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This paper reports on the spin glass-like coexistence of competing magnetic orders in oxygen-deficient V2O5 nanoparticles having a broad size distribution. X-ray photoelectron spectroscopy yields the surface chemical stoichiometry of nearly…

Different from other magnetically frustrated spinel systems, GeCu$_{2}$O$_{4}$ is a strongly tetragonal distorted spinel cuprate in which edge-sharing CuO$_{2}$ ribbons are running along alternating directions perpendicular to the $c$-axis.…

强关联电子 · 物理学 2018-05-02 L. Zhao , L. Muzica , U. Schwarz , A. C. Komarek

The resolution of geometric frustration in systems with continuous degrees of freedom often involves a cooperative inhomogeneous response and super-extensive energy scaling. In contrast, the frustration in frustrated Ising-like spin systems…

软凝聚态物质 · 物理学 2022-06-29 Snir Meiri , Efi Efrati

Nuclear magnetic resonance (NMR), electron paramagnetic resonance (EPR), magnetization measurements and electronic structure calculations in VOMoO4 are presented. It is found that VOMoO4 is a frustrated two-dimensional antiferromagnet on a…

强关联电子 · 物理学 2009-11-07 P. Carretta , N. Papinutto , C. B. Azzoni , M. C. Mozzati , E. Pavarini , S. Gonthier , P. Millet

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

强关联电子 · 物理学 2010-07-13 Gia-Wei Chern , Natalia Perkins

The A-site spinel material, CoAl2O4, is a physical realization of the frustrated diamond-lattice antiferromagnet, a model in which is predicted to contain unique incommensurate or `spin-spiral liquid' ground states. Our previous…

In frustrated magnets when magnetic ordering is suppressed down to low temperature, the formation of a quantum spin liquid becomes a possibility. How such a spin liquid manifests in the presence of conduction electrons is a question with…

强关联电子 · 物理学 2014-02-26 Jeffrey G. Rau , Hae-Young Kee

Phase inhomogeneity of otherwise chemically homogenous electronic systems is an essential ingredient leading to fascinating functional properties, such as high-$T_c$ superconductivity in cuprates, colossal magnetoresistance in manganites,…

强关联电子 · 物理学 2014-01-30 Andrej Zorko , Othon Adamopoulos , Matej Komelj , Denis Arćon , Alexandros Lappas

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

强关联电子 · 物理学 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

The structural and magnetic properties of spinel compounds $CoB_2O_4$ (B=Cr,Mn and Fe) are studied using the DFT+U method and generalized gradient approximation (GGA). We concentrate on understanding the trends in the properties of these…

强关联电子 · 物理学 2016-09-21 Debashish Das , Rajkumar Biswas , Subhradip Ghosh

The magnetic ground state of oxynitride pyrochlore Lu$_2$Mo$_2$O$_{5-y}$N$_2$, a candidate compound for the quantum spin liquid ($S=1/2$, Mo$^{5+}$), was studied by muon spin rotation/relaxation experiment. In contrast to Lu$_2$Mo$_2$O$_7$…

强关联电子 · 物理学 2023-01-11 S. K. Dey , K. Ishida , H. Okabe , M. Hiraishi , A. Koda , T. Honda , J. Yamaura , H. Kageyama , R. Kadono

Recent experimental studies on Fe substituted spinel CoCr$_{2}$O$_{4}$ have discovered multiple functional properties in the system such as temperature and composition dependent magnetic compensation, tunable exchange bias and…

材料科学 · 物理学 2018-08-29 Debashish Das , Subhradip Ghosh

Traditional frustration arises from the conflict between the spin alignments due to the geometry or the nature of the interactions. Here, we demonstrate a novel form of frustration, dubbed ``emergent frustration'', which is induced by the…

强关联电子 · 物理学 2025-04-21 Zehui Deng , Lu Liu , Wenan Guo , Hai-Qing Lin

Single crystal elastic and inelastic neutron scattering experiments are performed on the frustrated ferro-antiferromagnet SrZnVO(PO4)2 in high magnetic fields. The fully polarized state, the presaturation phase and the…

强关联电子 · 物理学 2022-08-31 F. Landolt , K. Povarov , Z. Yan , S. Gvasaliya , E. Ressouche , S. Raymond , V. O. Garlea , A. Zheludev

The mixed spin-(1/2, 3/2) Ising model on a decorated square lattice, which takes into account lattice vibrations of the spin-3/2 decorating magnetic ions at a quantum-mechanical level under the assumption of a perfect lattice rigidity of…

统计力学 · 物理学 2020-07-06 Jozef Strecka , Onofre Rojas , Sergio Martins de Souza

We have studied the structural, electronic and magnetic properties of spinel $\rm Co_3O_4$(111) surfaces and their interfaces with ZnO (0001) using density functional theory (DFT) within the Generalized Gradient Approximation with on-site…

材料科学 · 物理学 2018-03-21 Igor Kupchak , Natalia Serpak , Anatoli Shkrebtii , Roland Hayn

We investigated the isotropic spin-1/2 Heisenberg model on an anisotropic square lattice with competing exchange interactions, motivated by the unconventional magnetic behavior observed in the verdazyl-based compound (o-MePy-V)PF6. Using a…

强关联电子 · 物理学 2025-11-21 L. M. Ramos , M. Schmidt , F. M. Zimmer

Quantum spin liquids provide paradigmatic examples of highly entangled quantum states of matter. Frustration is the key mechanism to favor spin liquids over more conventional magnetically ordered states. Here we propose to engineer…

强关联电子 · 物理学 2021-11-29 Alessio Chiocchetta , Dominik Kiese , Carl Philipp Zelle , Francesco Piazza , Sebastian Diehl

Beyond a conventional classification of ferroelectricity, there is a class of materials where electronic degrees of freedom and electronic interactions are directly responsible for electric polarization and ferroelectric transition. This is…

强关联电子 · 物理学 2015-05-14 Sumio Ishihara

Spin fluctuations were studied over a wide momentum ($\hbar Q$) and energy ($E$) space in the frustrated $d$-electron heavy-fermion metal LiV$_2$O$_4$ by time-of-flight inelastic neutron scattering. We observed the overall $Q$$-$$E$…

强关联电子 · 物理学 2015-03-10 K. Tomiyasu , K. Iwasa , H. Ueda , S. Niitaka , H. Takagi , S. Ohira-Kawamura , T. Kikuchi , K. Nakajima , K. Yamada