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Lithium thiophosphate (LPS) is a promising solid electrolyte for next-generation lithium-ion batteries due to its superior energy storage, high ionic conductivity, and low-flammability components. Despite its potential, the high reactivity…

材料科学 · 物理学 2025-09-23 Hanna Türk , Davide Tisi , Michele Ceriotti

Most organic and inorganic surfaces (e.g., glass, nucleic acids or lipid membranes) become charged in aqueous solutions. The resulting ionic distribution induces effective interactions between the charged surfaces. Stacks of like-charged…

Control of order-disorder phase transitions is a fundamental materials science challenge, underpinning the development of energy storage technologies such as solid oxide fuel cells and batteries, ultra-high temperature ceramics, and durable…

This paper is concerned with the analysis of effective thermomechanical properties of multi- layered materials of interest for solid oxide fuel cells (SOFC) and lithium ions batteries fabrication. The recently developed asymptotic…

材料科学 · 物理学 2016-08-04 A. Bacigalupo , L. Morini , A. Piccolroaz

Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

数值分析 · 数学 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

When a liquid slams into a solid, the intermediate gas is squeezed out at a speed that diverges when approaching the moment of impact. Although there is mounting experimental evidence that instabilities form on the liquid interface during…

流体动力学 · 物理学 2023-06-22 Devaraj van der Meer

Dynamics of the 1D electron transport between two reservoirs are studied based on the inhomogeneous Tomonaga- Luttinger Liquid (ITLL) model in the case when the effect of the electron backscattering on the impurities is negligible. The…

凝聚态物理 · 物理学 2015-06-25 Vadim Ponomarenko

Understanding how to structure a porous electrode to facilitate fluid, mass, and charge transport is key to enhance the performance of electrochemical devices such as fuel cells, electrolyzers, and redox flow batteries (RFBs). Using a…

流体动力学 · 物理学 2024-06-19 Simone Dussi , Chris H. Rycroft

Lithium metal penetrations through the liquid-electrolyte-wetted porous separator and solid electrolytes are a major safety concern of next-generation rechargeable metal batteries. The penetrations were frequently discovered to occur…

应用物理 · 物理学 2020-08-13 Youngju Lee , Bingyuan Ma , Peng Bai

The structures of the liquid surface and the liquid-solid interface of sodium have been characterized with extensive first-principles molecular dynamics simulations. Friedel oscillations in the electronic charge density at the free surface…

材料科学 · 物理学 2007-05-23 Brent G. Walker , Nicola Marzari , Carla Molteni

Lithium metal batteries are seen as a critical piece towards electrifying aviation. During charging, plating of lithium metal, a critical failure mechanism, has been studied and mitigation strategies have been proposed. For electric…

化学物理 · 物理学 2021-03-09 Victor Venturi , Venkatasubramanian Viswanathan

A new era for energy storage devices, such as rechargeable batteries, has been opened in the last decades. However, commercially available energy storage devices are based mainly on critical elements such as Li, Co, Mn, P, Ni, and graphite…

材料科学 · 物理学 2024-11-18 Siripak Sangsinsorn , Sonia Dsoke , Oana Cojocaru-Mirédin

Effect of static charges on charge carrier transport in disordered organic materials is considered. Long range nature of Coulomb interaction requires to take into consideration a finite thickness of the transport layer. Presence of…

无序系统与神经网络 · 物理学 2007-05-23 Sergey Novikov

Generation of thermal convection flow in the liquid metal battery, a device recently proposed as a promising solution for the problem of the short-term energy storage, is analyzed using a numerical model. It is found that convection caused…

流体动力学 · 物理学 2017-01-25 Yuxin Shen , Oleg Zikanov

We introduce a simple and efficient model to describe the potential energy surface of lithium diffusing in a solid-state ionic conductor. First, we assume that the Li atoms are fully ionized and we neglect the weak dependence of the…

材料科学 · 物理学 2019-02-07 Leonid Kahle , Aris Marcolongo , Nicola Marzari

Distributions of potential and lithium content inside lithium ion batteries highly affects their performance and durability. An increased heterogeneity of the lithium distribution is expected in thick electrodes with high energy densities…

We use coarse-grained Monte Carlo simulations to study the elastic properties of charged membranes in solutions of monovalent and pentavalent counterions. The simulation results of the two cases reveal trends opposite to each other. The…

软凝聚态物质 · 物理学 2014-09-12 Yotam Y. Avital , Niels Grønbech-Jensen , Oded Farago

Amorphous organic semiconductors based on small molecules and polymers are used in many applications, most prominently organic light emitting diodes (OLEDs) and organic solar cells. Impurities and charge traps are omnipresent in most…

This paper explores the mechanical behaviour of the composite materials used in modern lithium-ion battery electrodes. These contain relatively high modulus active particle inclusions within a two-component matrix of liquid electrolyte…

计算物理 · 物理学 2024-10-16 J. M. Foster , A. F. Galvis , B. Protas , S. J. Chapman

This work presents a comprehensive study on the aging behavior of 18650-type lithium-ion batteries, focusing on the uneven intercalation of lithium ions during fast charging processes. It introduces a novel approach using color visual…

材料科学 · 物理学 2025-04-17 Yihan Shi , Qingrui Pan , Jitao Li , Xiaoze Shi , Youchang Wang , Peng Xiao
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