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相关论文: Radiative association of C(${}^3P$) and H${}^+$: T…

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We investigate the photodissociation of the metastable triplet state of HeH+ as well as its formation through the inverse process, radiative association. In models of astrophysical plasmas, HeH+ is assumed to be present only in the ground…

化学物理 · 物理学 2015-06-12 J. Loreau , S. Vranckx , M. Desouter-Lecomte , N. Vaeck , A. Dalgarno

We present calculated cross sections and rate coefficients for the formation of the dicarbon cation (C$_2^+$) by the radiative association process in collisions of a C$(^3P)$ atom and a C$^+(^2P^o)$ ion. Molecular structure calculations for…

原子物理 · 物理学 2019-10-24 James F. Babb , R. T. Smyth , B. M. McLaughlin

We illustrate some of the difficulties that may be encountered when computing photodissociation and radiative association cross sections from the same time-dependent approach based on wavepacket propagation. The total and partial…

化学物理 · 物理学 2015-06-12 S. Vranckx , J. Loreau , M. Desouter-Lecomte , N. Vaeck

The matrix elements and energies needed to calculate vibrational-rotational state resolved cross sections and rate coefficients for radiative association of H and p and for photodissociation of H${}_2^+$ are presented for applications to…

原子物理 · 物理学 2015-01-21 James F. Babb

Cross sections and rate coefficients for rovibronic excitation of the CH$^+$ ion by electron impact and dissociative recombination of CH$^+$ with electrons are evaluated using a theoretical approach combining an R-matrix method and…

星系天体物理 · 物理学 2025-11-25 Joshua Forer , Dávid Hvizdoš , Mehdi Ayouz , Chris H. Greene , Viatcheslav Kokoouline

Radiative charge exchange collisions between a carbon atom C(${}^3$P) and a helium ion He+, both in their ground state, are investigated theoretically. Detailed quantum chemistry calculations are carried out to obtain potential energy…

原子物理 · 物理学 2017-01-25 James F. Babb , B. M. McLaughlin

Radiative association processes leading to the formation of AgH in cold astrophysical environments are investigated for the first time using full quantum scattering theory. High accuracy potential energy curves and transition dipole moments…

原子物理 · 物理学 2026-03-27 Lin Jiang , Yu Wang , Yukun Yang , Xuanbing Qiu , Yali Tian , Guqing Guo , Ling Liu , Chuanliang Li , Yong Wu

We present a detailed theoretical study of the rotational excitation of CH$^+$ due to reactive and nonreactive collisions involving C$^+(^2P)$, H$_2$, CH$^+$, H and free electrons. Specifically, the formation of CH$^+$ proceeds through the…

We have developed the polyatomic extension of a recently established (M. Gustafsson, J. Chem. Phys, 138, 074308 (2013)) classical theory of radiative association in the absence of electronic transitions. The cross section of the process is…

化学物理 · 物理学 2021-10-22 Péter Szabó , Magnus Gustafsson

The dynamics of the reaction H + OH $\to$ O (3P) + H2 have been studied in a series of quasi-classical trajectory (QCT) calculations and transition state theory (TST) methods using high quality 3A' and 3A'' potential energy surfaces (PESs).…

太阳与恒星天体物理 · 物理学 2014-02-27 Xiaohu Li , Carina Arasa , Marc C. van Hemert , Ewine F. van Dishoeck

Radiative association cross sections and rates are computed, using a quantum approach, for the formation of C$_2$ molecules (dicarbon) during the collision of two ground state C($^3$P) atoms. We find that transitions originating in the…

宇宙学与河外天体物理 · 物理学 2021-03-29 James F. Babb , R. T. Smyth , B. M. McLaughlin

Photodissociation cross sections for the SH$^+$ radical are computed from all rovibrational (RV) levels of the ground electronic state X$~^3\Sigma^-$ for wavelengths from threshold to 500~\AA. The five electronic transitions, $2~ ^3\Sigma^-…

地球与行星天体物理 · 物理学 2016-05-04 E. C. McMillan , G. Shen , J. F. McCann , B. M. McLaughlin , P. C. Stancil

We have observed short-range photoassociation of LiRb to the two lowest vibrational states of the $d\,^3\Pi$ potential. These $d\,^3\Pi$ molecules then spontaneously decay to vibrational levels of the $a^3\,\Sigma^+$ state with generation…

The article presents calculated dissociative recombination (DR) rate coefficients for H+3 . The previous theoretical work on H+3 was performed using the adiabatic hyperspherical approximation to calculate the target ion vibrational states…

原子物理 · 物理学 2007-08-22 Samantha Fonseca dos Santos , Viatcheslav Kokoouline , Chris H. Greene

We establish a theoretical model to analyze the photoassociative (PA) spectroscopy of $(3)^3\Sigma^+$ state of $^{85}$Rb$^{133}$Cs molecule. The term energy, spin-spin coupling constants and hyperfine interaction constant of nine…

原子物理 · 物理学 2022-05-25 Zi-wei Wang , Zi-ang Li , Xu-hui Bai , Ting Gong , Zhong-hua Ji , Yan-ting Zhao , Gao-ren Wang

Rate constants have been measured for the C(3P) + CH3CN reaction between 50 K and 296 K using a continuous-flow supersonic reactor. C(3P) atoms were created by the in-situ pulsed laser photolysis of CBr4 at 266 nm, while the kinetics of…

星系天体物理 · 物理学 2021-03-26 Kevin M. Hickson , Jean-Christophe Loison , Valentine Wakelam

The cross section for resonant ion-pair formation in the collision of low-energy electrons with HF^+ is calculated by the solution of the time-dependent Schrodinger equation with multiple coupled states using a wave packet method. A…

原子物理 · 物理学 2015-05-13 J. B. Roos , A. E. Orel , AA. Larson

The first metastable triplet state of HeH$^+$ was found to be present in ion beam experiments, with its lifetime estimated to be between hundreds of milliseconds and thousand of seconds. In this work, we use {\it ab initio} methods to…

原子物理 · 物理学 2015-05-19 J. Loreau , J. Liévin , N. Vaeck

We used the multichannel quantum defect theory to compute cross sections and rate coefficients for the dissociative recombination of CH$^+$ initially in its lowest vibrational level $v_i^+ = 0$ with electrons of incident energy bellow $0.2$…

天体物理仪器与方法 · 物理学 2022-03-08 J. Zs. Mezei , M. D. Epée Epée , O. Motapon , I. F. Schneider

We aim to obtain accurate rate coefficients for the collisional excitation of CH+ by He for high gas temperatures. The ab initio coupled-cluster [CCSD(T)] approximation was used to compute the interaction potential energy. Cross sections…

太阳与恒星天体物理 · 物理学 2015-05-14 K. Hammami , L. C. Owono Owono , P. Staeuber
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