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The control of non-equilibrium phenomena in complex solids is an important research frontier, encompassing new effects like light induced superconductivity. Here, we show that coherent optical excitation of molecular vibrations in the…

Photo-excitation at terahertz and mid-infrared frequencies has emerged as a new way to manipulate functionalities in quantum materials, in some cases creating non-equilibrium phases that have no equilibrium analogue. In K$_3$C$_{60}$, a…

超导电性 · 物理学 2023-08-03 E. Rowe , B. Yuan , M. Buzzi , G. Jotzu , Y. Zhu , M. Fechner , M. Först , B. Liu , D. Pontiroli , M. Riccò , A. Cavalleri

Superconductivity in organic conductors is often tuned by the application of chemical or external pressure. With this type of tuning, orbital overlaps and electronic bandwidths are manipulated, whilst the properties of the molecular…

We report on a photo-induced transient state of YBa2Cu2O6+x in which transport perpendicular to the Cu-O planes becomes highly coherent. This effect is achieved by excitation with mid-infrared optical pulses, tuned to the resonant frequency…

超导电性 · 物理学 2014-06-04 S. Kaiser , C. R. Hunt , D. Nicoletti , W. Hu , I. Gierz , H. Y. Liu , M. Le Tacon , T. Loew , D. Haug , B. Keimer , A. Cavalleri

Far and mid infrared optical pulses have been shown to induce non-equilibrium unconventional orders in complex materials, including photo-induced ferroelectricity in quantum paraelectrics, magnetic polarization in antiferromagnets and…

Fullerene solids doped with alkali metals (A$_3$C$_{60}$, A = K, Rb, Cs) exhibit a superconducting transition temperature ($T_c$) as high as 40 K, and their unconventional superconducting properties have been a subject of debate. With…

超导电性 · 物理学 2023-10-24 Jianyu Li , Zhangkai Cao , Jiahao Su , Ruipeng Wang , Haipeng Li , Yusuke Nomura , Xiaosen Yang , Ho-Kin Tang

Recent experiments on K$_3$C$_{60}$ and layered copper-oxide materials have reported substantial changes in the optical response following application of an intense THz pulse. These data have been interpreted as the stimulation of a…

介观与纳米尺度物理 · 物理学 2019-01-02 Giuliano Chiriacò , Andrew J. Millis , Igor L. Aleiner

The discovery of a superconducting phase in sulfur hydride under high pressure with a critical temperature above 200 K has provided a new impetus to the search for even higher $T_c$. Theory predicted and experiment confirmed that the phase…

Hydrogen-based compounds have attracted significant attention in recent years due to the discovery of conventional superconductivity with high critical temperature under high pressure, rekindling hopes for searching room temperature…

超导电性 · 物理学 2024-11-20 Yao Ma , Mingqi Li , Wenjia Shi , Vei Wang , Pugeng Hou , Mi Pang

Metallic hydrogen and hydride materials stand as promising avenues to achieve room-temperature superconductivity. Characterized by their high phonon frequencies and moderate coupling strengths, several high-pressure hydrides were…

超导电性 · 物理学 2025-07-16 Chendi Xie , Adam D. Smith , Haoran Yan , Wei-Chih Chen , Yao Wang

Optical excitation in the cuprates has been shown to induce transient superconducting correlations above the thermodynamic transition temperature, $T_C$, as evidenced by the terahertz frequency optical properties in the non-equilibrium…

超导电性 · 物理学 2020-03-25 B. Liu , M. Först , M. Fechner , D. Nicoletti , J. Porras , T. Loew , B. Keimer , A. Cavalleri

Photoexcited K$_3$C$_{60}$ displays several properties reminiscent of equilibrium superconductivity, including transient optical spectra, pressure dependence, and I-V characteristics. However, these observations do not decisively establish…

超导电性 · 物理学 2025-02-28 G. De Vecchi , M. Buzzi , G. Jotzu , S. Fava , T. Gebert , G. Magnani , D. Pontiroli , M. Riccò , A. Cavalleri

The physics of optically-induced superconductivity remains poorly understood, with questions that range from the underlying microscopic mechanism to the macroscopic electrical response of the non-equilibrium phase. In this paper, we study…

By means of synchrotron X-ray diffraction, we studied the effect of high pressure, P, up to 13 GPa on the room temperature crystal structure of superconducting CaC6. In this P range, no change of the pristine space group symmetry,…

Superconductivity in the recently proposed ground-state structures of atomic metallic hydrogen is investigated over the pressure range 500 GPa to 3.5 TPa. Near molecular dissociation, the electron--phonon coupling $\lambda$ and renormalized…

超导电性 · 物理学 2015-05-28 Jeffrey M. McMahon , David M. Ceperley

We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter…

材料科学 · 物理学 2018-05-23 E. Uykur , R. Sankar , D. Schmitz , C. A. Kuntscher

Inspired by the striking discovery of metastable superconductivity in $\mathrm{K}_3\mathrm{C}_{60}$ at 100K, far above $T_{\textrm{c}}=20K$, we discuss possible mechanisms for long-lived, photo-induced superconductivity. Starting from a…

Pump-probe experiments performed on $\mathrm{K}_3\mathrm{C}_{60}$ have unveiled both optical and transport signatures of metastable light-induced superconductivity up to room temperature, far above $T_c$. Recent experiments have uncovered…

超导电性 · 物理学 2026-01-27 Sambuddha Chattopadhyay , Marios Michael , Andrea Cavalleri , Eugene Demler

Various transition metal trichalcogenides (TMTC) show the charge-density-wave and superconductivity, which provide an ideal platform to study the correlation between these two orderings and the mechanism of superconductivity. Currently,…

超导电性 · 物理学 2021-11-04 Binbin Yue , Wei Zhong , Wen Deng , Ting Wen , Yonggang Wang , Yunyu Yin , Pengfei Shan , Xiaohui Yu , Fang Hong

The discovery of superconductivity with a transition temperature (Tc) exceeding 40 K in La3Ni2O7 and (La,Pr)3Ni2O7 thin films at ambient pressure provides a viable platform for the experiments that can only be conducted under…

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