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相关论文: Is 1T-TaS$_2$ a 40 year old quantum spin liquid?

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The compounds 1T-TaX2 (X = S, Se) and 1T-NbSe2 have been considered as potential hosts of a quantum spin liquid phase. This is based on the widely held view that the Mott-Hubbard mechanism drives the insulating behaviour of its charge…

强关联电子 · 物理学 2025-09-23 C. J. Butler , M. Naritsuka , T. Hanaguri

1T-TaS$_2$ undergoes successive phase transitions upon cooling and eventually enters an insulating state of mysterious origin. Some consider this state to be a band insulator with interlayer stacking order, yet others attribute it to Mott…

强关联电子 · 物理学 2020-08-26 Y. D. Wang , W. L. Yao , Z. M. Xin , T. T. Han , Z. G. Wang , L. Chen , C. Cai , Yuan Li , Y. Zhang

1T-TaS$_2$ is a layered transition metal dichalgeonide with a very rich phase diagram. At T=180K it undergoes a metal to Mott insulator transition. Mott insulators usually display anti-ferromagnetic ordering in the insulating phase but…

强关联电子 · 物理学 2017-11-22 A. Ribak , I. Silber , C. Baines , K. Chashka , Z. Salman , Y. Dagan , A. Kanigel

Two-dimensional layered transition-metal-dichalcogenide compound 1T-TaS2 shows the rare coexistence of charge density wave (CDW) and electron correlation driven Mott transition. In addition, atomic-cluster spins on the triangular lattice of…

强关联电子 · 物理学 2022-07-28 Sudip Pal , Kranti Kumar , Rohit Sharma , A Banerjee , S B Roy , Je-Geun Park , A. K. Nigam , Sang-Wook Cheong

Strong electron correlation drives 1T-TaS2 from a half-filled metallic state into a Mott insulating phase, coexisting with a charge density wave at low temperatures. Under external stimuli such as pressure or ionic gating, superconductivity…

强关联电子 · 物理学 2026-03-04 Haiyang Chen , Zhiqiang Sun , Peng Chen

Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Strong electron-electron interaction can induce Mott insulating state, which is believed to host unusual correlated phenomena such as quantum spin liquid when quantum fluctuation dominates and unconventional superconductivity through…

强关联电子 · 物理学 2025-04-24 Qiang Gao , Haiyang Chen , Wen-shin Lu , Yang-hao Chan , Zhenhua Chen , Yaobo Huang , Zhengtai Liu , Peng Chen

The vicinity of a Mott insulating phase has constantly been a fertile ground for finding exotic quantum states, most notably the high Tc cuprates and colossal magnetoresistance manganites. The layered transition metal dichalcogenide 1T-TaS2…

强关联电子 · 物理学 2017-12-06 Shuang Qiao , Xintong Li , Naizhou Wang , Wei Ruan , Cun Ye , Peng Cai , Zhenqi Hao , Hong Yao , Xianhui Chen , Jian Wu , Yayu Wang , Zheng Liu

As one of the most intriguing states of matter, the chiral spin liquid (CSL) has attracted much scientific interest while its existence and mechanism in crystalline strongly correlated systems remain hotly debated. On the other hand, strong…

强关联电子 · 物理学 2024-04-09 Yixuan Huang , D. N. Sheng , Jian-Xin Zhu

A quantum spin liquid (QSL) is an exotic state of matter characterized by quantum entanglement and the absence of any broken symmetry. A long-standing open problem, which is a key for fundamental understanding the mysterious QSL states, is…

Mott insulating behavior is induced by strong electron correlation and can lead to exotic states of matter such as unconventional superconductivity and quantum spin liquids. Recent advances in van der Waals material synthesis enable the…

Here we report a comprehensive inelastic light scattering studies on 1T-TaS2 with different thickness. This compound is well known for its rich charge density wave phases. Along with that it has been one of the promising candidates for a…

强关联电子 · 物理学 2025-05-06 Vivek Kumar , Birender Singh , Pradeep Kumar

1$T$-TaS$_2$ is the only insulating transition-metal dichalcogenide (TMD) with an odd number of electrons per unit cell. This insulating state is non-magnetic, making it a potential spin-liquid candidate. The unusual electronic behavior…

强关联电子 · 物理学 2024-06-28 Amir Dalal , Jonathan Ruhman , Jörn W. F. Venderbos

Tuning the electronic properties of a matter is of fundamental interest in scientific research as well as in applications. Recently, the Mott insulator-metal transition has been reported in a pristine layered transition metal…

强关联电子 · 物理学 2020-05-29 Kunliang Bu , Wenhao Zhang , Ying Fei , Zongxiu Wu , Yuan Zheng , Jingjing Gao , Xuan Luo , Yu-Ping Sun , Yi Yin

1T-TaS$_2$ is a cluster Mott insulator on the triangular lattice with 13 Ta atoms forming a star of David cluster as the unit cell. We derive a two dimensional XXZ spin-1/2 model with four-spin ring exchange term to describe the effective…

强关联电子 · 物理学 2018-07-27 Wen-Yu He , Xiao Yan Xu , Gang Chen , K. T. Law , Patrick A. Lee

1T-tantalum disulphide (1T-TaS2) is a promising material to realize quantum spin liquid state and fractional excitations. Here, we take a closer look on the temperature dependent magnetic susceptibility of 1T-TaS2 at low magnetic fields to…

强关联电子 · 物理学 2022-07-28 Sudip Pal , S. B. Roy

The advent of twisted moir\'e heterostructures as a playground for strongly correlated electron physics has led to a plethora of experimental and theoretical efforts seeking to unravel the nature of the emergent superconducting and…

强关联电子 · 物理学 2022-05-06 Dominik Kiese , Yuchi He , Ciarán Hickey , Angel Rubio , Dante M. Kennes

Quantum spin liquids are quantum phases of matter featuring collectively entangled states and emergent fractional many-body excitations. While methods exist to probe three-dimensional quantum spin liquids experimentally, these techniques…

More than half a century after first being proposed by Sir Nevill Mott, the deceptively simple question of whether the interaction-driven electronic metal-insulator transition may be continuous remains enigmatic. Recent experiments on…

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

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