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Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

材料科学 · 物理学 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

We theoretically investigate the generation of ultrafast currents in insulators induced by strong few-cycle laser pulses. Ab initio simulations based on time-dependent density functional theory give insight into the atomic-scale properties…

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Stoner and Heisenberg excitations in magnetic materials are inherently different. The former involves an effective reduction of the exchange splitting, whereas the latter comprises excitation of spin-waves. In this work, we test the impact…

材料科学 · 物理学 2022-03-14 Mohamed F. Elhanoty , Olle Eriksson , Ronny Knut , Olof Karis , Oscar Grånäs

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Recent developments of the sources of intense and ultrashort X-ray pulses stimulate theoretical studies of phenomena occurring on ultrafast timescales. In the present study, spin-flip dynamics in transition metal complexes triggered by…

化学物理 · 物理学 2020-08-26 Vladislav Kochetov , Huihui Wang , Sergey I. Bokarev

Optical pump-probe setups are commonly used for excitation and investigation of the spin dynamics in various types of magnetic materials. However, usually the spatially homogeneous excitation is considered. In the present study we describe…

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

材料科学 · 物理学 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

All-optical switching in a ferromagnetic spin valve is studied here using atomistic spin drift-diffusion dynamics, which includes contributions from spin pumping and superdiffusive transport. We find the switching is governed principally by…

介观与纳米尺度物理 · 物理学 2026-02-23 Serban Lepadatu , Mohammed Gija , Alexey Dobrynin , Kevin McNeill , Mark Gubbins , Tim Mercer , Steven M. McCann , Philip Bissell

Synthetic ferrimagnets are composite magnetic structures formed from two or more anti- ferromagnetically coupled magnetic sublattices with different magnetic moments. Here we report on atomistic spin simulations of the laser-induced…

材料科学 · 物理学 2014-06-10 Richard F. L. Evans , Thomas A. Ostler , Roy W. Chantrell , Ilie Radu , Theo Rasing

Experimentally observed ultrafast all-optical magnetization reversal in ferrimagnetic metals and heterostructures based on antiferromagnetically coupled ferromagnetic $d-$ and $f-$metallic layers relies on intricate energy and angular…

强关联电子 · 物理学 2016-03-02 Alexandra Kalashnikova , Veniamin Kozub

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

Deterministic all-optical control of magnetization without an applied magnetic field has been reported for different materials such as ferrimagnetic and ferromagnetic thin films and granular recording media. These findings have challenged…

Quantum mechanical superexchange interactions form the basis of quantum magnetism in strongly correlated electronic media. We report on the direct measurement of superexchange interactions with ultracold atoms in optical lattices. After…

其他凝聚态物理 · 物理学 2008-04-17 S. Trotzky , P. Cheinet , S. Fölling , M. Feld , U. Schnorrberger , A. M. Rey , A. Polkovnikov , E. A. Demler , M. D. Lukin , I. Bloch

We have performed time-resolved resonant x-ray scattering studies in the Lanthanide metal Dy to reveal the dynamic response of the helical order exchange coupling to injection of unpolarized spins. The observed spin dynamics are…

By combining interface-sensitive non-linear magneto-optical experiments with femtosecond time resolution and ab-initio time-dependent density functional theory, we show that optically excited spin dynamics at Co/Cu(001) interfaces proceeds…

Faster magnetic recording technology is indispensable to massive data storage and big data sciences. {All-optical spin switching offers a possible solution}, but at present it is limited to a handful of expensive and complex rare-earth…

材料科学 · 物理学 2016-11-03 G. P. Zhang , Y. H. Bai , T. F. George

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

介观与纳米尺度物理 · 物理学 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

The anti-Stoner excitations are a spin-flips in which, effectively, an electron is promoted from a minority to a majority spin state, i.e., complementary to Stoner excitations and spin-waves. Since their spectral power is negligible in…

材料科学 · 物理学 2024-06-21 S. Paischer , D. Eilmsteiner , M. I. Katsnelson , A. Ernst , P. A. Buczek

Starting from the continuity equation for the magnetization in time-dependent spin-density functional theory, we derive an expression for the effective time-dependent magnetic fields driving the out-of-equilibrium spin dynamics in magnetic…

介观与纳米尺度物理 · 物理学 2017-01-18 Jacopo Simoni , Maria Stamenova , Stefano Sanvito