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A broken translation symmetry has recently been revealed in infinite-layer nickelates, which has piqued considerable interest in its origin and relation to superconductivity, as well as in its comparison to charge order in cuprates. Here,…

The discovery of unconventional superconductivity around 80 K in perovskite nickelates under high pressure has furnished a new platform to explore high-temperature unconventional superconductivity in addition to cuprates. Understanding the…

Magnetic ordering phenomena have a profound influence on the macroscopic properties of correlated-electron materials, but their realistic prediction remains a formidable challenge. An archetypical example is the ternary nickel oxide system…

We report detailed magnetization measurements on the perovskite oxide NdNiO$_3$. This system has a first order metal-insulator (M-I) transition at about 200 K which is associated with charge ordering. There is also a concurrent paramagnetic…

强关联电子 · 物理学 2016-01-11 Devendra Kumar , K. P. Rajeev , J. A. Alonso , M. J. Martinez-Lope

The discovery of superconductivity in square-planar low valence nickelates has ignited a vigorous debate regarding their essential electronic properties: Do these materials have appreciable oxygen charge-transfer character akin to the…

The magnetic properties of GdBaMn_{2}O_{5.0}, which exhibits charge ordering, are studied from 2 to 400 K using single crystals. In a small magnetic field applied along the easy axis, the magnetization M shows a temperature-induced reversal…

材料科学 · 物理学 2009-11-13 A. A. Taskin , Yoichi Ando

Rare-earth nickelates RNiO3 (R=rare-earth element) exhibit three kinds of phase transitions with decreasing temperature: a structural transition from a pseudo-cubic to a monoclinic phase, a metal- insulator transition (MIT), and a magnetic…

We investigate the order parameter dynamics of the stripe-ordered nickelate, La$_{1.75}$Sr$_{0.25}$NiO$_4$, using time-resolved resonant X-ray diffraction. In spite of distinct spin and charge energy scales, the two order parameters'…

The observation of superconductivity in infinite layer nickelate (Nd,Sr)NiO$_{2}$ thin films has led to rapid theoretical and experimental investigations of these copper-oxide-analogue systems [1-15]. Superconductivity has also been found…

In this letter, we report the structural, electronic and ferroelectric properties of the layered mixed-valent transition-metal compound, Sr$_{4}$Fe$_{6}$O$_{12}$ (SFO). We demonstrate how SFO undergoes a phase transition from a…

强关联电子 · 物理学 2025-02-05 Arindam Sarkar , Hena Das , Prashant Singh , Aftab Alam

We are reporting the dielectric response of La1.5Sr0.5NiO4, a system that presents a charge-ordered state above room temperature and a rearrangement of its charge-order pattern in the temperature region 160-200 K. A careful analysis of the…

材料科学 · 物理学 2009-11-10 J. Rivas , B. Rivas-Murias , A. Fondado , J. Mira , M. A. Senaris-Rodriguez

The consequences of varying the rare-earth element in the superconducting infinite-layer nickelates have been much debated. Here we show striking differences in the magnitude and anisotropy of the superconducting upper critical field across…

Double perovskites extend the design space for new materials, and they often host phenomena that don't exist in their parent perovskite compounds. Here, we present a detailed first principles study of the correlated double perovskite…

强关联电子 · 物理学 2020-08-05 Arpita Paul , Turan Birol

We present an unrestricted Hartree-Fock computation of charge-ordering instabilities of two-dimensional metals with antiferromagnetic exchange interactions, allowing for arbitrary ordering wavevectors and internal wavefunctions of the…

超导电性 · 物理学 2013-07-15 Subir Sachdev , Rolando La Placa

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

The short-range organization around Ni atoms in orthorhombic $R$NiO$_{3}$ ($R$=Pr,Nd,Eu) perovskites has been studied over a wide temperature range by Ni K-edge x-ray absorption spectroscopy. Our results demonstrate that two different Ni…

The electronic structure and magnetism in the sodium nickelate NaNiO_2 in the low-temperature phase is studied from density-functional calculations using the linear muffin-tin orbitals method. An antiferromagnetic solution with a magnetic…

强关联电子 · 物理学 2009-11-10 H. Meskine , S. Satpathy

Charge fluctuations in the quasi-one-dimensional material Li0.9Mo6O17 are analyzed based on a multi orbital extended Hubbard model. A charge ordering transition induced by Coulomb repulsion is found with a charge ordering pattern different…

强关联电子 · 物理学 2015-08-03 J. Merino , J. V. Alvarez

The recent discovery of superconductivity in infinite-layer nickelates has drawn considerable attention; however, a consensus on the fundamental building blocks and common ingredients necessary to understand and describe their ground states…

强关联电子 · 物理学 2023-12-07 Cheng Peng , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux , Chunjing Jia

A hypothetical layered oxide La_2NiMO_6 where NiO_2 and MO_2 planes alternate along the c-axis of ABO_3 perovskite lattice is considered theoretically. Here, M denotes a trivalent cation Al, Ga,... such that MO_2 planes are insulating and…

强关联电子 · 物理学 2010-05-11 Jiri Chaloupka , Giniyat Khaliullin