecular and atomistic spin dynamics is presented enabling simulations both in microcanonical and canonical ensembles without the necessity of additional phenomenological spin damping. Transfer of energy and angular…