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Single- and few-layer transition metal dichalcogenides have recently emerged as a new family of layered crystals with great interest, not only from the fundamental point of view, but also because of their potential application in ultrathin…

Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

The valley degree of freedom is a sought-after quantum number in monolayer transition-metal dichalcogenides. Similar to optical spin orientation in semiconductors, the helicity of absorbed photons can be relayed to the valley (pseudospin)…

介观与纳米尺度物理 · 物理学 2020-04-01 Min Yang , Cedric Robert , Zhengguang Lu , Dinh Van Tuan , Dmitry Smirnov , Xavier Marie , Hanan Dery

We study the conduction band spin splitting that arises in transition metal dichalcogenide (TMD) semiconductor monolayers such as MoS$_2$, MoSe$_2$, WS$_2$ and WSe$_2$ due to the combination of spin-orbit coupling and lack of inversion…

材料科学 · 物理学 2014-01-01 K. Kośmider , J. W. González , J. Fernández-Rossier

We present photoluminescence measurements in monolayer WSe$_2$, which point to the importance of the interaction between charged particles and excitonic complexes. The theoretical analysis highlights the key role played by exchange…

Electric field-controlled, two-dimensional (2D) exciton dynamics in transition metal dichalcogenide monolayers is a current research focus in condensed matter physics. We have experimentally investigated the spectral and temporal properties…

介观与纳米尺度物理 · 物理学 2019-12-11 Michael Engel , Mathias Steiner

Semiconducting transition metal dichalcogenides of group VI are well-known for their prominent excitonic effects and the transition from an indirect to a direct band gap when reduced to monolayers. While considerable efforts have elucidated…

The monolayers of semiconducting transition metal dichalcogenides host strongly bound excitonic complexes and are an excellent platform for exploring many-body physics. Here we demonstrate a controlled kinetic manipulation of the…

介观与纳米尺度物理 · 物理学 2022-04-05 Suman Chatterjee , Sarthak Das , Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

介观与纳米尺度物理 · 物理学 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of the Coulomb interaction leads to strongly correlated many-body states, including excitons and trions, that dominate the optical properties.…

We observe the interlayer A1s^I, A2s^I, and B1s^I excitons in bilayer WSe2 under applied electric fields using reflectance contrast spectroscopy. Remarkably, these interlayer excitons remain optically bright despite being well separated…

Single-layer transition metal dichalcogenides (TMDs) provide a promising material system to explore the electron's valley degree of freedom as a quantum information carrier. The valley degree of freedom in single-layer TMDs can be directly…

介观与纳米尺度物理 · 物理学 2019-10-09 Yanhao Tang , Kin Fai Mak , Jie Shan

Charged excitons (trions) are essential for the optical spectra in low dimensional doped monolayers (ML) of transitional metal dichalcogenides (TMDC). Using a direct diagonalization of the three-body Hamiltonian, we explore the low-lying…

材料科学 · 物理学 2023-01-23 Yaroslav V. Zhumagulov , Alexei Vagov , Dmitry R. Gulevich , Vasili Perebeinos

Many monolayer transition metal dichalcogenides, including MoS$_2$, MoSe$_2$, WS$_2$, and WSe$_2$, are direct bandgap two-dimensional (2D) semiconductors with sharp optical resonances at excitonic bound state frequencies. Recent experiments…

介观与纳米尺度物理 · 物理学 2025-10-27 Tobias M. R. Wolf , Tian Xie , Chenhao Jin , Allan H. MacDonald

Transition metal dichalcogenides represent an ideal testbed to study excitonic effects, spin-related phenomena and fundamental light-matter coupling in nanoscopic condensed matter systems. In particular, the valley degree of freedom, which…

In atomically thin two-dimensional semiconductors such as transition metal dichalcogenides (TMDs), controlling the density and type of defects promises to be an effective approach for engineering light-matter interactions. We demonstrate…

介观与纳米尺度物理 · 物理学 2018-08-15 Galan Moody , Kha Tran , Xiaobo Lu , Travis Autry , James M. Fraser , Richard P. Mirin , Li Yang , Xiaoqin Li , Kevin L. Silverman

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

介观与纳米尺度物理 · 物理学 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

We investigate the properties of momentum-dark excitons and trions formed in two-dimensional (2D) materials that exhibit an inverted Mexican-hat-shaped dispersion relation, taking monolayer InSe as an example. We employ variational…

介观与纳米尺度物理 · 物理学 2025-07-24 Lewis J. Burke , Mark T. Greenaway , Joseph J. Betouras

In many paradigmatic materials, like Transition Metal Dichalcogenides, the role played by the spin degrees of freedom is as important as the one played by the electron-electron interaction. Thus an accurate treatment of the two effects and…

Two-dimensional (2D) materials, such as graphene1, boron nitride2, and transition metal dichalcogenides (TMDs)3-5, have sparked wide interest in both device physics and technological applications at the atomic monolayer limit. These 2D…