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We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

High harmonic spectroscopy has the potential to combine attosecond temporal with sub-Angstrom spatial resolution of the early nuclear and multielectron dynamics in molecules. It involves strong field ionization of the molecule by the IR…

原子物理 · 物理学 2013-08-08 Valeria Serbinenko , Olga Smirnova

Motivated by recent experiments on radiative recombination of two-dimensional electrons in acceptor doped GaAs-AlGaAs heterojunctions as well as the success of a harmonic solid model in describing tunneling between two-dimensional electron…

强关联电子 · 物理学 2016-08-31 S. Kodiyalam , H. A. Fertig , S. Das Sarma

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

原子物理 · 物理学 2008-02-04 Avner Fleischer , Nimrod Moiseyev

Recent advancements in the generation of mid-infrared and terahertz laser pulses have enabled us to observe strong-field driven non-perturbative high-harmonic generation (HHG) from semiconductors, dielectrics, and semimetals. HHG has added…

光学 · 物理学 2022-03-22 M. S. Mrudul

High harmonic spectroscopy can access structural and dynamical information on molecular systems encoded in amplitude and phase of high harmonic generation (HHG) signals4. However, measurement of the harmonic phase is a daunting task. Here…

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

材料科学 · 物理学 2020-12-23 G. P. Zhang , Y. H. Bai

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

量子物理 · 物理学 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

光学 · 物理学 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High-harmonic generation (HHG) from liquids offers a potential pathway to attosecond spectroscopy in chemically complex and disordered environments, yet fundamental questions remain open: whether liquid harmonic emission preserves…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

强关联电子 · 物理学 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…

原子物理 · 物理学 2015-05-28 Elmar V. van der Zwan , Manfred Lein

High-harmonic generation (HHG), the hallmark effect of attosecond science, is a nonperturbative nonlinear process leading to the emission of high-harmonic light from gases and solids. In gases, extreme driving laser pulse intensities can…

We investigate the high-order harmonic generation (HHG) in doped semiconductors. The HHG is simulated with the single-electron time-dependent Schr\"{o}dinger equation (TDSE). The results show that the high-order harmonics in the second…

光学 · 物理学 2017-11-22 Tengfei Huang , Xiaosong Zhu , Liang Li , Xi Liu , Pengfei Lan , Peixiang Lu

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

材料科学 · 物理学 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

We explore with ab-initio theory high harmonic generation (HHG) from a series of gas-phase fullerenes (from C$_{20}$ to C$_{60}$, including isomers) under varying laser conditions (different ellipticities, angular orientations, intensities…

光学 · 物理学 2026-02-27 Km Akanksha Dubey , Ofer Neufeld

High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…

量子物理 · 物理学 2025-07-04 J. Rivera-Dean , P. Stammer , M. F. Ciappina , M. Lewenstein

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

原子物理 · 物理学 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein