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Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…

介观与纳米尺度物理 · 物理学 2017-08-31 Lucas V. Besteiro , Xiang-Tian Kong , Zhiming Wang , Gregory V. Hartland , Alexander O. Govorov

In plasmonics, and particularly in plasmonic photochemistry, the effect of hot-electron generation is an exciting phenomenon driving new fundamental and applied research. However, obtaining a microscopic description of the hot-electron…

The generation of the localized surface plasmon resonance (LSPR) on the surface of plasmonic structures in the nanoscale has paved the way for advanced biosensing, surpassing the conventional detection limits. The electric field enhancement…

光学 · 物理学 2023-12-12 Siddhartha Banerjee , Jolly Xavier

Metal nanoparticles are attractive for plasmon-enhanced generation of hot carriers, which may be harnessed in photochemical reactions. In this work, we analyze the coherent femtosecond dynamics of photon absorption, plasmon formation, and…

介观与纳米尺度物理 · 物理学 2021-01-14 Tuomas P. Rossi , Paul Erhart , Mikael Kuisma

The use of biomaterials - with techniques such as DNA-directed assembly or bio-directed synthesis - can surpass top-down fabrication techniques in creating plasmonic superstructures, in terms of spatial resolution, range of functionality…

We theoretically study hot electron generation through the emission of a dipole source coupled to a nanoresonator on a metal surface. In our hybrid approach, we solve the time-harmonic Maxwell's equations numerically and apply a quantum…

Metal nanoparticles are excellent light absorbers. The absorption processes create highly excited electron-hole pairs and recently there has been interest in harnessing these hot charge carriers for photocatalysis and solar energy…

介观与纳米尺度物理 · 物理学 2017-06-13 Gregory V. Hartland , Lucas V. Besteiro , Paul Johns , Alexander O. Govorov

Energetic or "hot" electrons and holes generated from the decay of localized surface plasmons in metallic nanoparticles have great potential for applications in photocatalysis, photovoltaics, and sensing. Here, we study the generation of…

光学 · 物理学 2024-12-20 Simão M. João , Ottavio Bassano , Johannes Lischner

Energetic and optical properties of plasmonic nanocrystals strongly depend on their sizes, shapes, and composition. Whereas using plasmonic nanoparticles in biotesting has become routine, applications of plasmonics in energy are still early…

Highly nonlinear optical processes, such as multiphoton photoemission, require high intensities, typically achieved with ultrashort laser pulses and, hence, were first observed with the advent of picosecond laser technology. An alternative…

Plasmonic structures are renowned for their capability to efficiently convert light into heat at the nanoscale. However, despite the possibility to generate deep sub-wavelength electromagnetic hot spots, the formation of extremely localized…

Hot electrons generated from the decay of localized surface plasmons in metallic nanostructures have the potential to transform photocatalysis, photodetection and other optoelectronic applications. However, the understanding of hot-carrier…

In this paper we use layer potentials and asymptotic analysis techniques to analyze the heat generation due to nanoparticles when illuminated at their plasmonic resonance. We consider arbitrary-shaped particles and both single and multiple…

偏微分方程分析 · 数学 2017-03-02 Habib Ammari , Francisco Romero , Matias Ruiz

In this paper, we investigate the photothermal effects of the plasmon resonance. Metal nanoparticles efficiently generate heat in the presence of electromagnetic radiation. The process is strongly enhanced when a fixed frequency of the…

偏微分方程分析 · 数学 2013-12-17 Xiaoping Fang , Youjun Deng , Jing Li

New type of plasmonic nanoparticles - silver octopods that can be synthesized with a variety of shapes - have been demonstrated to show versatile optical response using the discrete dipole approximation. The octopods show a complex behavior…

介观与纳米尺度物理 · 物理学 2015-05-13 Ivan I. Naumov , Zhiyong Li , Alexander M. Bratkovsky

Hot electrons and holes generated from the decay of localized surface plasmons (LSPs) in aluminum nanostructures have significant potential for applications in photocatalysis, photodetection and other optoelectronic devices. Here, we…

光学 · 物理学 2025-11-03 Gengyue Dong , Simão João , Hanwen Jin , Johannes Lischner

Plasmonic nanoparticles hold great promise as photon handling elements and as channels for coherent transfer of energy and information in future all-optical computing devices. Coherent energy oscillations between two spatially separated…

介观与纳米尺度物理 · 物理学 2017-09-13 Eva-Maria Roller , Lucas V. Besteiro , Claudia Pupp , Larousse Khosravi Khorashad , Alexander O. Govorov , Tim Liedl

Hot electrons and holes generated from the decay of localized surface plasmons in metallic nanoparticles can be harnessed for applications in solar energy conversion and sensing. In this paper, we study the generation of hot carriers in…

介观与纳米尺度物理 · 物理学 2024-02-09 Shreyas Ramachandran , Simao Joao , Hanwen Jin , Johannes Lischner

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

介观与纳米尺度物理 · 物理学 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats

Understanding the interplay between illumination and the electron distribution in metallic nanostructures is a crucial step towards developing applications such as plasmonic photo-catalysis for green fuels, nano-scale photo-detection and…

光学 · 物理学 2019-07-23 Yonatan Dubi , Yonatan Sivan
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