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Engineering of the dielectric environment represents a powerful strategy to control the electronic and optical properties of two-dimensional (2D) materials without compromising their structural integrity. Here we show that the recent…

材料科学 · 物理学 2020-11-18 Anders C. Riis-Jensen , Morten N. Gjerding , Saverio Russo , Kristian S. Thygesen

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

介观与纳米尺度物理 · 物理学 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

材料科学 · 物理学 2019-11-04 Xiaoyang Zheng , Xian Zhang

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

介观与纳米尺度物理 · 物理学 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

The existence of strongly bound excitons is one of the hallmarks of the newly discovered atomically thin semi-conductors. While it is understood that the large binding energy is mainly due to the weak dielectric screening in two dimensions…

材料科学 · 物理学 2016-01-20 Simone Latini , Thomas Olsen , Kristian S. Thygesen

Excitons in transition metal dichalcogenides (TMDs) have emerged as a promising platform for novel applications ranging from optoelectronic devices to quantum optics and solid state quantum simulators. While much progress has been made…

High energy (C, D) excitons possess remarkable influence over the optical properties of layered transition metal dichalcogenides (TMDCs) and comprehensive understanding of these may have revolutionary effect on 2D opto-electronic devices.…

Monolayer semiconductors, given their thickness at the atomic scale, present unique electrostatic environments due to the sharp interfaces between the semiconductor film and surrounding materials. These interfaces significantly impact both…

介观与纳米尺度物理 · 物理学 2026-05-22 Kelly Y. Muñoz-Gómez , Hanz Y. Ramírez-Gómez

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…

介观与纳米尺度物理 · 物理学 2023-08-15 Jenny Hu , Etienne Lorchat , Xueqi Chen , Kenji Watanabe , Takashi Taniguchi , Tony F. Heinz , Puneet A. Murthy , Thibault Chervy

Atomically thin layers of transition metal dichalcogenides (TMDCs) exhibit exceptionally strong Coulomb interaction between charge carriers due to the two-dimensional carrier confinement in connection with weak dielectric screening. The van…

材料科学 · 物理学 2018-07-18 A. Steinhoff , T. O. Wehling , M. Rösner

Dark excitons in transition metal dichalcogenides (TMD) have been so far neglected in the context of polariton physics due to their lack of oscillator strength. However, in tungsten-based TMDs, dark excitons are known to be the…

As the bound state of two oppositely charged particles, excitons emerge from optically excited semiconductors as the electronic analogue of a hydrogen atom. In the two-dimensional (2D) case, realized either in quantum well systems or truly…

光学 · 物理学 2022-05-13 Tobias Graß , Utso Bhattacharya , Julia Sell , Mohammad Hafezi

We theoretically examined how the dielectric screening of two-dimensional layered materials affects the dipolar interaction between interlayer excitons in few-layer van der Waals structures. Our analysis indicates that the dipolar…

介观与纳米尺度物理 · 物理学 2024-02-14 Yuhang Hou , Hongyi Yu

We theoretically study the effect of the dielectric environment on the exciton ground state of CdSe and CdTe/CdSe/CdTe nanorods. We show that insulating environments enhance the exciton recombination rate and blueshift the emission peak by…

介观与纳米尺度物理 · 物理学 2015-05-20 Miquel Royo , Juan Ignacio Climente , José Luis Movilla , Josep Planelles

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

材料科学 · 物理学 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

We propose to engineer topological exciton structures in layered transition metal dichalcogenides through hybridizing different Rydberg states, which can be induced by a periodic electrostatic potential remotely imprinted from charge…

介观与纳米尺度物理 · 物理学 2025-10-09 Na Zhang , Wang Yao , Hongyi Yu

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal…

In this work, we present a comprehensive theoretical and computational investigation of exciton fine structures of WSe$_2$-monolayers, one of the best known two-dimensional (2D) transition-metal dichalcogenides (TMD's), in various…

介观与纳米尺度物理 · 物理学 2023-02-23 Wei-Hua Li , Jhen-Dong Lin , Ping-Yuan Lo , Guan-Hao Peng , Ching-Yu Hei , Shao-Yu Chen , Shun-Jen Cheng

Transition-metal dichalcogenide bilayers exhibit a rich exciton landscape including layer-hybridized excitons, i.e. excitons which are of partly intra- and interlayer nature. In this work, we study hybrid exciton-exciton interactions in…

介观与纳米尺度物理 · 物理学 2023-06-28 Daniel Erkensten , Samuel Brem , Raul Perea-Causin , Joakim Hagel , Fedele Tagarelli , Edoardo Lopriore , Andras Kis , Ermin Malic

Controlling excitons and their transport in two-dimensional (2D) transition metal dichalcogenides (TMDs) heterostructures is central to advancing photonics and electronics on-chip integration. We investigate the controlled generation and…

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